Robust long-range magnetic correlation across antiphase domain boundaries in Sr2CrReO6

Yuan, Bo; Kim, Subin; Chun, Sae Hwan; Jin, Wentao; Nelson, Christie S.; Hauser, Adam J.; Yang, F. Y.; Kim, Young-June

doi:10.1103/physrevb.103.064410

Title: Robust long-range magnetic correlation across antiphase domain boundaries in Sr₂CrReO₆

Journal Article · Fri Feb 05 00:00:00 EST 2021 · Physical Review B

DOI:https://doi.org/10.1103/physrevb.103.064410· OSTI ID:1771137

^[1]; Kim, Subin ^[1]; Chun, Sae Hwan ^[1]; Jin, Wentao ^[2]; Nelson, Christie S. ^[3];

^[4]; Yang, F. Y. ^[5]; Kim, Young-June ^[1]

Univ. of Toronto, ON (Canada)
Beihang Univ., Beijing (China)
Brookhaven National Lab. (BNL), Upton, NY (United States). National Synchrotron Light Source II (NSLS-II)
Univ. of Alabama, Tuscaloosa, AL (United States)
The Ohio State Univ., Columbus, OH (United States)

Here, we report a resonant elastic x-ray scattering study of a thin-film sample of Sr₂CrReO₆, which has one of the highest ferrimagnetic transition temperatures among ordered double perovskites.We found resonantly enhanced magnetic Bragg peaks at Q = (odd, odd, odd) at both the rhenium L₂ and L₃ edges, which coincide with the structural Bragg peaks of Sr₂CrReO₆. By analyzing the widths of these Bragg peaks, we extracted very different structural and magnetic correlation lengths. The former is about 15 nm, while the latter is constrained by the instrumental resolution to be at least 90 nm. We argue that a finite structural correlation length is consistent with the existence of antiphase nanodomains in our sample. On the other hand, a much larger magnetic correlation length indicates that the magnetic correlation extends far beyond the boundaries of individual domains and is consistent with strong antiferromagnetic coupling between different antiphase domains. Last, from the azimuthal dependence of the magnetic intensity, we show that the magnetic moments lie perpendicular to the c axis, which explains the earlier bulk magnetization data.

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Research Organization:: Brookhaven National Lab. (BNL), Upton, NY (United States). National Synchrotron Light Source II (NSLS-II)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); Natural Sciences and Engineering Research Council of Canada (NSERC); Canada Foundation for Innovation (CFI); Ontario Research Fund (ORF); National Science Foundation (NSF)

Grant/Contract Number:: SC0012704; DMR-2011876

OSTI ID:: 1771137

Report Number(s):: BNL-221144-2021-JAAM; TRN: US2206889

Journal Information:: Physical Review B, Vol. 103, Issue 6; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Title: Robust long-range magnetic correlation across antiphase domain boundaries in Sr₂CrReO₆