Time-domain thermoreflectance

Mohan, Ramya; Khan, Samreen; Wilson, Richard B.; Hopkins, Patrick E.

doi:10.1038/s43586-025-00425-8

Time-domain thermoreflectance

Journal Article · Thu Aug 28 00:00:00 EDT 2025 · Nature Reviews Methods Primers

DOI:https://doi.org/10.1038/s43586-025-00425-8· OSTI ID:2997110

Mohan, Ramya ^[1]; ^[2]; Wilson, Richard B. ^[2]; ^[1]

University of Virginia, Charlottesville, VA (United States)
University of California, Riverside, CA (United States)

Time-domain thermoreflectance (TDTR) has been instrumental in measuring the heat transfer properties of bulk and nanostructured materials over the past two decades. In this Primer, we describe the optical and thermal aspects of TDTR, with an in-depth discussion on the theory, apparatus design and implementation. We present examples that illustrate the ability of TDTR to measure thermal conductivity tensors, thermal conductance across material interfaces, and volumetric heat capacity of thin films, 2D materials and bulk materials. The ability of TDTR to spatially resolve thermal properties is useful for studying heterogeneous material systems, such as materials processed in or subjected to extreme environments. We consider current limitations of pump–probe metrologies and discuss recent advancements of TDTR, such as time-resolved magneto-optic Kerr effect (TR-MOKE), beam-offset TDTR/TR-MOKE, steady-state thermoreflectance, frequency-domain thermoreflectance and laser-flash TDTR. Lastly, we present an outlook on anticipated technological developments to further expand the ability of TDTR to measure nanoscale thermal properties.

View Accepted Manuscript (DOE)

Research Organization:: The Pennsylvania State University, University Park, PA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0021118; SC0021230

OSTI ID:: 2997110

Journal Information:: Nature Reviews Methods Primers, Journal Name: Nature Reviews Methods Primers Journal Issue: 1 Vol. 5; ISSN 2662-8449

Publisher:: Springer Science and Business Media LLCCopyright Statement

Country of Publication:: United States

Language:: English

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