Comparative time-resolved photoemission from the Cu(100) and Cu(111) surfaces

Ambrosio, Marcelo J.; Thumm, Uwe

doi:10.1103/physreva.94.063424

Comparative time-resolved photoemission from the Cu(100) and Cu(111) surfaces

Journal Article · Wed Dec 28 23:00:00 EST 2016 · Physical Review A

DOI:https://doi.org/10.1103/physreva.94.063424· OSTI ID:1535720

Ambrosio, Marcelo J. ^[1]; Thumm, Uwe ^[2]

Kansas State Univ., Manhattan, KS (United States). J.R. Macdonald Lab.; DOE/OSTI
Kansas State Univ., Manhattan, KS (United States). J.R. Macdonald Lab.

Motivated by the striking dependence of the valence electronic structure of transition metal surfaces on their crystallographic orientation, and by emerging experiments on laser-assisted extended ultraviolet (XUV) photoemission from solid surfaces, we calculate photoemission spectra from Cu(100) and Cu(111) surfaces as a function of the photoelectron final kinetic energy and the delay between the ionizing attosecond XUV pulse train and assisting infrared (IR) laser pulse. Our numerical simulations predict distinct differences in delay-dependent photoelectron energy distributions and photoemission time delays for Cu(100) and Cu(111) surfaces. Furthermore, these differences can be scrutinized experimentally with existing technology in a suggested in situ comparative RABBITT (reconstruction of attosecond beating by interference of two-photon transitions) configuration by placing the two surfaces on a sliding platform while keeping all optical components and pathlengths fixed. Our calculations also show that the inclusion of the Fresnel-reflected incident IR pulse at the metal-vacuum interface modifies photoelectron spectra and photoemission time delays in a characteristic way that reveals the degree of spatial location of the initial electronic states.

View Accepted Manuscript (DOE)

Research Organization:: Kansas State Univ., Manhattan, KS (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)

Grant/Contract Number:: FG02-86ER13491

OSTI ID:: 1535720

Alternate ID(s):: OSTI ID: 1338077

Journal Information:: Physical Review A, Journal Name: Physical Review A Journal Issue: 6 Vol. 94; ISSN 2469-9926

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Comparative time-resolved photoemission from the Cu(100) and Cu(111) surfaces

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