Itinerant G-type antiferromagnetic order in SrCr2As2

Das, Pinaki; Sangeetha, N. S.; Lindemann, George R.; Heitmann, T. W.; Kreyssig, Andreas; Goldman, Alan I.; McQueeney, Robert J.; Johnston, David C.; Vaknin, David

doi:10.1103/PhysRevB.96.014411

Itinerant G-type antiferromagnetic order in ${SrCr}_{2} {As}_{2}$

Journal Article · Fri Jul 07 00:00:00 EDT 2017 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.96.014411· OSTI ID:1374740

Das, Pinaki ^[1]; Sangeetha, N. S. ^[1]; Lindemann, George R. ^[1]; Heitmann, T. W. ^[2]; Kreyssig, Andreas ^[1]; Goldman, Alan I. ^[1]; McQueeney, Robert J. ^[1]; Johnston, David C. ^[1]; Vaknin, David ^[1]

Ames Lab. and Iowa State Univ., Ames, IA (United States)
Univ. of Missouri, Columbia, MO (United States)

Here, neutron-diffraction and magnetic susceptibility studies of polycrystalline SrCr₂As₂ reveal that this compound is an itinerant G-type antiferromagnet below the Néel temperature T_N = 590(5) K with the Cr magnetic moments aligned along the tetragonal c axis. The system remains tetragonal to the lowest measured temperature (~12 K). The lattice parameter ratio c/a and the magnetic moment saturate at about the same temperature below ~200 K, indicating a possible magnetoelastic coupling. The ordered moment μ = 1.9(1)μ_B/Cr, measured at T = 12 K, is significantly reduced compared to its localized value (4μ_B/Cr) due to the itinerant character brought about by hybridization between the Cr 3d and As 4p orbitals.

View Accepted Manuscript (DOE)

Research Organization:: Ames Lab. (AMES), Ames, IA (United States)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-07CH11358

OSTI ID:: 1374740

Alternate ID(s):: OSTI ID: 1368612

Report Number(s):: IS-J--9412

Journal Information:: Physical Review B, Journal Name: Physical Review B Journal Issue: 1 Vol. 96; ISSN 2469-9950; ISSN PRBMDO

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

References (40)

