Photoelectron–residual-ion interaction in angle-resolved streaked shake-up ionization of helium

Shi, Hongyu; Thumm, Uwe

doi:10.1103/PhysRevA.111.013119

Photoelectron–residual-ion interaction in angle-resolved streaked shake-up ionization of helium

Journal Article · Mon Jan 27 23:00:00 EST 2025 · Physical Review A

DOI:https://doi.org/10.1103/PhysRevA.111.013119· OSTI ID:3003086

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Kansas State Univ., Manhattan, KS (United States)

Streaked photoelectron emission spectra access the correlated dynamics of photoelectrons and residual target electrons with attosecond temporal resolution. Here, we calculated ab initio single-ionization spectra for photoemission from helium atoms by colinearly polarized ultrashort XUV and assisting few-femtosecond IR pulses. Distinguishing direct and shake-up ionization resulting in ground-state and excited (𝑛 = 2, 3) He⁺ residual ions, respectively, we examined the effects of the correlated photoemission dynamics on the photoelectron phase accumulation as a function of the observable photoelectron detection direction and kinetic energy and XUV–IR pulse delay. We tracked the dynamical evolution of the residual ion in relative streaked photo- emission delays and found dominant contributions for shake-up emission from the residual-ion–photoelectron interaction. These are in very good and fair agreement, respectively, for 𝑛 = 2 and 𝑛 = 3 shake-up photoemission along the pulse-polarization directions, with previous experimental and theoretical investigations [Ossiander et al., Nat. Phys. 13, 280 (2017)] and reveal a strong photoemission-direction dependence for shake-up ionization due to the coupling between the photoelectron and evolving residual-ion charge distribution in the IR-laser field.

View Accepted Manuscript (DOE)

Research Organization:: Kansas State Univ., Manhattan, KS (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division (CSGB)

Grant/Contract Number:: FG02-86ER13491

OSTI ID:: 3003086

Journal Information:: Physical Review A, Journal Name: Physical Review A Journal Issue: 1 Vol. 111; ISSN 2469-9934; ISSN 2469-9926

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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