Effects of chemical bonding on heat transport across interfaces

Losego, Mark D.; Grady, Martha E.; Sottos, Nancy R.; Cahill, David G.; Braun, Paul V.

doi:10.1038/nmat3303

Effects of chemical bonding on heat transport across interfaces

Journal Article · Sun Apr 22 00:00:00 EDT 2012 · Nature Materials

DOI:https://doi.org/10.1038/nmat3303· OSTI ID:1875140

Losego, Mark D. ^[1]; Grady, Martha E. ^[2]; Sottos, Nancy R. ^[2]; Cahill, David G. ^[2]; Braun, Paul V. ^[2]

Univ. of Illinois at Urbana-Champaign, IL (United States); University of Illinois
Univ. of Illinois at Urbana-Champaign, IL (United States)

Interfaces often dictate heat flow in micro- and nanostructured systems. However, despite the growing importance of thermal management in micro- and nanoscale devices, a unified understanding of the atomic-scale structural features contributing to interfacial heat transport does not exist. Herein, we experimentally demonstrate a link between interfacial bonding character and thermal conductance at the atomic level. Our experimental system consists of a gold film transfer-printed to a self-assembled monolayer (SAM) with systematically varied termination chemistries. Using a combination of ultrafast pump–probe techniques (time-domain thermoreflectance, TDTR, and picosecond acoustics) and laser spallation experiments, we independently measure and correlate changes in bonding strength and heat flow at the gold–SAM interface. For example, we experimentally demonstrate that varying the density of covalent bonds within this single bonding layer modulates both interfacial stiffness and interfacial thermal conductance. Here, we believe that this experimental system will enable future quantification of other interfacial phenomena and will be a critical tool to stimulate and validate new theories describing the mechanisms of interfacial heat transport. Ultimately, these findings will impact applications, including thermoelectric energy harvesting, microelectronics cooling, and spatial targeting for hyperthermal therapeutics.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Illinois at Urbana-Champaign, IL (United States)

Sponsoring Organization:: Air Force Office of Scientific Research (AFOSR); National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: FG02-07ER46453; FG02-07ER46471

OSTI ID:: 1875140

Journal Information:: Nature Materials, Journal Name: Nature Materials Journal Issue: 6 Vol. 11; ISSN 1476-1122

Publisher:: Springer NatureCopyright Statement

Country of Publication:: United States

Language:: English

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Length-Dependent Thermal Transport along Molecular Chains Meier, T.; Menges, F.; Nirmalraj, P. Physical Review Letters, Vol. 113, Issue 6 https://doi.org/10.1103/physrevlett.113.060801	journal	August 2014
Study of the effect of adhesion and anharmonicity of atomic vibrations on the thermal conductance of “metal–dielectric” interfaces Slepnev, A. G. Physics of the Solid State, Vol. 59, Issue 7 https://doi.org/10.1134/s1063783417070277	journal	July 2017
Nanophononics: state of the art and perspectives Volz, Sebastian; Ordonez-Miranda, Jose; Shchepetov, Andrey The European Physical Journal B, Vol. 89, Issue 1 https://doi.org/10.1140/epjb/e2015-60727-7	journal	January 2016
Thermal Transport across Solid Interfaces with Nanoscale Imperfections: Effects of Roughness, Disorder, Dislocations, and Bonding on Thermal Boundary Conductance Hopkins, Patrick E. ISRN Mechanical Engineering, Vol. 2013 https://doi.org/10.1155/2013/682586	journal	January 2013
Electron transfer across a thermal gradient Craven, Galen T.; Nitzan, Abraham arXiv https://doi.org/10.48550/arxiv.1607.07010	text	January 2016
Enhanced Thermal Conduction Through Nanostructured Interfaces Park, Woosung; Sood, Aditya; Park, Joonsuk Taylor & Francis https://doi.org/10.6084/m9.figshare.4876790	text	January 2017

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36 MATERIALS SCIENCE
Nanoscale materials
Surfaces
interfaces and thin films

Effects of chemical bonding on heat transport across interfaces

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