Superconductivity in quasi-one-dimensional Cs2Cr3As3 with large interchain distance Tang, Zhang-Tu; Bao, Jin-Ke; Wang, Zhen Science China Materials, Vol. 58, Issue 1 https://doi.org/10.1007/s40843-015-0021-x	journal	January 2015
Recent advances in magnetic structure determination by neutron powder diffraction Rodríguez-Carvajal, Juan Physica B: Condensed Matter, Vol. 192, Issue 1-2 https://doi.org/10.1016/0921-4526(93)90108-I	journal	October 1993
Spin fluctuations in iron pnictides and chalcogenides: From antiferromagnetism to superconductivity Inosov, Dmytro S. Comptes Rendus Physique, Vol. 17, Issue 1-2 https://doi.org/10.1016/j.crhy.2015.03.001	journal	January 2016
Frustrated magnetic interactions, giant magneto–elastic coupling, and magnetic phonons in iron–pnictides Yildirim, Taner Physica C: Superconductivity, Vol. 469, Issue 9-12 https://doi.org/10.1016/j.physc.2009.03.038	journal	May 2009
Iron-based superconductors: Current status of materials and pairing mechanism Hosono, Hideo; Kuroki, Kazuhiko Physica C: Superconductivity and its Applications, Vol. 514 https://doi.org/10.1016/j.physc.2015.02.020	journal	July 2015
High-temperature superconductivity in iron pnictides and chalcogenides Si, Qimiao; Yu, Rong; Abrahams, Elihu Nature Reviews Materials, Vol. 1, Issue 4 https://doi.org/10.1038/natrevmats.2016.17	journal	March 2016
Superconductivity in the vicinity of antiferromagnetic order in CrAs Wu, Wei; Cheng, Jinguang; Matsubayashi, Kazuyuki Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms6508	journal	November 2014
What drives nematic order in iron-based superconductors? Fernandes, R. M.; Chubukov, A. V.; Schmalian, J. Nature Physics, Vol. 10, Issue 2 https://doi.org/10.1038/nphys2877	journal	January 2014
The puzzle of high temperature superconductivity in layered iron pnictides and chalcogenides Johnston, David C. Advances in Physics, Vol. 59, Issue 6 https://doi.org/10.1080/00018732.2010.513480	journal	October 2010
Relation between the specific heat and susceptibility of an antiferromagnet Fisher, Michael E. Philosophical Magazine, Vol. 7, Issue 82 https://doi.org/10.1080/14786436208213705	journal	October 1962
Collinear antiferromagnetism in trigonal SrMn ₂ As ₂ revealed by single-crystal neutron diffraction Das, Pinaki; Sangeetha, N. S.; Pandey, Abhishek Journal of Physics: Condensed Matter, Vol. 29, Issue 3 https://doi.org/10.1088/0953-8984/29/3/035802	journal	November 2016
Antiferromagnetism in ( Ca 0.85 Sr 0.15 ) CuO 2 , the parent of the cuprate family of superconducting compounds Vaknin, D.; Caignol, E.; Davies, P. K. Physical Review B, Vol. 39, Issue 13 https://doi.org/10.1103/PhysRevB.39.9122	journal	May 1989
Lattice collapse and quenching of magnetism in CaFe 2 As 2 under pressure: A single-crystal neutron and x-ray diffraction investigation Goldman, A. I.; Kreyssig, A.; Prokeš, K. Physical Review B, Vol. 79, Issue 2 https://doi.org/10.1103/PhysRevB.79.024513	journal	January 2009
Electronic structure and magnetism in BaMn 2 As 2 and BaMn 2 Sb 2 An, Jiming; Sefat, A. S.; Singh, D. J. Physical Review B, Vol. 79, Issue 7 https://doi.org/10.1103/PhysRevB.79.075120	journal	February 2009
Itinerant antiferromagnetism in BaCr 2 As 2 : Experimental characterization and electronic structure calculations Singh, D. J.; Sefat, A. S.; McGuire, M. A. Physical Review B, Vol. 79, Issue 9 https://doi.org/10.1103/PhysRevB.79.094429	journal	March 2009
Magnetic, transport, and thermal properties of single crystals of the layered arsenide BaMn 2 As 2 Singh, Yogesh; Ellern, A.; Johnston, D. C. Physical Review B, Vol. 79, Issue 9 https://doi.org/10.1103/PhysRevB.79.094519	journal	March 2009
Magnetic and lattice coupling in single-crystal SrFe 2 As 2 : A neutron scattering study Li, Haifeng; Tian, Wei; Zarestky, Jerel L. Physical Review B, Vol. 80, Issue 5 https://doi.org/10.1103/PhysRevB.80.054407	journal	August 2009
Magnetic order in BaMn 2 As 2 from neutron diffraction measurements Singh, Yogesh; Green, M. A.; Huang, Q. Physical Review B, Vol. 80, Issue 10 https://doi.org/10.1103/PhysRevB.80.100403	journal	September 2009
Magnetic exchange interactions in BaMn 2 As 2 : A case study of the J 1 - J 2 - J c Heisenberg model Johnston, D. C.; McQueeney, R. J.; Lake, B. Physical Review B, Vol. 84, Issue 9 https://doi.org/10.1103/PhysRevB.84.094445	journal	September 2011
Optical properties of the iron-pnictide analog BaMn 2 As 2 Antal, A.; Knoblauch, T.; Singh, Y. Physical Review B, Vol. 86, Issue 1 https://doi.org/10.1103/PhysRevB.86.014506	journal	July 2012
Crystal and magnetic structure of CaCo 1.86 As 2 studied by x-ray and neutron diffraction Quirinale, D. G.; Anand, V. K.; Kim, M. G. Physical Review B, Vol. 88, Issue 17 https://doi.org/10.1103/PhysRevB.88.174420	journal	November 2013
