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Reconstruction of the complex angle-dependent photoionization transition dipole from a laser-dressed streaking experiment

Journal Article · · Physical Review A
 [1];  [2];  [3];  [2]
  1. Kansas State Univ., Manhattan, KS (United States); DOE/OSTI
  2. Kansas State Univ., Manhattan, KS (United States)
  3. Kansas State Univ., Manhattan, KS (United States); Liaoning Normal Univ., Dalian (China)

We study the retrieval of the angular dependence of the photoionization transition dipole phase of an attosecond XUV pulse in order to reconstruct the whole photoelectron wave packet after the photoemission process. Using a one-electron model Ar atom, we show that the full electron wave packet can be reconstructed from IR-free photoelectron angular distributions and the streaking electron spectra in an IR-dressed XUV photoionization, with photoelectrons along the common polarization direction of the two pulses. The method relies on the validity of the strong-field approximation so it is valid only for higher energy photoelectrons. Here, we also point out that a single photoionization group time delay is not enough to represent a photoemission process; instead, a complete characterization of the electron wave packet requires the retrieval of the spectral phase over the whole bandwidth of the wave packet.

Research Organization:
Kansas State Univ., Manhattan, KS (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Chemical Sciences, Geosciences & Biosciences Division; National Natural Science Foundation of China
Grant/Contract Number:
FG02-86ER13491
OSTI ID:
1610043
Alternate ID(s):
OSTI ID: 1481048
Journal Information:
Physical Review A, Journal Name: Physical Review A Journal Issue: 5 Vol. 98; ISSN PLRAAN; ISSN 2469-9926
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (40)

Attosecond and Strong-Field Physics book January 2018
Attosecond metrology journal November 2001
Time-resolved atomic inner-shell spectroscopy journal October 2002
Attosecond spectroscopy in condensed matter journal October 2007
Electron localization following attosecond molecular photoionization journal June 2010
Following a chemical reaction using high-harmonic interferometry journal July 2010
Reconstruction and control of a time-dependent two-electron wave packet journal December 2014
Direct observation of electron propagation and dielectric screening on the atomic length scale journal January 2015
Calculation of matrix elements for mixed extreme-ultraviolet$ndash$infrared two-photon above-threshold ionization of argon journal August 2002
Empirical formula for static field ionization rates of atoms and molecules by lasers in the barrier-suppression regime journal July 2005
Attosecond delays in photoionization: time and quantum mechanics journal October 2014
Atomic delay in helium, neon, argon and krypton journal December 2014
Angular resolved time delay in photoemission journal December 2014
Volkov transform generalized projection algorithm for attosecond pulse characterization journal July 2016
A new method for accurate retrieval of atomic dipole phase or photoionization group delay in attosecond photoelectron streaking experiments journal October 2017
Lifetime Matrix in Collision Theory journal April 1960
Lower Limit for the Energy Derivative of the Scattering Phase Shift journal April 1955
Frequency-resolved optical gating for complete reconstruction of attosecond bursts journal January 2005
Critical evaluation of attosecond time delays retrieved from photoelectron streaking measurements journal May 2016
Angular dependence of photoemission time delay in helium journal December 2016
Phase-retrieval algorithm for the characterization of broadband single attosecond pulses journal April 2017
Angle-resolved Wigner time delay in atomic photoionization: The 4 d subshell of free and confined Xe journal November 2017
Phase Measurement of Resonant Two-Photon Ionization in Helium journal March 2010
Attosecond Resolved Electron Release in Two-Color Near-Threshold Photoionization of N 2 journal March 2011
Probing Single-Photon Ionization on the Attosecond Time Scale journal April 2011
Attosecond Control in Photoionization of Hydrogen Molecules journal July 2011
Resonance Effects in Photoemission Time Delays journal September 2015
Attosecond Streak Camera journal April 2002
Quantum Theory of Attosecond XUV Pulse Measurement by Laser Dressed Photoionization journal April 2002
Mapping the Dissociative Ionization Dynamics of Molecular Nitrogen with Attosecond Time Resolution journal December 2015
Attosecond chronoscopy of photoemission journal August 2015
Observation of a Train of Attosecond Pulses from High Harmonic Generation journal June 2001
Single-Cycle Nonlinear Optics journal June 2008
Attosecond Ionization and Tunneling Delay Time Measurements in Helium journal December 2008
Delay in Photoemission journal June 2010
Ultrafast electron dynamics in phenylalanine initiated by attosecond pulses journal October 2014
Direct time-domain observation of attosecond final-state lifetimes in photoemission from solids journal June 2016
Attosecond dynamics through a Fano resonance: Monitoring the birth of a photoelectron journal November 2016
Tailoring a 67 attosecond pulse through advantageous phase-mismatch journal January 2012
Energy-dependent photoemission delays from noble metal surfaces by attosecond interferometry journal January 2015

Cited By (4)

Method for spectral phase retrieval of single attosecond pulses utilizing the autocorrelation of photoelectron streaking spectra journal March 2019
Time delays from one-photon transitions in the continuum conference January 2020
Time delays from one-photon transitions in the continuum journal January 2020
Time delays from one-photon transitions in the continuum text January 2020

Figures / Tables (7)


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