Surface Passivation to Improve the Performance of Perovskite Solar Cells

Lee, Hayeon; Li, Dawen

doi:10.3390/en17215282

Surface Passivation to Improve the Performance of Perovskite Solar Cells

Journal Article · Thu Oct 24 00:00:00 EDT 2024 · Energies

DOI:https://doi.org/10.3390/en17215282· OSTI ID:2506128

^[1]; Li, Dawen ^[1]

University of Alabama, Tuscaloosa, AL (United States)

Perovskite solar cells (PSCs) suffer from a quick efficiency drop after fabrication, partly due to surface defects, and efficiency can be further enhanced with the passivation of surface defects. Herein, surface passivation is reviewed as a method to improve both the stability and efficiency of PSCs, with an emphasis on the chemical mechanism of surface passivation. Various molecules are utilized as surface passivants, such as halides, Lewis acids and bases, amines (some result in low-dimensional perovskite), and polymers. Multifunctional molecules are a promising group of passivants, as they are capable of passivating multiple defects with various functional groups. This review categorizes these passivants, in addition to considering the potential and limitations of each type of passivant. Additionally, surface passivants for Sn-based PSCs are discussed since this group of PSCs has poor photovoltaic performance compared to their lead-based counterpart due to their severe surface defects. Lastly, future perspectives on the usage of surface passivation as a method to improve the photovoltaic performance of PSCs are addressed to provide a direction for upcoming research and practical applications.

View Accepted Manuscript (DOE)

Research Organization:: University of Alabama, Tuscaloosa, AL (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Renewable Power Office. Solar Energy Technologies Office

Grant/Contract Number:: EE0010242

OSTI ID:: 2506128

Journal Information:: Energies, Journal Name: Energies Journal Issue: 21 Vol. 17; ISSN 1996-1073

Publisher:: MDPICopyright Statement

Country of Publication:: United States

Language:: English

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14 SOLAR ENERGY
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Surface Passivation to Improve the Performance of Perovskite Solar Cells

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