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Photon energy conversion by near-zero permittivity nonlinear materials

Patent ·
OSTI ID:1414408
Efficient harmonic light generation can be achieved with ultrathin films by coupling an incident pump wave to an epsilon-near-zero (ENZ) mode of the thin film. As an example, efficient third harmonic generation from an indium tin oxide nanofilm (.lamda./42 thick) on a glass substrate for a pump wavelength of 1.4 .mu.m was demonstrated. A conversion efficiency of 3.3.times.10.sup.-6 was achieved by exploiting the field enhancement properties of the ENZ mode with an enhancement factor of 200. This nanoscale frequency conversion method is applicable to other plasmonic materials and reststrahlen materials in proximity of the longitudinal optical phonon frequencies.
Research Organization:
Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC04-94AL85000
Assignee:
National Technology & Engineering Solutions of Sandia, LLC (Albuquerque, NM)
Patent Number(s):
9,846,348
Application Number:
15/040,799
OSTI ID:
1414408
Country of Publication:
United States
Language:
English

References (6)

Berreman mode and epsilon near zero mode journal January 2012
Directional perfect absorption using deep subwavelength low-permittivity films journal August 2014
Enhanced third harmonic generation from the epsilon-near-zero modes of ultrathin films journal April 2015
Singularity-driven second- and third-harmonic generation at ε-near-zero crossing points journal December 2011
Harmonic generation in multiresonant plasma films journal October 2013
Electric field enhancement in ɛ-near-zero slabs under TM-polarized oblique incidence journal January 2013

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