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INFRARED ABSORPTION STUDY OF URANYL SALT SOLUTIONS IN ORGANIC SOLVENTS. I. THE SPECTRA OF COORDINATION BOUND WATER IN HYDRATED URANYL NITRATE IN THE REGION OF VALENCE VIBRATION FREQUENCIES (in Russian)

Journal Article · · Zhur. Fiz. Khim.
OSTI ID:4172870
Measurements were made of the infrared absorption spectra of solutions of hydrated uranyl nitrates (with various isotope modifications of water) in ethyl ether, BETA , BETA 'dichlorodiethyl ether, dipropyl sulphide, acetonitrile, and nitromethane in the region of the OH (OD) valence vibrations. The conclusion was drawn that the water in the coordination sphere of hexa-valent uranium is polarized and that acid-base types of linkages are formed between the hydrate water and the solvent molecules. When an additional number of water molecules is coordinated with the dihydrate of uranyl nitrate they are less firmly bound to uranium than the first two molecules. The acidity of the water coordinated with uranyl nitrate corfirms the comparability of the mechanism of ether extraction for the hydrates of uranyl nitrate, on the one hand, and for acids and metal acid complexes on the other. (tr-auth)
Research Organization:
Originating Research Org. not identified
NSA Number:
NSA-14-013679
OSTI ID:
4172870
Journal Information:
Zhur. Fiz. Khim., Journal Name: Zhur. Fiz. Khim. Vol. Vol: 34
Country of Publication:
Country unknown/Code not available
Language:
Russian

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