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U.S. Department of Energy
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Chemical and spectroscopic studies of metal oxide surfaces

Conference ·
OSTI ID:126281
 [1]
  1. Texas A & M Univ., College Station, TX (United States)

A new approach to the study of oxide surfaces will be described. Thin oxide films ({approximately} 100{Angstrom}) of SiO{sub 2}, Al{sub 2}O{sub 3}, NiO, and MgO supported on a refractory metal substrate (e.g., Mo or W) have been prepared by depositing the oxide metal precursor in a background of oxygen (ca. 1x10{sup -5} Tort). These thin-film oxide samples facilitate investigation by an array of surface techniques, including high resolution electron energy loss spectroscopy (HREELS) and infrared reflection absorption spectroscopy (IRAS). In addition, the growth of small Cu and Pd particles, prepared by vacuum vapor deposition, on alumina and silica films have been studied. Nitric oxide decomposition and reaction with carbon monoxide on the Cu and Pd particles has been investigated using TPD, HREELS, IRAS. These systems will be compared with respect to their special chemistry for the CO/NO reaction.

OSTI ID:
126281
Report Number(s):
CONF-950402--
Country of Publication:
United States
Language:
English