Deep Eutectic Solvents: A Review of Fundamentals and Applications

Hansen, Benworth B.; Spittle, Stephanie; Chen, Brian; Poe, Derrick; Zhang, Yong; Klein, Jeffrey M.; Horton, Alexandre; Adhikari, Laxmi; Zelovich, Tamar; Doherty, Brian W.; Gurkan, Burcu; Maginn, Edward J.; Ragauskas, Arthur; Dadmun, Mark; Zawodzinski, Thomas A.; Baker, Gary A.; Tuckerman, Mark E.; Savinell, Robert F.; Sangoro, Joshua R.

doi:10.1021/acs.chemrev.0c00385

Deep Eutectic Solvents: A Review of Fundamentals and Applications

Journal Article · Mon Dec 14 00:00:00 EST 2020 · Chemical Reviews

DOI:https://doi.org/10.1021/acs.chemrev.0c00385· OSTI ID:1808446

Hansen, Benworth B. ^[1]; Spittle, Stephanie ^[2]; ^[3]; Poe, Derrick ^[4]; ^[4]; ^[3]; Horton, Alexandre ^[2]; ^[5]; ^[6]; ^[6]; ^[3]; ^[4]; ^[2]; ^[2]; ^[2]; ^[5]; ^[6]; ^[3]; ^[2]

Univ. of Tennessee, Knoxville, TN (United States); The University of Tennessee Knoxville
Univ. of Tennessee, Knoxville, TN (United States)
Case Western Reserve Univ., Cleveland, OH (United States)
Univ. of Notre Dame, IN (United States)
Univ. of Missouri, Columbia, MO (United States)
New York Univ. (NYU), NY (United States)

Deep eutectic solvents (DESs) are an emerging class of mixtures characterized by significant depressions in melting points compared to those of the neat constituent components. These green materials are promising for applications as inexpensive ’designer’ solvents exhibiting a host of tunable physicochemical properties. Here, a detailed review of the current literature reveals the lack of predictive understanding of the microscopic mechanisms that govern the structure-property relationships in this class of solvents. Complex hydrogen bonding behavior is postulated as the root cause of their melt-ing point depressions and physicochemical properties; to understand these hydrogen bonded networks, it is imperative to study these systems as dynamic entities using both simulations and experiments. This review emphasizes recent research efforts in order to elucidate the next steps needed to develop a fundamental framework for understanding DESs. It covers recent developments in DES research, frames outstanding scientific questions, and identifies gainful research thrusts that would advance the field towards predictive models and fundamental understanding of these solvents.

View Accepted Manuscript (DOE)

Research Organization:: Case Western Reserve Univ., Cleveland, OH (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0019409

