Spectroscopic signatures of next-nearest-neighbor hopping in the charge and spin dynamics of doped one-dimensional antiferromagnets

Kumar, Umesh; Price, Gregorgy; Stiwinter, Kenneth; Nocera, Alberto; Johnson, Steven; Datta, Trianjan

doi:10.1103/physrevb.102.075134

Title: Spectroscopic signatures of next-nearest-neighbor hopping in the charge and spin dynamics of doped one-dimensional antiferromagnets

Journal Article · Mon Aug 24 00:00:00 EDT 2020 · Physical Review. B

DOI:https://doi.org/10.1103/physrevb.102.075134· OSTI ID:1711392

^[1]; Price, Gregorgy ^[2]; Stiwinter, Kenneth ^[2]; Nocera, Alberto ^[3]; Johnson, Steven ^[4];

^[2]

Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Univ. of Tennessee, Knoxville, TN (United States)
Augusta Univ., GA (United States)
Univ. of British Columbia, Vancouver, BC (Canada)
Univ. of Tennessee, Knoxville, TN (United States)

In this work, we study the impact of next-nearest-neighbor (nnn) hopping on the low-energy collective excitations of strongly correlated doped antiferromagnetic cuprate spin chains. Specifically, we use exact diagonalization and the density matrix renormalization group method to study the single-particle spectral function, the dynamical spin and charge structure factors, and the Cu L-edge resonant inelastic x-ray scattering (RIXS) intensity of the doped t-t'-J model for a set of t' values. We find evidence for the breakdown of spin-charge separation as |t'| increases and identify its fingerprints in the dynamical response functions. The inclusion of nnn hopping couples the spinon and holon excitations, resulting in the formation of a spin-polaron, where a ferromagnetic spin polarization cloud dresses the doped carrier. The spin-polaron manifests itself as additional spectral weight in the dynamical correlation functions, which appear simultaneously in the spin- and charge-sensitive channels. We also demonstrate that RIXS can provide a unique view of the spin-polaron, due to its sensitivity to both the spin and charge degrees of freedom.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA); USDOE Laboratory Directed Research and Development (LDRD) Program; National Science Foundation (NSF); Sun Yat-Sen University

Grant/Contract Number:: 89233218CNA000001; DMR-1842056; OEMT-2017-KF-06

OSTI ID:: 1711392

Report Number(s):: LA-UR-20-22832; TRN: US2204653

Journal Information:: Physical Review. B, Vol. 102, Issue 7; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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