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NATURAL RADIOACTIVITY OF SAMARIUM AND NEODYMIUM

Journal Article · · Nature
DOI:https://doi.org/10.1038/185601a0· OSTI ID:4195082
Thin samples containing about 50 mu gm/cm/sup 2/ of natural samarium, 0.3 mu gm/cm/sup 2/ of natural uranium, and 0.5 mu gm/cm/sup 2/ of elemental boron were analyzed in a grid-type ionization chamber in the presence of a thermal nuclear flux of 1.5 x 10/sup 3/ n/cm/sup 2/ obtained from a polonium- beryllium source. The neutrons absorbed by boron gave rise to alpha particles with energies of 1.797 and 1.474 Mev, respectively, which were recorded photographically together with the samarium and uranium alpha particles for the purposes of calibration. By the use of exposures several days long, spectra containing 10/sup 4/ to 10/sup 5/ pulses were obtained and analysed with a spectrophotometer. The result for the alpha energy of saraarium-147 is E = 2.20 plus or minus 0.03 Mev. The specific activity of samarium147 was measured by counting the alpha particles from 28.9 mgm of samarium which were vacuum- evaporated on a source plate of diameter 200 mm. Taking into account self- absorption and back-scattering, a value of 7.00 plus or minus 0.3 counts/min/ mgm of natural samarium is obtained, which corresponds to a half-life of 1.14 plus or minus 0.05 x 10/sup 11/ yr. for the isotope 147. An attempt to detect the natural alpha activity of neodymium was made using a 200-mm source plate on which 36 mgm of neodymium were evaporated. In spite of appreciable thorium contamination a weak line was observed at 2.0 plus or minus 0.1 Mev., inagreement with investigations made by the emulsion method. (auth)
Research Organization:
Univ. of Helsinki
Sponsoring Organization:
USDOE
NSA Number:
NSA-14-009430
OSTI ID:
4195082
Journal Information:
Nature, Journal Name: Nature Vol. Vol: 185
Country of Publication:
Country unknown/Code not available
Language:
English

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