OSTI ID:: 1808446

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 3 Vol. 121; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Characterization and Modeling of the Liquid Phase of Deep Eutectic Solvents Based on Fatty Acids/Alcohols and Choline Chloride Crespo, Emanuel A.; Silva, Liliana P.; Martins, Mónia A. R. Industrial & Engineering Chemistry Research, Vol. 56, Issue 42 https://doi.org/10.1021/acs.iecr.7b02382	journal	October 2017
The Role of Polyfunctionality in the Formation of [Ch]Cl-Carboxylic Acid-Based Deep Eutectic Solvents Crespo, Emanuel A.; Silva, Liliana P.; Martins, Mónia A. R. Industrial & Engineering Chemistry Research, Vol. 57, Issue 32 https://doi.org/10.1021/acs.iecr.8b01249	journal	July 2018
Surface Tension of 50 Deep Eutectic Solvents: Effect of Hydrogen-Bonding Donors, Hydrogen-Bonding Acceptors, Other Solvents, and Temperature Chen, Yu; Chen, Wenjun; Fu, Li Industrial & Engineering Chemistry Research, Vol. 58, Issue 28 https://doi.org/10.1021/acs.iecr.9b00867	journal	June 2019
Surface Tension of Tricyanomethanide- and Tetracyanoborate-Based Imidazolium Ionic Liquids by Using the Pendant Drop Method Koller, Thomas M.; Rausch, Michael H.; Pohako-Esko, Kaija Journal of Chemical & Engineering Data, Vol. 60, Issue 9 https://doi.org/10.1021/acs.jced.5b00303	journal	July 2015
Physical Properties of the Pure Deep Eutectic Solvent, [ChCl]:[Lev] (1:2) DES, and Its Binary Mixtures with Alcohols Sas, Olalla González; Fidalgo, Rubén; Domínguez, Irene Journal of Chemical & Engineering Data, Vol. 61, Issue 12 https://doi.org/10.1021/acs.jced.6b00563	journal	October 2016
Molar Enthalpy of Mixing for Choline Chloride/Urea Deep Eutectic Solvent + Water System Ma, Chunyan; Guo, Yanhua; Li, Dongxue Journal of Chemical & Engineering Data, Vol. 61, Issue 12 https://doi.org/10.1021/acs.jced.6b00569	journal	October 2016
Viscosities and Carbon Dioxide Solubilities of Guanidine Carbonate and Malic Acid-Based Eutectic Solvents Mirza, Nouman R.; Nicholas, Nathan J.; Wu, Yue Journal of Chemical & Engineering Data, Vol. 62, Issue 1 https://doi.org/10.1021/acs.jced.6b00680	journal	November 2016
Carbon Dioxide Solubilities in Decanoic Acid-Based Hydrophobic Deep Eutectic Solvents Zubeir, Lawien F.; van Osch, Dannie J. G. P.; Rocha, Marisa A. A. Journal of Chemical & Engineering Data, Vol. 63, Issue 4 https://doi.org/10.1021/acs.jced.7b00534	journal	March 2018
Effect of Ethylene, Diethylene, and Triethylene Glycols and Glycerol on the Physicochemical Properties and Phase Behavior of Benzyltrimethyl and Benzyltributylammonium Chloride Based Deep Eutectic Solvents at 283.15–343.15 K Basaiahgari, Anusha; Panda, Somenath; Gardas, Ramesh L. Journal of Chemical & Engineering Data, Vol. 63, Issue 7 https://doi.org/10.1021/acs.jced.8b00213	journal	March 2018
From Molecular Fragments to the Bulk: Development of a Neural Network Potential for MOF-5 Eckhoff, Marco; Behler, Jörg Journal of Chemical Theory and Computation, Vol. 15, Issue 6 https://doi.org/10.1021/acs.jctc.8b01288	journal	April 2019
Subpicosecond Solvation Response and Partial Viscosity Decoupling of Solute Diffusion in Ionic Acetamide Deep Eutectic Solvents: Fluorescence Up-Conversion and Fluorescence Correlation Spectroscopic Measurements Subba, Navin; Tarif, Ejaj; Sen, Pratik The Journal of Physical Chemistry B, Vol. 124, Issue 10 https://doi.org/10.1021/acs.jpcb.0c00061	journal	February 2020
Complete Solvation Dynamics of Coumarin 153 in Tetraalkylammonium Bromide-Based Deep Eutectic Solvents Hossain, Sk Saddam; Paul, Sneha; Samanta, Anunay The Journal of Physical Chemistry B, Vol. 124, Issue 12 https://doi.org/10.1021/acs.jpcb.0c00594	journal	March 2020
