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Hydrocarbons and carbon monoxide in the atmosphere of Mexico city

Journal Article · · Journal of the Air and Waste Management Association
; ;  [1];  [2];  [3]
  1. Universidad Nacional Autonoma de Mexico, Mexico City (Mexico)
  2. Instituto Nacional de Ecologia, Mexico City (Mexico)
  3. Servicio LOA, Mexico City (Mexico)

In Mexico City, the use and composition of fuels determine that carbon monoxide (CO) comes mostly from mobile sources, and sulfur dioxide (SO{sub 2}) from fixed and mobile sources. By simultaneously measuring hydrocarbons (HC), CO, and SO{sub 2} in the atmosphere of Mexico City, the relative amounts coming from different sources can be estimated. Assuming that some HC are emitted proportionally to CO emissions, we can establish that [HC]{sub 1} = m1{center_dot}[CO], where the proportionality constant m1 corresponds to the ratio of emissions factor for HC and CO in mobile sources. Similarly for fuels containing sulfur, it can be assumed that [HC]{sub 2} = m2{center_dot}[SO{sub 2}]. In this way, the total HC are [HC]{sub total}= [HC]{sub 0} +m1{center_dot}[CO]+m2{center_dot}[SO{sub 2}], where [HC]{sub 0}, corresponds mainly to other sources like solvent evaporation, gas consumption, and natural emissions. In this way, it can be estimated that in Mexico City 75% of average HC comes from mobile sources, 5% from sulfur-related sources, and 19% from natural sources and solvent evaporation. Compared with the HC/CO ratio measured in the exhaust pipe of vehicles, we estimated that 70% of HC emitted from mobile sources are evaporative losses, and only 30% come through the exhaust system. 26 refs., 7 figs., 3 tabs.

Sponsoring Organization:
USDOE
OSTI ID:
171472
Journal Information:
Journal of the Air and Waste Management Association, Journal Name: Journal of the Air and Waste Management Association Journal Issue: 12 Vol. 45; ISSN JAWAEB; ISSN 1047-3289
Country of Publication:
United States
Language:
English

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