Dual-step photocarrier injection by mixture layer of ZnO QDs and MoS2 NPs on hybrid PdAu NPs

Mandavkar, Rutuja; Lin, Shusen; Kulkarni, Rakesh; Burse, Shalmali; Habib, Md Ahasan; Kunwar, Sundar; Lee, Jihoon

doi:10.1016/j.materresbull.2022.111832

Title: Dual-step photocarrier injection by mixture layer of ZnO QDs and MoS₂ NPs on hybrid PdAu NPs

Journal Article · Mon Mar 21 00:00:00 EDT 2022 · Materials Research Bulletin

DOI:https://doi.org/10.1016/j.materresbull.2022.111832· OSTI ID:1995150

Mandavkar, Rutuja ^[1]; Lin, Shusen ^[1];

^[1]; Burse, Shalmali ^[1];

^[1];

^[2]; Lee, Jihoon ^[1]

Kwangwoon Univ., Seoul (Korea, Republic of)
Kwangwoon Univ., Seoul (Korea, Republic of); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States). Center for Integrated Nanotechnologies (CINT)

Hybrid UV-photodetector (PD) design consisted of various compatible nano-material systems are drawing significant research interests due to their improved device tunability and functionality. A hybrid ZnO–MoS₂/HNP UV-PD design is demonstrated by the mixture layer of zinc oxide (ZnO) quantum dot (QD) and molybdenum di-sulfate (MoS₂) nanoparticles (NPs) on the plasmonic hybrid PdAu NP template. The proposed design exhibits an excellent photocurrent of 1.45×10^-3 A under the 54.9 mW/mm2 at ± 10 V due to a dual step enhancement of photo-carrier injection. It then leads to the significantly improved performance factors of photo-responsivity 1430 mA/mm² and detectivity 4.50 × 10¹⁰ jones at 0.34 mW/mm². The rise time (T_r) and fall time (T_f) of 3.37 and 0.35 s are obtained for the ZnO–MoS₂/HNP PD. Finally, the demonstrated performance factors indicate that the hybrid ZnO–MoS₂/HNP UV-PD platform is one of the best UV-PDs as summarized in Table 1.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA); USDOE Laboratory Directed Research and Development (LDRD) Program; National Research Foundation of Korea (NRF)

Grant/Contract Number:: 89233218CNA000001; NRF-2019R1A2C4069438; NRF-2018R1A6A1A03025242

OSTI ID:: 1995150

Report Number(s):: LA-UR-22-25124

Journal Information:: Materials Research Bulletin, Vol. 151; ISSN 0025-5408

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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36 MATERIALS SCIENCE
Material Science
Dual-step photocarrier injection
UV photodetectors
ZnO QDsMoS2 NPs
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FDTD simulation

Title: Dual-step photocarrier injection by mixture layer of ZnO QDs and MoS2 NPs on hybrid PdAu NPs

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References (49)

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Title: Dual-step photocarrier injection by mixture layer of ZnO QDs and MoS₂ NPs on hybrid PdAu NPs