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Defect formation and carrier doping in epitaxial films of the infinite layer compound

Technical Report ·
DOI:https://doi.org/10.2172/219355· OSTI ID:219355
; ;  [1]
  1. Oak Ridge National Lab., TN (United States). Solid State Div.; and others

The correlation between defect formation and carrier doping in epitaxial films of the infinite layer compound SrCuO{sub 2} has been studied via molecular beam epitaxy controlled layer-by-layer growth experiments, chemically resolved scanning transmission electron microscopy, scanning tunneling microscopy, x-ray diffraction, electrical transport measurements, and post-growth oxidation-reduction annealing. Based on the complementary information provided by these experiments, it is concluded that the carrier doping is dominated by the formation of an electron-doped, Sr and O deficient matrix under mildly oxidizing growth conditions. Hole-doping is induced by extended defects containing excess Sr atoms and may lead to superconductivity after high-temperature oxidation.

Research Organization:
Oak Ridge National Lab., TN (United States)
Sponsoring Organization:
USDOE, Washington, DC (United States); Japan Society for the Promotion of Science, Tokyo (Japan); Yamada Science Foundation (Japan)
OSTI ID:
219355
Report Number(s):
CONF-960163--21; ON: DE96008665
Country of Publication:
United States
Language:
English