Magnetic structure and spin excitations in BaMn 2 Bi 2 Calder, S.; Saparov, B.; Cao, H. B. Physical Review B, Vol. 89, Issue 6 https://doi.org/10.1103/PhysRevB.89.064417	journal	February 2014
Itinerant and local-moment magnetism in EuCr 2 As 2 single crystals Paramanik, U. B.; Prasad, R.; Geibel, C. Physical Review B, Vol. 89, Issue 14 https://doi.org/10.1103/PhysRevB.89.144423	journal	April 2014
Unconventional superconductivity in quasi-one-dimensional Rb 2 Cr 3 As 3 Tang, Zhang-Tu; Bao, Jin-Ke; Liu, Yi Physical Review B, Vol. 91, Issue 2 https://doi.org/10.1103/PhysRevB.91.020506	journal	January 2015
Pressure-induced collapsed-tetragonal phase in SrCo 2 As 2 Jayasekara, W. T.; Kaluarachchi, U. S.; Ueland, B. G. Physical Review B, Vol. 92, Issue 22 https://doi.org/10.1103/PhysRevB.92.224103	journal	December 2015
Magnetic structures of the Eu and Cr moments in EuCr 2 As 2 : Neutron diffraction study Nandi, S.; Xiao, Y.; Qureshi, N. Physical Review B, Vol. 94, Issue 9 https://doi.org/10.1103/PhysRevB.94.094411	journal	September 2016
Strong magnetic correlations to 900 K in single crystals of the trigonal antiferromagnetic insulators SrMn 2 As 2 and CaMn 2 As 2 Sangeetha, N. S.; Pandey, Abhishek; Benson, Zackery A. Physical Review B, Vol. 94, Issue 9 https://doi.org/10.1103/PhysRevB.94.094417	journal	September 2016
Angle-resolved photoemission observation of Mn-pnictide hybridization and negligible band structure renormalization in BaMn 2 As 2 and BaMn 2 Sb 2 Zhang, W. -L.; Richard, P.; van Roekeghem, A. Physical Review B, Vol. 94, Issue 15 https://doi.org/10.1103/PhysRevB.94.155155	journal	October 2016
Pressure-induced transition to the collapsed tetragonal phase in BaC r 2 A s 2 Naumov, P. G.; Filsinger, K.; Barkalov, O. I. Physical Review B, Vol. 95, Issue 14 https://doi.org/10.1103/PhysRevB.95.144106	journal	April 2017
Antiferromagnetic structure and electronic properties of BaCr 2 As 2 and BaCrFeAs 2 Filsinger, Kai A.; Schnelle, Walter; Adler, Peter Physical Review B, Vol. 95, Issue 18 https://doi.org/10.1103/PhysRevB.95.184414	journal	May 2017
Is BaCr 2 As 2 symmetrical to BaFe 2 As 2 with respect to half 3 d shell filling? Richard, P.; van Roekeghem, A.; Lv, B. Q. Physical Review B, Vol. 95, Issue 18 https://doi.org/10.1103/PhysRevB.95.184516	journal	May 2017
Anisotropy, Itineracy, and Magnetic Frustration in High- T C Iron Pnictides Han, Myung Joon; Yin, Quan; Pickett, Warren E. Physical Review Letters, Vol. 102, Issue 10 https://doi.org/10.1103/PhysRevLett.102.107003	journal	March 2009
Superconductivity in Quasi-One-Dimensional K 2 Cr 3 As 3 with Significant Electron Correlations Bao, Jin-Ke; Liu, Ji-Yong; Ma, Cong-Wei Physical Review X, Vol. 5, Issue 1 https://doi.org/10.1103/PhysRevX.5.011013	journal	February 2015
Superconductivity in iron compounds Stewart, G. R. Reviews of Modern Physics, Vol. 83, Issue 4 https://doi.org/10.1103/RevModPhys.83.1589	journal	December 2011
A common thread: The pairing interaction for unconventional superconductors Scalapino, D. J. Reviews of Modern Physics, Vol. 84, Issue 4 https://doi.org/10.1103/RevModPhys.84.1383	journal	October 2012
Colloquium : The unexpected properties of alkali metal iron selenide superconductors Dagotto, Elbio Reviews of Modern Physics, Vol. 85, Issue 2 https://doi.org/10.1103/RevModPhys.85.849	journal	May 2013
Antiferromagnetic order and spin dynamics in iron-based superconductors Dai, Pengcheng Reviews of Modern Physics, Vol. 87, Issue 3 https://doi.org/10.1103/RevModPhys.87.855	journal	August 2015
Zur Struktur ternärer Übergangsmetallarsenide/On the Structure of Ternary Arsenides Pfisterer, Martin; Nagorsen, Günter Zeitschrift für Naturforschung B, Vol. 35, Issue 6 https://doi.org/10.1515/znb-1980-0611	journal	June 1980
Bindungsverhältnisse und magnetische Eigenschaften ternärer Arsenide ET2As2 / Bonding and Magnetic Properties in Ternary Arsenides ET2As2 Pfisterer, Martin; Nagorsen, Günter Zeitschrift für Naturforschung B, Vol. 38, Issue 7 https://doi.org/10.1515/znb-1983-0704	journal	July 1983
Superconductivity of 2.2 K under Pressure in Helimagnet CrAs Kotegawa, Hisashi; Nakahara, Shingo; Tou, Hideki Journal of the Physical Society of Japan, Vol. 83, Issue 9 https://doi.org/10.7566/JPSJ.83.093702	journal	September 2014

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Prediction of antiferromagnetism in barium chromium phosphide confirmed after synthesis Jishi, R. A.; Rodriguez, J. P.; Haugan, T. J. Journal of Physics: Condensed Matter, Vol. 32, Issue 2 https://doi.org/10.1088/1361-648x/ab45dc	journal	October 2019
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