Nonlinear Pauli susceptibilities in Sr3Ru2O7 and universal features of itinerant metamagnetism

Shivaram, B. S.; Luo, Jing; Chern, Gia-Wei; Phelan, Daniel; Fittipaldi, R.; Vecchione, A.

doi:10.1103/PhysRevB.97.100403

Nonlinear Pauli susceptibilities in ${Sr}_{3} {Ru}_{2} O_{7}$ and universal features of itinerant metamagnetism

Journal Article · Mon Mar 12 00:00:00 EDT 2018 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.97.100403· OSTI ID:1426769

Shivaram, B. S. ^[1]; Luo, Jing ^[1]; Chern, Gia-Wei ^[1]; Phelan, Daniel ^[2]; Fittipaldi, R. ^[3]; Vecchione, A. ^[3]

Univ. of Virginia, Charlottesville, VA (United States)
Argonne National Lab. (ANL), Argonne, IL (United States)
Univ. di Salerno (Italy)

We report, for the first time, measurements of the third order, x₃ and fifth order, x₅, susceptibilities in an itinerant oxide metamagnet, Sr₃Ru₂O₇ for magnetic fields both parallel and perpendicular to the c-axis. These susceptibilities exhibit maxima in their temperature dependence such that T₁ ≈ 2T₃ ≈ 4T₅ where the T_i are the position in temperature where a peak in the i-th order susceptibility occurs. These features taken together with the scaling of the critical field with the temperature T₁ observed in a diverse variety of itinerant metamagnets find a natural explanation in a single band model with one Van Hove singularity (VHS) and onsite repulsion U. The separation of the VHS from the Fermi energy V, sets a single energy scale, which is the primary driver for the observed features of itinerant metamagnetism at low temperatures.

View Accepted Manuscript (DOE)

Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1426769

Journal Information:: Physical Review B, Journal Name: Physical Review B Journal Issue: 10 Vol. 97; ISSN 2469-9950; ISSN PRBMDO

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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