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Title: Magnetism and superconductivity in Fe1+yTe1-xSex

Journal Article · · Journal of Physics. Condensed Matter
ORCiD logo [1];  [2];  [1]
  1. Brookhaven National Lab. (BNL), Upton, NY (United States)
  2. National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States)

Neutron scattering has played a significant role in characterizing magnetic and structural correlations in Fe$$_{1+y}$$Te$$_{1-x}$$Se$$_x$$ and their connections with superconductivity. Here we review several key aspects of the physics of iron chalcogenide superconductors where neutron studies played a key role. These topics include the phase diagram of Fe$$_{1+y}$$Te$$_{1-x}$$Se$$_{x}$$, where the doping-dependence of structural transitions can be understood from a mapping to the anisotropic random field Ising model. We then discuss orbital-selective Mott physics in the Fe chalcogenide series, where temperature-dependent magnetism in the parent material provided one of the earliest cases for orbital-selective correlation effects in a Hund's metal. Finally, we elaborate on the character of local magnetic correlations revealed by neutron scattering, its dependence on temperature and composition, and the connections to nematicity and superconductivity.

Research Organization:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC0012704
OSTI ID:
1558251
Report Number(s):
BNL-212008-2019-JAAM
Journal Information:
Journal of Physics. Condensed Matter, Vol. 32, Issue 37; ISSN 0953-8984
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 10 works
Citation information provided by
Web of Science

References (106)

