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The {sup 194}Os/{sup 194}Ir generator: Production and purification of {sup 194}Os

Conference ·
OSTI ID:10120231

Iridium-194 (t{sub {1/2}} = 19.15 h) decays by {beta}-particle emission (E{sub {beta}}{sup max} = 2.236 MeV) and is a potential candidate for radioimmunotherapy [1,2]. An important characteristic is availability of carrier-free {sup 194}Ir from {beta}-decay of {sup 194}Os (t{sub {1/2}} = 6 y). The {sup 194}Os parent nuclei is produced in a fission nuclear reactor with double neutron capture on {sup 192}Os (41.0% natural abundance). We report here the preliminary nuclear data for production of {sup 194}OS and discuss the feasibility of producing sufficient quantities of {sup 194}Os required for the fabrication of the large-scale generators for further studies. In addition, we describe a novel gas- thermochromatographic method (GTC) for the one step conversion of metallic Os to OsO{sub 4} and subsequent separation and purification of OsO{sub 4}. 6 refs., 1 fig., 1 tab.

Research Organization:
Oak Ridge National Lab., TN (United States)
Sponsoring Organization:
USDOE, Washington, DC (United States)
DOE Contract Number:
AC05-84OR21400
OSTI ID:
10120231
Report Number(s):
CONF-920418--3-Extd.Abst.; ON: DE92007235
Country of Publication:
United States
Language:
English