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Title: The effects of ACRT on melt undercooling during the growth of CZT via the traveling heater method: Ekman versus Taylor-Görtler flows

Journal Article · · Journal of Crystal Growth
ORCiD logo [1];  [2]
  1. Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Univ. of Minnesota, Minneapolis, MN (United States)
  2. Univ. of Minnesota, Minneapolis, MN (United States)

For the first time, a comprehensive model for the traveling heater method, including detailed species transport and phase-change thermodynamics, is applied to understand the effects of accelerated crucible rotation (ACRT) on the growth of cadmium zinc telluride. Here, a rotation schedule that is designed from classical considerations does not completely mix the melt, rather undercooled regions of localized melt are swept periodically across the growth interface. Even without melt homogenization, these ACRT-driven flows disrupt the persistent undercooling that occurs during THM growth without rotation. An ACRT schedule designed to promote Ekman flows results in lower levels of melt undercooling than a schedule designed to promote Taylor-Görtler flows and greater mixing.

Research Organization:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA); National Science Foundation (NSF)
Grant/Contract Number:
89233218CNA000001; DMR-10007885
OSTI ID:
1829662
Report Number(s):
LA-UR-21-29740
Journal Information:
Journal of Crystal Growth, Vol. 577; ISSN 0022-0248
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (39)

Effect of accelerated crucible rotation on melt composition in high-pressure vertical Bridgman growth of cadmium zinc telluride journal February 2000
Transition in circular Couette flow journal March 1965
Flux growth of large crystals by accelerated crucible-rotation technique journal March 1971
Bridgman growth of Cdx Hg1-xTe using acrt journal November 1986
Interfaces and flow regimes in ACRT grown CdxHg1−xTe crystals journal June 1988
The role of accelerated crucible rotation in the growth of Hg1−xCdxTe and CdTe/CdZnTe journal January 1994
Accelerated crucible rotation: Hydrodynamics and stirring effect journal February 1972
Phase-Field Study of the Cellular Bifurcation in Dilute Binary Alloys journal May 2007
Controlling Te inclusion during direct mixed solution growth of large size CdZnTe crystal conference September 2018
Growth and characterization of CdTe single crystals for radiation detectors
  • Funaki, Minoru; Ozaki, Tsutomu; Satoh, Kazuyuki
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 436, Issue 1-2, p. 120-126 https://doi.org/10.1016/S0168-9002(99)00607-5
journal October 1999
Growth and interface study of 2in diameter CdZnTe by THM technique journal September 2010
Controlling nucleation during unseeded THM growth of CdZnTe crystal journal March 2020
A fundamental limitation on growth rates in the traveling heater method journal October 2016
Application of the accelerated crucible rotation technique to the Bridgman growth of CdxHg1− xTe: Simulations and crystal growth journal December 1984
Growth of CdZnTe crystals by the traveling heater method journal September 2013
Towards optimization of ACRT schedules applied to the gradient freeze growth of cadmium zinc telluride journal December 2017
Buoyancy and rotation in small-scale vertical Bridgman growth of cadmium zinc telluride using accelerated crucible rotation journal December 2001
P-T-X phase equilibrium and vapor pressure scanning of non-stoichiometry in CdTe journal April 1996
Analysis of the traveling heater method for the growth of cadmium telluride journal November 2016
LIX. On convection currents in a horizontal layer of fluid, when the higher temperature is on the under side journal December 1916
Effects of ampoule rotation on vertical zone-melting crystal growth: steady rotation versus accelerated crucible rotation technique (ACRT) journal May 1999
Effects of cycle patterns of accelerated crucible rotation technique (ACRT) on the flows, interface, and segregation in vertical Bridgman crystal growth journal December 2007
ACRT: A review of models journal January 1986
Growth of large, high purity, low cost, uniform CdZnTe crystals by the “cold travelling heater method” journal April 1994
Characterization of detector-grade CdZnTe crystals grown by traveling heater method (THM) journal February 2010
Phase-field simulations and geometrical characterization of cellular solidification fronts journal January 2014
Stability of a Planar Interface During Solidification of a Dilute Binary Alloy journal February 1964
Numerical analysis on Hg1−xCdxTe growth by ACRT-VBM journal February 2000
Analysis of the accelerated crucible rotation technique applied to the gradient freeze growth of cadmium zinc telluride journal June 2017
Growth interface of CdZnTe grown from Te solution with THM technique under static magnetic field journal November 2005
Effect of ACRT rotation parameters on Bridgman grown CdxHg1−xTe crystals journal April 1989
Modification of growth interface of CdZnTe crystals in THM process by ACRT journal February 2018
Optimizing ACRT to reduce inclusion formation during the VGF growth of cadmium zinc telluride: II. Application to experiments journal December 2021
The redistribution of solute atoms during the solidification of metals journal July 1953
A numerical study of convection during THM growth of CdTe with ACRT journal October 1997
Numerical analysis of Cd1−xZnxTe crystal growth by the vertical Bridgman method using the accelerated crucible rotation technique journal October 2000
Bridgman growth and assessment of CdTe and CdZnTe using the accelerated crucible rotation technique journal January 1993
Growth and Characterization of Detector-Grade Cd0.9Zn0.1Te Crystals by the Traveling Heater Method with the Accelerated Crucible Rotation Technique journal October 2017
Centrifugal instabilities during spin-down to rest in finite cylinders. Numerical experiments journal January 1981