Measurement of the sound velocity and Grüneisen parameter of polystyrene at inertial confinement fusion conditions

McCoy, C. A.; Hu, S. X.; Marshall, M. C.; Polsin, D. N.; Fratanduono, D. E.; Ding, Y. H.; Celliers, P. M.; Boehly, T. R.; Meyerhofer, D. D.

doi:10.1103/physrevb.102.184102

Title: Measurement of the sound velocity and Grüneisen parameter of polystyrene at inertial confinement fusion conditions

Journal Article · Thu Nov 05 00:00:00 EST 2020 · Physical Review B

DOI:https://doi.org/10.1103/physrevb.102.184102· OSTI ID:1714353

^[1];

^[2]; Marshall, M. C. ^[2]; Polsin, D. N. ^[2]; Fratanduono, D. E. ^[3]; Ding, Y. H. ^[2];

^[3]; Boehly, T. R. ^[2];

^[4]

Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Univ. of Rochester, NY (United States). Lab. for Laser Energetics
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

The principal Hugoniot, sound velocity, and Grüneisen parameter of polystyrene were measured at conditions relevant to shocks in inertial confinement fusion implosions, from 100 to 1000 GPa. The sound velocity is in good agreement with quantum molecular dynamics calculations and all tabular equation of state models at pressures below 200 GPa. Above 200 GPa, the experimental results agree with two of the examined tables, but do not agree with the most recent table developed for design of ICF experiments. The Grüneisen parameter increases with density below ~3.1 g/cm³ and approaches the asymptotic value for an ideal gas after complete dissociation. This behavior is in good agreement with quantum molecular dynamics results and previous work but is not represented by any of the tabular models. Finally, the discrepancy between tabular models and experimental measurement of the sound velocity and Grüneisen parameter is sufficient to impact simulations of ICF experiments.

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Research Organization:: Univ. of Rochester, NY (United States). Lab. for Laser Energetics; Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: NA0003856; AC04-94AL85000; AC52-07NA27344

OSTI ID:: 1714353

Alternate ID(s):: OSTI ID: 1721620; OSTI ID: 1867107

Report Number(s):: 2020-243,1596,2551; SAND-2020-12136J; LLNL-JRNL-835042; 2020-243, 1596, 2551; TRN: US2204758

Journal Information:: Physical Review B, Vol. 102, Issue 18; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Title: Measurement of the sound velocity and Grüneisen parameter of polystyrene at inertial confinement fusion conditions

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