First-Principles Calculations of the Electronic Structure of Tetragonal α -FeTe and α -FeSe Crystals: Evidence for a Bicollinear Antiferromagnetic Order journal April 2009
Experimental observation of incoherent-coherent crossover and orbital-dependent band renormalization in iron chalcogenide superconductors journal December 2015
Neutron-Diffraction Measurements of Magnetic Order and a Structural Transition in the Parent BaFe 2 As 2 Compound of FeAs-Based High-Temperature Superconductors journal December 2008
Observation of universal strong orbital-dependent correlation effects in iron chalcogenides journal July 2015
Enhanced low-energy magnetic excitations via suppression of the itinerancy in Fe 0.98 z Cu z Te 0.5 Se 0.5 journal October 2013
Density functional study of FeS, FeSe, and FeTe: Electronic structure, magnetism, phonons, and superconductivity journal October 2008
The Key Ingredients of the Electronic Structure of FeSe journal March 2018
The phase diagrams of iron-based superconductors: Theory and experiments journal January 2016
Measurement of Coherent Polarons in the Strongly Coupled Antiferromagnetically Ordered Iron-Chalcogenide Fe 1.02 Te using Angle-Resolved Photoemission Spectroscopy journal January 2013
Magnetic order close to superconductivity in the iron-based layered LaO1-xF x FeAs systems journal May 2008
Magnetic excitations of Fe 1 + y Se x Te 1 − x in magnetic and superconductive phases journal March 2010
Multiband magnetism and superconductivity in Fe-based compounds journal February 2009
Multiple topological states in iron-based superconductors journal September 2018
Local atomic structure of superconducting FeSe 1 x Te x journal April 2010
Thermal evolution of antiferromagnetic correlations and tetrahedral bond angles in superconducting FeTe 1 x Se x journal March 2016
Spin Waves in the ( π , 0 ) Magnetically Ordered Iron Chalcogenide Fe 1.05 Te journal February 2011
Local-moment magnetism in superconducting FeTe 0.35 Se 0.65 as seen via inelastic neutron scattering journal August 2011
Two-component Coulomb glass in insulators with a local attraction journal May 2012
Magnetic ground state of FeSe journal July 2016
Evidence for weak electronic correlations in iron pnictides journal July 2009
Magnetic, transport, and optical properties of monolayer copper oxides journal July 1998
Normal-State Hourglass Dispersion of the Spin Excitations in FeSe x Te 1 x journal October 2010
Magnetic neutron scattering studies on the Fe-based superconductor system Fe1+yTe1xSex journal July 2015
Antiferromagnetic order and spin dynamics in iron-based superconductors journal August 2015
Extreme sensitivity of superconductivity to stoichiometry in Fe 1 + δ Se journal January 2009
Spin-liquid polymorphism in a correlated electron system on the threshold of superconductivity journal August 2015
Superconductivity gets an iron boost journal March 2010
Superconductivity in the PbO-type structure  -FeSe journal September 2008
Superconductivity, magnetism, and stoichiometry of single crystals of Fe 1 + y ( Te 1 x S x ) z journal December 2009
Momentum dependence and nodes of the superconducting gap in the iron pnictides journal October 2009
Investigation of the Spin-Glass Regime between the Antiferromagnetic and Superconducting Phases in Fe 1+ y Se x Te 1- x journal November 2010
Kinetic frustration and the nature of the magnetic and paramagnetic states in iron pnictides and iron chalcogenides journal September 2011
Doping Driven ( π , 0) Nesting and Magnetic Properties of Fe 1 + x Te Superconductors journal August 2009
On the multi-orbital band structure and itinerant magnetism of iron-based superconductors journal January 2011
Electrical resistivity across a nematic quantum critical point journal February 2019
Strong Correlations from Hund’s Coupling journal April 2013
Temperature-Dependent Transformation of the Magnetic Excitation Spectrum on Approaching Superconductivity in Fe 1 + y x ( Ni / Cu ) x Te 0.5 Se 0.5 journal November 2012
What drives nematic order in iron-based superconductors? journal January 2014
The Electron-Pairing Mechanism of Iron-Based Superconductors journal April 2011
First-order magnetic and structural phase transitions in Fe 1 + y Se x Te 1 x journal February 2009
Strong coupling to magnetic fluctuations in the charge dynamics of iron-based superconductors journal July 2010
X-ray diffuse scattering study of local distortions in Fe 1 + x Te induced by excess Fe journal May 2011
Dimensional Crossover and Charge Order in Half-Doped Manganites and Cobaltites journal July 2003
Two kinds of in-plane resistivity anisotropy in Fe 1 + δ Te ( δ = 0.09 ) as seen via synchrotron radiation x-ray diffraction and in situ resistivity measurements journal May 2015
Spin Gap and Resonance at the Nesting Wave Vector in Superconducting FeSe 0.4 Te 0.6 journal August 2009
Suppression of phase separation and giant enhancement of superconducting transition temperature in FeSe 1− x Te x thin films journal February 2015
A common thread: The pairing interaction for unconventional superconductors journal October 2012
From (π,0) magnetic order to superconductivity with (π,π) magnetic resonance in Fe1.02Te1−xSex journal July 2010
Impact of dynamic orbital correlations on magnetic excitations in the normal state of iron-based superconductors journal September 2012
The metal–insulator transition in Fe 1.01− x Cu x Se journal July 2009
Unconventional electronic reconstruction in undoped ( Ba , Sr ) Fe 2 As 2 across the spin density wave transition journal November 2009
Modified magnetism within the coherence volume of superconducting Fe 1 + δ Se x Te 1 x journal September 2014
Substitution of Ni for Fe in superconducting Fe 0.98 Te 0.5 Se 0.5 depresses the normal-state conductivity but not the magnetic spectral weight journal January 2015
