skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Counting the electrons in a multiphoton ionization by elastic scattering of microwaves

Journal Article · · Scientific Reports
 [1]; ORCiD logo [2];  [3];  [1];  [2];  [1]
  1. Purdue Univ., West Lafayette, IN (United States). School of Aeronautics and Astronautics
  2. Purdue Univ., West Lafayette, IN (United States). School of Mechanical Engineering
  3. Princeton Univ., NJ (United States). Dept. of Mechanical and Aerospace Engineering

Multiphoton ionization (MPI) is a fundamental first step in high-energy laser-matter interaction and is important for understanding the mechanism of plasma formation. With the discovery of MPI more than 50 years ago, there were numerous attempts to determine the basic physical constants of this process in direct experiments, namely photoionization rates and cross-sections of the MPI; however, no reliable data was available until now, and the spread in the literature values often reaches 2–3 orders of magnitude. This is due to the inability to conduct absolute measurements of plasma electron numbers generated by MPI, which leads to uncertainties and, sometimes, contradictions between MPI cross-section values utilized by different researchers across the field. Here, we report the first direct measurement of absolute plasma electron numbers generated at MPI of air, and subsequently we precisely determine the ionization rate and cross-section of eight-photon ionization of oxygen molecule by 800 nm photons σ8 = (3.3 ± 0.3)×10-130 W-8m16s-1. The method, based on the absolute measurement of the electron number created by MPI using elastic scattering of microwaves off the plasma volume in Rayleigh regime, establishes a general approach to directly measure and tabulate basic constants of the MPI process for various gases and photon energies.

Research Organization:
Purdue Univ., West Lafayette, IN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Fusion Energy Sciences (FES); National Science Foundation (NSF)
Grant/Contract Number:
SC0018156; 1465061
OSTI ID:
1499979
Journal Information:
Scientific Reports, Vol. 8; ISSN 2045-2322
Publisher:
Nature Publishing GroupCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 36 works
Citation information provided by
Web of Science

References (33)

Laser Electron Accelerator journal July 1979
Principles and applications of compact laser–plasma accelerators journal June 2008
Conductivity Measurements of Femtosecond Laser–Plasma Filaments journal October 2007
A Generalization of the Dielectric Ellipsoid Problem journal August 1945
Femtosecond laser guiding of a high-voltage discharge and the restoration of dielectric strength in air and nitrogen journal December 2012
Effect of power losses on self-focusing of high-intensity laser beam in gases journal April 2013
Effect of quantum interference on tunneling photoionization rates of N2 and O2 molecules journal March 2005
Femtosecond filamentation in transparent media journal March 2007
Microwave diagnostics of small plasma objects journal August 2005
Ultrashort filaments of light in weakly ionized, optically transparent media journal September 2007
Tailoring the air plasma with a double laser pulse journal June 2011
Gas Discharge Physics book January 1991
High-order harmonic generation in rare gases with a 1-ps 1053-nm laser journal February 1993
Electromagnetic beam propagation in nonlinear media journal January 2015
High intensity laser mass spectrometry — a review journal May 1997
Semi-empirical model for the rate of tunnel ionization of N2 and O2 molecule in an intense Ti:sapphire laser pulse journal May 1999
Dissociative ionization of NO in an intense laser field: a route towards enhanced ionization journal April 1997
Triggering and guiding electric discharge by a train of ultraviolet picosecond pulses combined with a long ultraviolet pulse journal March 2012
Conductivity and discharge guiding properties of mid-IR laser filaments journal October 2016
Non-equilibrium plasma produced by intense pulse lasers and relative diagnostics journal November 2013
Tunnel and multiphoton ionization of atoms and ions in a strong laser field (Keldysh theory) journal September 2004
Electric discharge during electrosurgery journal April 2015
Femtosecond laser electronic excitation tagging for quantitative velocity imaging in air journal January 2011
High-order harmonic generation using intense femtosecond pulses journal February 1993
Experimental and theoretical analysis of resonant multiphoton ionization of benzene journal January 1985
Gas discharge physics journal August 1993
Ultrashort filaments of light in weakly ionized, optically transparent media journal September 2008
Classical Electrodynamics, 3rd ed . journal September 1999
Tunnel and multiphoton ionization of atoms and ions in a strong laser field (Keldysh theory) [Tunnel'naya i mnogofotonnaya ionizatsiya atomov i ionov v sil'nom lazernom pole (teoriya Keldysha)] journal January 2004
Conductivity and Discharge Guiding Properties of Mid-IR Laser Filaments conference January 2016
Conductivity and Discharge Guiding Properties of Mid-IR Laser Filaments text January 2016
Plasma filament investigation by transverse optical interferometry and terahertz scattering journal January 2011
Ultrashort filaments of light in weakly-ionized, optically-transparent media text January 2006

Cited By (3)

Direct measurement of electron numbers created at near-infrared laser-induced ionization of various gases journal May 2019
Pressure-scaling characteristics of femtosecond two-photon laser-induced fluorescence of carbon monoxide journal January 2019
Direct measurement of electron numbers created at infrared laser-induced ionization of various gases text January 2018

Figures / Tables (7)


Similar Records

Multiphoton ionization of C[sub 60]
Journal Article · Thu Mar 18 00:00:00 EST 1993 · Journal of Physical Chemistry; (United States) · OSTI ID:1499979

X-ray-laser interaction with matter and the role of multiphoton ionization: Free-electron-laser studies on neon and helium
Journal Article · Tue May 15 00:00:00 EDT 2007 · Physical Review. A · OSTI ID:1499979

Multiphoton ionization of atomic cesium
Conference · Sun Jan 01 00:00:00 EST 1984 · OSTI ID:1499979