From Salt in Solution to Solely Ions: Solvation of Methyl Viologen in Deep Eutectic Solvents and Ionic Liquids Klein, Jeffrey M.; Squire, Henry; Dean, William The Journal of Physical Chemistry B, Vol. 124, Issue 29 https://doi.org/10.1021/acs.jpcb.0c03296	journal	June 2020
Liquid Structure and Transport Properties of the Deep Eutectic Solvent Ethaline Zhang, Yong; Poe, Derrick; Heroux, Luke The Journal of Physical Chemistry B, Vol. 124, Issue 25 https://doi.org/10.1021/acs.jpcb.0c04058	journal	May 2020
Combined Small-Angle Neutron Scattering, Diffusion NMR, and Molecular Dynamics Study of a Eutectogel: Illuminating the Dynamical Behavior of Glyceline Confined in Bacterial Cellulose Gels Smith, Chip J.; Wagle, Durgesh V.; Bhawawet, Nakara The Journal of Physical Chemistry B, Vol. 124, Issue 35 https://doi.org/10.1021/acs.jpcb.0c04916	journal	August 2020
Dynamic Solvent Control of a Reaction in Ionic Deep Eutectic Solvents: Time-Resolved Fluorescence Measurements of Reactive and Nonreactive Dynamics in (Choline Chloride + Urea) Melts Das, Anuradha; Biswas, Ranjit The Journal of Physical Chemistry B, Vol. 119, Issue 31 https://doi.org/10.1021/acs.jpcb.5b04936	journal	July 2015
Nanoscale Spatial Heterogeneity in Deep Eutectic Solvents Kaur, Supreet; Gupta, Aditya; Kashyap, Hemant K. The Journal of Physical Chemistry B, Vol. 120, Issue 27 https://doi.org/10.1021/acs.jpcb.6b04187	journal	June 2016
Improved Force Field Model for the Deep Eutectic Solvent Ethaline: Reliable Physicochemical Properties Ferreira, Elisabete S. C.; Voroshylova, Iuliia V.; Pereira, Carlos M. The Journal of Physical Chemistry B, Vol. 120, Issue 38 https://doi.org/10.1021/acs.jpcb.6b07233	journal	September 2016
Resilience of Malic Acid Natural Deep Eutectic Solvent Nanostructure to Solidification and Hydration Hammond, Oliver S.; Bowron, Daniel T.; Jackson, Andrew J. The Journal of Physical Chemistry B, Vol. 121, Issue 31 https://doi.org/10.1021/acs.jpcb.7b05454	journal	July 2017
Solute Rotation and Translation Dynamics in an Ionic Deep Eutectic Solvent Based on Choline Chloride Hossain, Sk Saddam; Samanta, Anunay The Journal of Physical Chemistry B, Vol. 121, Issue 46 https://doi.org/10.1021/acs.jpcb.7b08472	journal	November 2017
Proton-Coupled Electron Transfer and Substituent Effects in Catechol-Based Deep Eutectic Solvents: Gross and Fine Tuning of Redox Activity Smith, Parker J.; Goeltz, John C. The Journal of Physical Chemistry B, Vol. 121, Issue 48 https://doi.org/10.1021/acs.jpcb.7b10169	journal	November 2017
First-Principles Molecular Dynamics Study of a Deep Eutectic Solvent: Choline Chloride/Urea and Its Mixture with Water Fetisov, Evgenii O.; Harwood, David B.; Kuo, I-Feng William The Journal of Physical Chemistry B, Vol. 122, Issue 3 https://doi.org/10.1021/acs.jpcb.7b10422	journal	January 2018
Glycerol Hydrogen-Bonding Network Dominates Structure and Collective Dynamics in a Deep Eutectic Solvent Faraone, A.; Wagle, D. V.; Baker, G. A. The Journal of Physical Chemistry B, Vol. 122, Issue 3 https://doi.org/10.1021/acs.jpcb.7b11224	journal	January 2018
Unusual Temperature Dependence of Nanoscale Structural Organization in Deep Eutectic Solvents Kaur, Supreet; Kashyap, Hemant K. The Journal of Physical Chemistry B, Vol. 122, Issue 20 https://doi.org/10.1021/acs.jpcb.8b02378	journal	April 2018
OPLS Force Field for Choline Chloride-Based Deep Eutectic Solvents Doherty, Brian; Acevedo, Orlando The Journal of Physical Chemistry B, Vol. 122, Issue 43 https://doi.org/10.1021/acs.jpcb.8b06647	journal	August 2018
Solvation Structure and Dynamics of Li ⁺ in Ternary Ionic Liquid–Lithium Salt Electrolytes Huang, Qianwen; Lourenço, Tuanan C.; Costa, Luciano T. The Journal of Physical Chemistry B, Vol. 123, Issue 2 https://doi.org/10.1021/acs.jpcb.8b08859	journal	December 2018
