skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Modeling strategy for progressive failure prediction in lithium-ion batteries under mechanical abuse

Journal Article · · eTransportation
 [1];  [1];  [2];  [1];  [3]; ORCiD logo [2]
  1. Hunan University, Changsha (China)
  2. Northwestern Polytechnical University (China)
  3. National Renewable Energy Lab. (NREL), Golden, CO (United States)

The prediction for the internal failure of lithium-ion batteries (LIBs) under external mechanical abuse loading remains a challenge for safe design. This paper systematically studies the modeling approach for progressive failure simulation and short-circuit prediction. Hemispherical indentation experiments are conducted on a battery specimen containing 5 representative sandwich (RS) layers to examine the deformation and progressive failure behavior of battery components. Three different models, viz, a high-fidelity detailed model, an intermediate homogenized model and a fully homogenized model, are developed and employed to simulate the progressive failure in a multi-layer battery specimen. The simulation results obtained using the three models all correlate well with experimental phenomena, capturing the overall stress-strain response and ultimate failure of the battery structure. The numerical results can help us understand the failure behavior and the mechanism for mechanical abuse-induced short circuit in LIBs. The feasibility of the three models for use in progressive failure prediction is compared by analyzing the capability of the models in predicting the critical failure events, the computational efficiency of the models, and the feasibility to implement coupled mechanical-electrochemical-thermal simulations. The results of this work provide useful insights on practical choices for the modeling strategy and safety design of LIBs under mechanical abuse conditions.

Research Organization:
National Renewable Energy Lab. (NREL), Golden, CO (United States)
Sponsoring Organization:
USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Vehicle Technologies Office
Grant/Contract Number:
AC36-08GO28308
OSTI ID:
1764943
Report Number(s):
NREL/JA-5700-76871; MainId:10515; UUID:13ee0818-5c9b-4542-8e4b-458efb045aca; MainAdminID:19295
Journal Information:
eTransportation, Vol. 7; ISSN 2590-1168
Publisher:
ElsevierCopyright Statement
Country of Publication:
United States
Language:
English

References (35)

Computational model of 18650 lithium-ion battery with coupled strain rate and SOC dependencies journal June 2016
Dynamic impact tests on lithium-ion cells journal October 2017
Coupled mechanical-electrical-thermal modeling for short-circuit prediction in a lithium-ion cell under mechanical abuse journal September 2015
Progressive mechanical indentation of large-format Li-ion cells journal February 2017
Characterizing and modeling mechanical properties and onset of short circuit for three types of lithium-ion pouch cells journal February 2014
Mechanical testing and macro-mechanical finite element simulation of the deformation, fracture, and short circuit initiation of cylindrical Lithium ion battery cells journal September 2012
Safety issues and mechanisms of lithium-ion battery cell upon mechanical abusive loading: A review journal January 2020
Homogenized mechanical properties for the jellyroll of cylindrical Lithium-ion cells journal November 2013
Calibration and finite element simulation of pouch lithium-ion batteries for mechanical integrity journal March 2012
Internal configuration of prismatic lithium-ion cells at the onset of mechanically induced short circuit journal February 2016
Dynamic impact response of lithium-ion batteries, constitutive properties and failure model journal January 2019
Impact of Tab Location on Large Format Lithium-Ion Pouch Cell Based on Fully Coupled Tree-Dimensional Electrochemical-Thermal Modeling journal November 2014
Communication—Multi-Physics battery Safety Simulations across Length Scales journal January 2019
Thermal runaway mechanism of lithium ion battery for electric vehicles: A review journal January 2018
Coupled effect of strain rate and solvent on dynamic mechanical behaviors of separators in lithium ion batteries journal April 2016
Effect of packaging and cooling plates on mechanical response and failure characteristics of automotive Li-ion battery modules journal November 2018
Mechanical behavior of representative volume elements of lithium-ion battery cells under compressive loading conditions journal January 2014
A comparative investigation of aging effects on thermal runaway behavior of lithium-ion batteries journal November 2019
A representative-sandwich model for simultaneously coupled mechanical-electrical-thermal simulation of a lithium-ion cell under quasi-static indentation tests journal December 2015
Modelling of cracks developed in lithium-ion cells under mechanical loading journal January 2015
State of Charge Dependent Mechanical Integrity Behavior of 18650 Lithium-ion Batteries journal February 2016
Strain distribution and failure mode of polymer separators for Li-ion batteries under biaxial loading journal February 2018
A detailed computational model for cylindrical lithium-ion batteries under mechanical loading: From cell deformation to short-circuit onset journal February 2019
Modeling extreme deformations in lithium ion batteries journal May 2020
Safety assessment of electrically cycled cells at high temperatures under mechanical crush loads journal November 2020
Constitutive behavior and progressive mechanical failure of electrodes in lithium-ion batteries journal July 2017
Microscale failure mechanisms leading to internal short circuit in Li-ion batteries under complex loading scenarios journal July 2016
Deformation and failure of lithium-ion batteries treated as a discrete layered structure journal October 2019
Data-Driven Safety Envelope of Lithium-Ion Batteries for Electric Vehicles journal November 2019
Mechanical behavior of representative volume elements of lithium-ion battery modules under various loading conditions journal February 2014
Coupled Mechanical–Electrochemical–Thermal Study on the Short-Circuit Mechanism of Lithium-Ion Batteries under Mechanical Abuse journal August 2020
Features of mechanical behavior of EV battery modules under high deformation rate journal October 2019
Computational models for simulations of lithium-ion battery cells under constrained compression tests journal November 2013
Dynamic mechanical integrity of cylindrical lithium-ion battery cell upon crushing journal July 2015
Deformation and failure characteristics of four types of lithium-ion battery separators journal September 2016