Research Progress and Perspectives on Pre‐Sodiation Strategies for Sodium‐Ion Batteries

Lin, Siyuan; Zhang, Haihan; Shu, Chengyong; Hua, Weibo; Wang, Xiaowei; Zhao, Yuxin; Luo, Jintian; Tang, Zexun; Wu, Yuping; Tang, Wei

doi:10.1002/adfm.202409628

Research Progress and Perspectives on Pre‐Sodiation Strategies for Sodium‐Ion Batteries

Journal Article · Mon Aug 12 00:00:00 EDT 2024 · Advanced Functional Materials

DOI:https://doi.org/10.1002/adfm.202409628· OSTI ID:2570355

^[1]; Zhang, Haihan ^[1]; Shu, Chengyong ^[1]; Hua, Weibo ^[1]; Wang, Xiaowei ^[2]; Zhao, Yuxin ^[3]; Luo, Jintian ^[4]; Tang, Zexun ^[5]; Wu, Yuping ^[6]; ^[1]

Xi'an Jiaotong Univ., Shaanxi (China)
Argonne National Laboratory (ANL), Argonne, IL (United States)
CNPC Tubular Goods Research Institute (TGRI) (China)
Guangdong Jiana Energy Technology Co., Ltd. (China)
Hunan Institute of Engineering (China)
Southeast Univ., Nanjing (China)

Sodium‐ion batteries (SIBs) with abundant elements have garnered significant attention from researches as a promise compensation to lithium‐ion batteries (LIBs). However, the large‐scale commercial application of SIBs is partially hindered by the limited initial coulombic efficiency (ICE) due to the irreversible formation of solid electrolyte interphase (SEI) and intercalation into the defects in the anode. Similar to pre‐lithiation techniques, pre‐sodiation approaches are considered to be one of the most direct and effective way to compensate for the loss of active sodium at the anode side of SIBs during the initial cycle. In this context, additional sodium ions are pre‐injected to the cathode/anode material by chemical/electrochemical methods, aiming to improve battery span life and energy density. Here, this review delves into the necessity and impact of pre‐sodiation techniques, compiling the latest research progress, for instance, self‐sacrificing cathode additives, over‐sodiated cathode materials, direct contact and solution chemical pre‐sodiation. Notably, the research mechanisms underlying solution chemical pre‐sodiation are highlighted. This comprehensive overview aims to foster a deeper understanding of the pre‐sodiation techniques and expects to provide guidance for realizing the commercial application of high energy density sodium‐ion batteries.

View Accepted Manuscript (DOE)

Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 2570355

Journal Information:: Advanced Functional Materials, Journal Name: Advanced Functional Materials Journal Issue: 51 Vol. 34; ISSN 1616-301X; ISSN 1616-3028

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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