Magnetoelectric phase diagrams of multiferroicGdMn2O5

Bukhari, S. H.; Kain, Th.; Schiebl, M.; Shuvaev, A.; Pimenov, Anna; Kuzmenko, A. M.; Wang, X.; Cheong, S. -W.; Ahmad, J.; Pimenov, A.

doi:10.1103/physrevb.94.174446

Title: Magnetoelectric phase diagrams of multiferroicGdMn2O5

Journal Article · Mon Nov 28 00:00:00 EST 2016 · Physical Review B

DOI:https://doi.org/10.1103/physrevb.94.174446· OSTI ID:1535786

Bukhari, S. H. ^[1]; Kain, Th. ^[2]; Schiebl, M. ^[2]; Shuvaev, A. ^[2]; Pimenov, Anna ^[2]; Kuzmenko, A. M. ^[3]; Wang, X. ^[4]; Cheong, S. -W. ^[5]; Ahmad, J. ^[6]; Pimenov, A. ^[2]

Bahauddin Zakariya University, Multan (Pakistan); Vienna Univ. of Technology (Austria)
Vienna Univ. of Technology (Austria)
Russian Academy of Sciences (RAS), Moscow (Russian Federation)
Univ. of Science and Technology of China, Beijing (China); Rutgers Univ., Piscataway, NJ (United States)
Rutgers Univ., Piscataway, NJ (United States)
Bahauddin Zakariya University, Multan (Pakistan)

Electric and magnetic properties of multiferroic GdMn₂O₅ in external magnetic fields were investigated to map out the magnetoelectric phases in this material. Due to strong magnetoelectric coupling, the dielectric permittivity is highly sensitive to phase boundaries in GdMn₂O₅, which allowed us to construct the field-temperature phase diagrams. Several phase transitions are observed which are strongly field dependent with respect to field orientation and strength. The phase diagram for a magnetic field along the crystallographic a axis corresponds well to a polarization step, as induced by 90° rotation of Gd magnetic moments. Our results support the model of two ferroelectric sublattices, Mn-Mn and Gd-Mn, with strong R -Mn (4f - 3d) interaction for the polarization in R Mn₂O₅.

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Research Organization:: Rutgers Univ., Piscataway, NJ (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: FG02-07ER46382

OSTI ID:: 1535786

Alternate ID(s):: OSTI ID: 1333583

Journal Information:: Physical Review B, Vol. 94, Issue 17; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 22 works

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Abnormal dependence of multiferroicity on high-temperature electro-poling in GdMn ₂ O ₅ Zheng, S. H.; Gong, J. J.; Li, Y. Q. Journal of Applied Physics, Vol. 126, Issue 17 https://doi.org/10.1063/1.5120971	journal	November 2019
Enhanced antiferromagnetic transition and magnetodielectric study in cobalt and holmium co-substituted multiferroic Bi ₂ Fe ₄ O ₉ Mohapatra, S. R.; Kaushik, S. D.; Singh, A. K. Materials Research Express, Vol. 5, Issue 1 https://doi.org/10.1088/2053-1591/aaa655	journal	January 2018
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Optical phonons and its effect on physical properties of rare-earth orthoferrites R FeO ₃ ( R = La, Nd, Gd, Dy, Er): IR reflectivity measurements Jamil, Muhammad Tufiq; Ahmad, Javed; Bukhari, Syed Hamad International Journal of Modern Physics B, Vol. 32, Issue 21 https://doi.org/10.1142/s0217979218502296	journal	August 2018

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