Photophysical Behavior and Fluorescence Quenching of l -Tryptophan in Choline Chloride-Based Deep Eutectic Solvents Kadyan, Anu; Juneja, Shreya; Pandey, Siddharth The Journal of Physical Chemistry B, Vol. 123, Issue 35 https://doi.org/10.1021/acs.jpcb.9b04659	journal	August 2019
Liquid Structure and Dynamics of Tetraalkylammonium Bromide-Based Deep Eutectic Solvents: Effect of Cation Chain Length Hossain, Sk Saddam; Paul, Sneha; Samanta, Anunay The Journal of Physical Chemistry B, Vol. 123, Issue 31 https://doi.org/10.1021/acs.jpcb.9b04955	journal	July 2019
Interaction and Dynamics in a Fully Biodegradable Glucose-Containing Naturally Abundant Deep Eutectic Solvent: Temperature-Dependent Time-Resolved Fluorescence Measurements Tarif, Ejaj; Mondal, Jayanta; Biswas, Ranjit The Journal of Physical Chemistry B, Vol. 123, Issue 44 https://doi.org/10.1021/acs.jpcb.9b06783	journal	October 2019
Structural and Dynamical Properties of a Deep Eutectic Solvent Confined Inside a Slit Pore Shen, Yan; He, Xiaoxia; Hung, Francisco R. The Journal of Physical Chemistry C, Vol. 119, Issue 43 https://doi.org/10.1021/acs.jpcc.5b08172	journal	October 2015
Nanostructure of Deep Eutectic Solvents at Graphite Electrode Interfaces as a Function of Potential Chen, Zhengfei; McLean, Ben; Ludwig, Michael The Journal of Physical Chemistry C, Vol. 120, Issue 4 https://doi.org/10.1021/acs.jpcc.5b10624	journal	January 2016
Structure and Dynamics of the Liquid–Water/Zinc-Oxide Interface from Machine Learning Potential Simulations Quaranta, Vanessa; Behler, Jörg; Hellström, Matti The Journal of Physical Chemistry C, Vol. 123, Issue 2 https://doi.org/10.1021/acs.jpcc.8b10781	journal	December 2018
Liquid–Liquid Phase Transition and Its Phase Diagram in Deeply-Cooled Heavy Water Confined in a Nanoporous Silica Matrix Wang, Zhe; Ito, Kanae; Leão, Juscelino B. The Journal of Physical Chemistry Letters, Vol. 6, Issue 11 https://doi.org/10.1021/acs.jpclett.5b00827	journal	May 2015
Differential Microscopic Mobility of Components within a Deep Eutectic Solvent Wagle, Durgesh V.; Baker, Gary A.; Mamontov, Eugene The Journal of Physical Chemistry Letters, Vol. 6, Issue 15 https://doi.org/10.1021/acs.jpclett.5b01192	journal	July 2015
Proton Transport in Imidazoles: Unraveling the Role of Supramolecular Structure Cosby, Tyler; Holt, Adam; Griffin, Philip J. The Journal of Physical Chemistry Letters, Vol. 6, Issue 19 https://doi.org/10.1021/acs.jpclett.5b01887	journal	September 2015
Accurate Probabilities for Highly Activated Reaction of Polyatomic Molecules on Surfaces Using a High-Dimensional Neural Network Potential: CHD ₃ + Cu(111) Gerrits, N.; Shakouri, Khosrow; Behler, Jörg The Journal of Physical Chemistry Letters, Vol. 10, Issue 8 https://doi.org/10.1021/acs.jpclett.9b00560	journal	March 2019
Aggregation of Carbocyanine Dyes in Choline Chloride-Based Deep Eutectic Solvents in the Presence of an Aqueous Base Pal, Mahi; Yadav, Anita; Pandey, Siddharth Langmuir, Vol. 33, Issue 38 https://doi.org/10.1021/acs.langmuir.7b01981	journal	August 2017
Deep Eutectic Solvent-Induced Structural Transition of Microemulsions Explored with Small-Angle X-ray Scattering Sakuragi, Mina; Tsutsumi, Shinsuke; Kusakabe, Katsuki Langmuir, Vol. 34, Issue 42 https://doi.org/10.1021/acs.langmuir.8b02565	journal	September 2018
On the Performance of Confined Deep Eutectic Solvents and Ionic Liquids for Separations of Carbon Dioxide from Methane: Molecular Dynamics Simulations Shen, Yan; Abedin, Rubaiyet; Hung, Francisco R. Langmuir, Vol. 35, Issue 10 https://doi.org/10.1021/acs.langmuir.8b03990	journal	February 2019
Sugar-Based Natural Deep Eutectic Mixtures as Green Intercalating Solvents for High-Yield Preparation of Stable MoS ₂ Nanosheets: Application to Electrocatalysis of Hydrogen Evolution Reaction Mohammadpour, Zahra; Abdollahi, Seyyed Hossein; Safavi, Afsaneh ACS Applied Energy Materials, Vol. 1, Issue 11 https://doi.org/10.1021/acsaem.8b00838	journal	October 2018
