Ultrafast extreme ultraviolet photoemission without space charge

Corder, Christopher; Zhao, Peng; Bakalis, Jin; Li, Xinlong; Kershis, Matthew D.; Muraca, Amanda R.; White, Michael G.; Allison, Thomas K.

doi:10.1063/1.5045578

Title: Ultrafast extreme ultraviolet photoemission without space charge

Journal Article · Thu Sep 06 00:00:00 EDT 2018 · Structural Dynamics

DOI:https://doi.org/10.1063/1.5045578· OSTI ID:1483745

Corder, Christopher ^[1]; Zhao, Peng ^[1]; Bakalis, Jin ^[1]; Li, Xinlong ^[1]; Kershis, Matthew D. ^[2]; Muraca, Amanda R. ^[1];

^[3]; Allison, Thomas K. ^[1]

Stony Brook Univ., Stony Brook, NY (United States)
Brookhaven National Lab. (BNL), Upton, NY (United States)
Stony Brook Univ., Stony Brook, NY (United States); Brookhaven National Lab. (BNL), Upton, NY (United States)

Time- and Angle-resolved photoelectron spectroscopy from surfaces can be used to record the dynamics of electrons and holes in condensed matter on ultrafast time scales. However, ultrafast photoemission experiments using extreme-ultraviolet (XUV) light have previously been limited by either space-charge effects, low photon flux, or limited tuning range. In this article, we describe XUV photoelectron spectroscopy experiments with up to 5 nA of average sample current using a tunable cavity-enhanced high-harmonic source operating at 88 MHz repetition rate. The source delivers >10¹¹ photons/s in isolated harmonics to the sample over a broad photon energy range from 18 to 37 eV with a spot size of 58 × 100 μm². From photoelectron spectroscopy data, we place conservative upper limits on the XUV pulse duration and photon energy bandwidth of 93 fs and 65 meV, respectively. In conclusion, the high photocurrent, lack of strong space charge distortions of the photoelectron spectra, and excellent isolation of individual harmonic orders allow us to observe laser-induced modifications of the photoelectron spectra at the 10^–4 level, enabling time-resolved XUV photoemission experiments in a qualitatively new regime.

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Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0012704; SC0016017

OSTI ID:: 1483745

Alternate ID(s):: OSTI ID: 1468879

Report Number(s):: BNL-209507-2018-JAAM

Journal Information:: Structural Dynamics, Vol. 5, Issue 5; ISSN 2329-7778

Publisher:: American Crystallographic Association/AIPCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 51 works

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Spin-ARPES EUV Beamline for Ultrafast Materials Research and Development Nie, Zhonghui; Turcu, Ion Cristian Edmond; Li, Yao Applied Sciences, Vol. 9, Issue 3 https://doi.org/10.3390/app9030370	journal	January 2019
A High Resolution XUV Grating Monochromator for the Spectral Selection of Ultrashort Harmonic Pulses Fabris, Nicola; Miotti, Paolo; Frassetto, Fabio Applied Sciences, Vol. 9, Issue 12 https://doi.org/10.3390/app9122502	journal	June 2019
High-flux ultrafast extreme-ultraviolet photoemission spectroscopy at 18.4 MHz pulse repetition rate Saule, T.; Heinrich, S.; Schötz, J. GSI Helmholtzzentrum fuer Schwerionenforschung, GSI, Darmstadt https://doi.org/10.15120/gsi-2019-00262	text	January 2019
Time- and momentum-resolved photoemission studies using time-of-flight momentum microscopy at a free-electron laser Kutnyakhov, Dmytro; Xian, R. P.; Dendzik, M. Deutsches Elektronen-Synchrotron, DESY, Hamburg https://doi.org/10.3204/pubdb-2020-00522	text	January 2020
Extreme ultraviolet time-resolved photoelectron spectroscopy of aqueous aniline solution: enhanced surface concentration and pump-induced space charge effect West, Christopher W.; Nishitani, Junichi; Higashimura, Chika Taylor & Francis https://doi.org/10.6084/m9.figshare.12062994	text	January 2020
Cavity-Enhanced Noncollinear High-Harmonic Generation Hogner, Maximilian; Saule, Tobias; Heinrich, Stephan 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) https://doi.org/10.1109/cleoe-eqec.2019.8871690	conference	June 2019
Time- and momentum-resolved photoemission studies using time-of-flight momentum microscopy at a free-electron laser Kutnyakhov, D.; Xian, R. P.; Dendzik, M. Deutsches Elektronen-Synchrotron, DESY, Hamburg https://doi.org/10.3204/pubdb-2019-04797	text	January 2020
Extreme ultraviolet time-resolved photoelectron spectroscopy of aqueous aniline solution: enhanced surface concentration and pump-induced space charge effect West, Christopher W.; Nishitani, Junichi; Higashimura, Chika Taylor & Francis https://doi.org/10.6084/m9.figshare.12062994.v1	text	January 2020
Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate Puppin, M.; Deng, Y.; Nicholson, C. W. arXiv https://doi.org/10.48550/arxiv.1811.06939	text	January 2018
Extreme Ultraviolet Time- and Angle-Resolved Photoemission Spectroscopy with 21.5 meV Resolution using High-Order Harmonic Generation from a Turn-Key Yb:KGW Amplifier Liu, Yangyang; Beetar, John E.; Hosen, Md Mofazzel arXiv https://doi.org/10.48550/arxiv.1907.10497	text	January 2019
An open-source, end-to-end workflow for multidimensional photoemission spectroscopy Xian, Rui Patrick; Acremann, Yves; Agustsson, Steinn Ymir arXiv https://doi.org/10.48550/arxiv.1909.07714	text	January 2019
Time-Resolved Momentum Microscopy with a 1 MHz High-Harmonic Extreme Ultraviolet Beamline Keunecke, M.; Möller, C.; Schmitt, D. arXiv https://doi.org/10.48550/arxiv.2003.01602	text	January 2020
Broadband ultraviolet-visible frequency combs from cascaded high-harmonic generation in quasi-phase-matched waveguides Rutledge, Jay; Catanese, Anthony; Hickstein, Daniel D. arXiv https://doi.org/10.48550/arxiv.2102.04670	text	January 2021

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