Method of thermally-stabilizing an oxygen transport membrane-based reforming system

Kelly, Sean M.; Swami, Sadashiv M.; Peck, John D.

Title: Method of thermally-stabilizing an oxygen transport membrane-based reforming system

Patent · Tue Nov 06 00:00:00 EST 2018

OSTI ID:1493314

Kelly, Sean M.; Swami, Sadashiv M.; Peck, John D.

A method of operating an oxygen transport membrane based reforming system employing one or more packs of thermally coupled panels of reformer tubes and oxygen transport membrane ("OTM") reactors close to thermo-neutral point is provided. The method produces syngas by converting a hydrocarbon-containing feed, such as natural gas in the reformer tubes of a pack by endothermic steam reforming reactions. The heat required for endothermic reforming reactions is provided by exothermic oxidizing reactions occurring inside the OTM reactors of the pack. At a thermo-neutral point the heat released by exothermic reactions matches the heat required to support endothermic reactions and heat losses in the pack. The method modulates the flow rate of hydrocarbon-containing feed and/or steam-to-carbon ratio of the combined feed to the pack to maintain the surface temperature of oxygen transport membrane reactors below a target maximum temperature. The syngas product oxygen-to-carbon ratio is maintained within a desired target range such that the OTM based reforming system is operated close to thermo-neutral point.

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Research Organization:: Praxair, Inc., Danbury, CT (United States)

Sponsoring Organization:: USDOE

DOE Contract Number:: FC26-07NT43088

Assignee:: PRAXAIR TECHNOLOGY, INC. (Danbury, CT)

Patent Number(s):: 10,118,823

Application Number:: 14/969,486

OSTI ID:: 1493314

Resource Relation:: Patent File Date: 2015 Dec 15

Country of Publication:: United States

Language:: English

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Method And System For Producing Methanol Using An Integrated Oxygen Transport Membrane Based Reforming System Stuckert, Ines; Chakravarti, Shrikar; Drnevich, Raymond https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20140323597 US Patent Application 14/078859; 20140323597	patent-application	October 2014
Fuel cell system with integrated fuel processor Kelley, Richard H. https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/20070122667 US Patent Application 11/288775; 20070122667	patent-application	May 2007
Oxygen enriching apparatus, controller, and recording medium Yagi, Hideaki; Akiyama, Junichi https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/7077133 US Patent Document 7,077,133	patent	July 2006
Process for the water vapor reforming of a hydrocarbon or a hydrocarbon derivative, reforming system operable thereby, and fuel cell operating process Autenrieth, Rainer; Boneberg, Stefan; Heil, Dietmar https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6268075 US Patent Document 6,268,075	patent	July 2001
Method and apparatus for producing carbon dioxide Prasad, Ravi; Gottzmann, Christian Friedrich; Keskar, Nitin Ramesh https://doi.org/https://image-ppubs.uspto.gov/dirsearch-public/print/downloadPdf/6537514 US Patent Document 6,537,514	patent	March 2003

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