Novel Deep-Eutectic-Solvent-Infused Carbon Nanofiber Networks as High Power Density Green Battery Cathodes Kawase, Koki; Abe, Jyunichiro; Tenjimbayashi, Mizuki ACS Applied Materials & Interfaces, Vol. 10, Issue 18 https://doi.org/10.1021/acsami.8b03099	journal	April 2018
Batch and Flow Nanomanufacturing of Large Quantities of Colloidal Silver and Gold Nanocrystals Using Deep Eutectic Solvents Adhikari, Laxmi; Larm, Nathaniel E.; Baker, Gary A. ACS Sustainable Chemistry & Engineering, Vol. 8, Issue 39 https://doi.org/10.1021/acssuschemeng.0c04244	journal	September 2020
Tuning Task-Specific Ionic Liquids for the Extractive Desulfurization of Liquid Fuel Zhao, Hua; Baker, Gary A.; Wagle, Durgesh V. ACS Sustainable Chemistry & Engineering, Vol. 4, Issue 9 https://doi.org/10.1021/acssuschemeng.6b00972	journal	August 2016
Characterization of Lignin Streams during Bionic Liquid-Based Pretreatment from Grass, Hardwood, and Softwood Dutta, Tanmoy; Papa, Gabriella; Wang, Eileen ACS Sustainable Chemistry & Engineering, Vol. 6, Issue 3 https://doi.org/10.1021/acssuschemeng.7b02991	journal	January 2018
Rapid Microwave-Assisted Synthesis of Silver Nanoparticles in a Halide-Free Deep Eutectic Solvent Adhikari, Laxmi; Larm, Nathaniel E.; Bhawawet, Nakara ACS Sustainable Chemistry & Engineering, Vol. 6, Issue 5 https://doi.org/10.1021/acssuschemeng.8b00050	journal	February 2018
Quantum Chemical Evaluation of Deep Eutectic Solvents for the Extractive Desulfurization of Fuel Wagle, Durgesh V.; Zhao, Hua; Deakyne, Carol A. ACS Sustainable Chemistry & Engineering, Vol. 6, Issue 6 https://doi.org/10.1021/acssuschemeng.8b00224	journal	March 2018
Tunable Hydrophobic Eutectic Solvents Based on Terpenes and Monocarboxylic Acids Martins, Mónia A. R.; Crespo, Emanuel A.; Pontes, Paula V. A. ACS Sustainable Chemistry & Engineering, Vol. 6, Issue 7 https://doi.org/10.1021/acssuschemeng.8b01203	journal	May 2018
Design and Characterization of Sugar-Based Deep Eutectic Solvents Using Conductor-like Screening Model for Real Solvents Silva, Liliana P.; Fernandez, Luis; Conceição, João H. F. ACS Sustainable Chemistry & Engineering, Vol. 6, Issue 8 https://doi.org/10.1021/acssuschemeng.8b02042	journal	June 2018
A Search for Natural Hydrophobic Deep Eutectic Solvents Based on Natural Components van Osch, Dannie J. G. P.; Dietz, Carin H. J. T.; van Spronsen, Jaap ACS Sustainable Chemistry & Engineering, Vol. 7, Issue 3 https://doi.org/10.1021/acssuschemeng.8b03520	journal	January 2019
Efficient and Selective Extraction of ^99m TcO ₄ ^– from Aqueous Media Using Hydrophobic Deep Eutectic Solvents Phelps, Tim E.; Bhawawet, Nakara; Jurisson, Silvia S. ACS Sustainable Chemistry & Engineering, Vol. 6, Issue 11 https://doi.org/10.1021/acssuschemeng.8b03950	journal	October 2018
Determination of the Total Vapor Pressure of Hydrophobic Deep Eutectic Solvents: Experiments and Perturbed-Chain Statistical Associating Fluid Theory Modeling Dietz, Carin H. J. T.; Creemers, Jeremy T.; Meuleman, Merijn A. ACS Sustainable Chemistry & Engineering, Vol. 7, Issue 4 https://doi.org/10.1021/acssuschemeng.8b05449	journal	January 2019
Probing the Environmental Toxicity of Deep Eutectic Solvents and Their Components: An In Silico Modeling Approach Halder, Amit Kumar; Cordeiro, M. Natália D. S. ACS Sustainable Chemistry & Engineering, Vol. 7, Issue 12 https://doi.org/10.1021/acssuschemeng.9b01306	journal	May 2019
Argentous Deep Eutectic Solvent Approach for Scaling Up the Production of Colloidal Silver Nanocrystals Adhikari, Laxmi; Larm, Nathaniel E.; Baker, Gary A. ACS Sustainable Chemistry & Engineering, Vol. 7, Issue 13 https://doi.org/10.1021/acssuschemeng.9b01777	journal	May 2019
