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Atomically Abrupt Topological p–n Junction

Journal Article · · ACS Nano
 [1];  [2];  [3];  [4];  [5];  [3];  [1]
  1. Inst. for Basic Science, Pohang (Korea, Republic of); Pohang Univ. of Science and Technology (POSTECH) (Korea, Republic of)
  2. Univ. of Utah, Salt Lake City, UT (United States)
  3. Pohang Univ. of Science and Technology (POSTECH) (Korea, Republic of). Dept. of Physics
  4. Pohang Univ. of Science and Technology (POSTECH) (Korea, Republic of). Pohang Accelerator Lab.
  5. Univ. of Utah, Salt Lake City, UT (United States); Collaborative Innovation Center of Quantum Matter, Beijing (China)
Topological insulators (TI’s) are a new class of quantum matter with extraordinary surface electronic states, which bear great potential for spintronics and error-tolerant quantum computing. In order to put a TI into any practical use, these materials need to be fabricated into devices whose basic units are often p–n junctions. Interesting electronic properties of a ‘topological’ p–n junction were proposed theoretically such as the junction electronic state and the spin rectification. However, the fabrication of a lateral topological p–n junction has been challenging because of materials, process, and fundamental reasons. Here, we demonstrate an innovative approach to realize a p–n junction of topological surface states (TSS’s) of a three-dimensional (3D) topological insulator (TI) with an atomically abrupt interface. When a ultrathin Sb film is grown on a 3D TI of Bi2Se3 with a typical n-type TSS, the surface develops a strongly p-type TSS through the substantial hybridization between the 2D Sb film and the Bi2Se3 surface. Thus, the Bi2Se3 surface covered partially with Sb films bifurcates into areas of n- and p-type TSS’s as separated by atomic step edges with a lateral electronic junction of as short as 2 nm. This approach opens a different avenue toward various electronic and spintronic devices based on well-defined topological p–n junctions with the scalability down to atomic dimensions.
Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). National Energy Research Scientific Computing Center (NERSC)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)
Grant/Contract Number:
FG02-04ER46148
OSTI ID:
1487451
Journal Information:
ACS Nano, Journal Name: ACS Nano Journal Issue: 10 Vol. 11; ISSN 1936-0851
Publisher:
American Chemical Society (ACS)Copyright Statement
Country of Publication:
United States
Language:
English

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A 2D nonsymmorphic Dirac semimetal in a chemically modified group-VA monolayer with a black phosphorene structure journal January 2019
Anisotropic electronic structure of antimonene journal November 2019
Recovery of surface state bands after desorption of Te capping layer on (Bi 1− x Sb x ) 2 Te 3 ternary topological insulators journal September 2019
Fabry–Perot interferometry in Weyl semi-metals journal December 2018
Spintronic signatures of Klein tunneling in topological insulators journal November 2017