Disappearance of static magnetic order and evolution of spin fluctuations in Fe 1 + δ Se x Te 1 x journal September 2010
Strong correlations and spin-density-wave phase induced by a massive spectral weight redistribution in α -Fe 1.06 Te journal October 2010
Coexistence of superconductivity and short-range double-stripe spin correlations in Te-vapor annealed FeTe 1 x Se x ( x 0.2 ) journal June 2018
Charge and Magnetic Order in L a 0.5 S r 1.5 Mn O 4 journal March 1996
Using disorder to detect locally ordered electron nematics via hysteresis journal July 2011
Spin dynamics and orbital-antiphase pairing symmetry in iron-based superconductors journal October 2014
Magnetic order tuned by Cu substitution in Fe 1.1 z Cu z Te journal July 2012
Low-temperature phase diagram of Fe 1 + y Te studied using x-ray diffraction journal September 2013
Incommensurate itinerant antiferromagnetic excitations and spin resonance in the FeTe 0.6 Se 0.4 superconductor journal June 2010
Phase diagram and gap anisotropy in iron-pnictide superconductors journal February 2010
Tellurium substitution effect on superconductivity of the α-phase iron selenide journal October 2008
Spin anisotropy of the resonance peak in superconducting FeSe 0.5 Te 0.5 journal May 2011
Unusual Relationship between Magnetism and Superconductivity in FeTe 0.5 Se 0.5 journal May 2010
Inelastic Neutron Scattering Study of a Nonmagnetic Collapsed Tetragonal Phase in Nonsuperconducting CaFe 2 As 2 : Evidence of the Impact of Spin Fluctuations on Superconductivity in the Iron-Arsenide Compounds journal November 2013
Magnetism in Parent Iron Chalcogenides: Quantum Fluctuations Select Plaquette Order journal October 2012
Theory of the evolution of magnetic order in Fe 1 + y Te compounds with increasing interstitial iron journal October 2014
Spatial complexity due to bulk electronic nematicity in a superconducting underdoped cuprate journal January 2012
Coherence–incoherence crossover in the normal state of iron oxypnictides and importance of Hund's rule coupling journal February 2009
The energy gap of the compound FeSe0.5Te0.5 determined by specific heat and Point Contact Spectroscopy journal October 2015
Ubiquitous signatures of nematic quantum criticality in optimally doped Fe-based superconductors journal May 2016
Tunable ( δ π , δ π )-Type Antiferromagnetic Order in α -Fe(Te,Se) Superconductors journal June 2009
Nanoscale chemical phase separation in FeTe 0.55 Se 0.45 as seen via scanning tunneling spectroscopy journal June 2011
Structural instabilities in lanthanum cuprate superconductors journal April 1994
Coupling of spin and orbital excitations in the iron-based superconductor FeSe 0.5 Te 0.5 journal June 2010
A key role for unusual spin dynamics in ferropnictides journal December 2008
Superconductivity close to magnetic instability in Fe ( Se 1 x Te x ) 0.82 journal December 2008
Reversed anisotropy of the in-plane resistivity in the antiferromagnetic phase of iron tellurides journal April 2015
Continuous magnetic and structural phase transitions in Fe 1 + y Te journal February 2012
Recent advances in iron-based superconductors toward applications journal April 2018
Magnetic-crystallographic phase diagram of the superconducting parent compound Fe 1 + x Te journal August 2011
Fermi Surface Topology and Low-Lying Quasiparticle Dynamics of Parent Fe 1 + x Te / Se Superconductor journal July 2009
Interstitial iron tuning of the spin fluctuations in the nonsuperconducting parent phase Fe 1 + x Te journal July 2011
Competition between commensurate and incommensurate magnetic ordering in Fe 1 + y Te journal April 2012
Electronic properties of single-crystalline Fe 1.05 Te and Fe 1.03 Se 0.30 Te 0.70 journal April 2009
Evolution of spin excitations into the superconducting state in FeTe1−xSex journal January 2010
FeTe 0.55 Se 0.45 : A multiband superconductor in the clean and dirty limit journal April 2015
Quenched disorder and vestigial nematicity in the pseudogap regime of the cuprates journal May 2014
Strong interplay between stripe spin fluctuations, nematicity and superconductivity in FeSe journal December 2015
Orbital superconductivity, defects, and pinned nematic fluctuations in the doped iron chalcogenide FeSe 0.45 Te 0.55 journal August 2017
Unconventional s-Wave Superconductivity in Fe(Se,Te) journal April 2010
FeAs-Based Superconductivity: A Case Study of the Effects of Transition Metal Doping on BaFe 2 As 2 journal August 2010
Spin fluctuations and superconductivity in powders of Fe 1 + x Te 0.7 Se 0.3 as a function of interstitial iron concentration journal March 2012
Isotropic superconducting gaps with enhanced pairing on electron Fermi surfaces in FeTe 0.55 Se 0.45 journal March 2012
Effect of magnetic field on the spin resonance in FeTe 0.5 Se 0.5 as seen via inelastic neutron scattering journal March 2010
Effects of Ni and Co doping on the physical properties of tetragonal FeSe0.5Te0.5 superconductor journal July 2010
Tetragonal-to-Orthorhombic Structural Phase Transition at 90 K in the Superconductor Fe 1.01 Se journal July 2009
High-temperature superconductivity in iron pnictides and chalcogenides journal March 2016
Ferro-Orbital Ordering Transition in Iron Telluride Fe 1 + y Te journal May 2014
Evolution of two-step structural phase transition in Fe1+dTe detected by low-temperature x-ray diffraction journal June 2012
Neutron scattering resonance and the iron-pnictide superconducting gap journal April 2009
Surprising loss of three-dimensionality in low-energy spin correlations on approaching superconductivity in Fe 1 + y Te 1 x Se x journal October 2017
Unified Picture for Magnetic Correlations in Iron-Based Superconductors journal September 2010
Unconventional Temperature Enhanced Magnetism in Fe 1.1 Te journal November 2011