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Temperature dependence of electron attachment to methylene chloride

Journal Article · · Journal of Chemical Physics
DOI:https://doi.org/10.1063/1.478820· OSTI ID:348147
 [1];  [2];  [1];  [1]
  1. Oak Ridge National Laboratory, P.O. Box 2008, Oak Ridge, Tennessee 37831-6122 (United States)
  2. Department of Physics, University of Tennessee, Knoxville, Tennessee 37996-1200 (United States)

Temperature dependence of dissociative electron attachment to methylene chloride in the electron energy range of 0{endash}10 eV was studied in a high-temperature electron swarm apparatus. The measurements were made using N{sub 2} and Ar as buffer gases. From the measured electron attachment rate constants, the electron attachment cross sections at 300, 400, and 500 K were determined using an unfolding technique. The maximum electron attachment cross sections at 300, 400, and 500 K were {approx}3.1{times}10{sup {minus}18}, {approx}8.2{times}10{sup {minus}18}, and {approx}1.7{times}10{sup {minus}17} cm{sup 2}, and occurred at electron energies of {approx}0.8, {approx}0.65, and {approx}0.55 eV, respectively. The increase in electron attachment to methylene chloride with temperature is attributed to the increase in the vibrational energy of the molecule. {copyright} {ital 1999 American Institute of Physics.}

OSTI ID:
348147
Journal Information:
Journal of Chemical Physics, Journal Name: Journal of Chemical Physics Journal Issue: 18 Vol. 110; ISSN JCPSA6; ISSN 0021-9606
Country of Publication:
United States
Language:
English

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