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Mesoscale modeling of hydrated morphologies of sulfonated polysulfone ionomers Wang, Chen; Paddison, Stephen J. Soft Matter, Vol. 10, Issue 6 https://doi.org/10.1039/C3SM52330F	journal	January 2014
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Enhanced extraction of bioactive natural products using tailor-made deep eutectic solvents: application to flavonoid extraction from Flos sophorae Nam, Min Woo; Zhao, Jing; Lee, Min Sang Green Chemistry, Vol. 17, Issue 3 https://doi.org/10.1039/C4GC01556H	journal	January 2015
A detailed study of cholinium chloride and levulinic acid deep eutectic solvent system for CO ₂ capture via experimental and molecular simulation approaches Ullah, Ruh; Atilhan, Mert; Anaya, Baraa Physical Chemistry Chemical Physics, Vol. 17, Issue 32 https://doi.org/10.1039/C5CP03364K	journal	January 2015
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Significantly improving the solubility of non-steroidal anti-inflammatory drugs in deep eutectic solvents for potential non-aqueous liquid administration Lu, Chao; Cao, Jun; Wang, Ning MedChemComm, Vol. 7, Issue 5 https://doi.org/10.1039/C5MD00551E	journal	January 2016
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Hybrid green nonaqueous media: tetraethylene glycol modifies the properties of a (choline chloride + urea) deep eutectic solvent Kadyan, Anu; Behera, Kamalakanta; Pandey, Siddharth RSC Advances, Vol. 6, Issue 36 https://doi.org/10.1039/C6RA03726G	journal	January 2016
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Excited-state dynamics of mononucleotides and DNA strands in a deep eutectic solvent Zhang, Yuyuan; de La Harpe, Kimberly; Hariharan, Mahesh Faraday Discussions, Vol. 207 https://doi.org/10.1039/C7FD00205J	journal	January 2018
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A green and efficient method for the synthesis of pyrroles using a deep eutectic solvent ([CholineCl][ZnCl ₂ ] ₃ ) under solvent-free sonication Truong Nguyen, Hai; Nguyen Chau, Duy-Khiem; Tran, Phuong Hoang New J. Chem., Vol. 41, Issue 21 https://doi.org/10.1039/C7NJ02396K	journal	January 2017
Ammonium based stabilizers effectively counteract urea-induced denaturation in a small protein: insights from molecular dynamics simulations Sarkar, Soham; Ghosh, Soumadwip; Chakrabarti, Rajarshi RSC Advances, Vol. 7, Issue 83 https://doi.org/10.1039/C7RA10712A	journal	January 2017
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Multiple hydrogen bond coordination in three-constituent deep eutectic solvents enhances lignin fractionation from biomass Xia, Qinqin; Liu, Yongzhuang; Meng, Juan Green Chemistry, Vol. 20, Issue 12 https://doi.org/10.1039/C8GC00900G	journal	January 2018
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Natural solvent-assisted synthesis of amphiphilic co-polymeric nanomicelles for prolonged release of camptothecin delivery Pradeepkumar, Periyakaruppan; Elgorban, Abdallah Mohamed; Bahkali, Ali Hassan New Journal of Chemistry, Vol. 42, Issue 12 https://doi.org/10.1039/C8NJ00901E	journal	January 2018
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Environmentally Friendly Approach to Knoevenagel Condensation of Rhodanine in Choline Chloride: Urea Deep Eutectic Solvent and QSAR Studies on Their Antioxidant Activity Molnar, Maja; Brahmbhatt, Harshad; Rastija, Vesna Molecules, Vol. 23, Issue 8 https://doi.org/10.3390/molecules23081897	journal	July 2018
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Electrodeposition from Deep Eutectic Solvents Bernasconi, R.; Panzeri, G.; Accogli, A. Progress and Developments in Ionic Liquids https://doi.org/10.5772/64935	book	February 2017

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