Ion Correlation Effects in Salt-Doped Block Copolymers

Brown, Jonathan R.; Seo, Youngmi; Hall, Lisa M.

doi:10.1103/PhysRevLett.120.127801

Title: Ion Correlation Effects in Salt-Doped Block Copolymers

Journal Article · Thu Mar 22 00:00:00 EDT 2018 · Physical Review Letters

DOI:https://doi.org/10.1103/PhysRevLett.120.127801· OSTI ID:1468577

Brown, Jonathan R. ^[1]; Seo, Youngmi ^[2]; Hall, Lisa M. ^[1]

The Ohio State Univ., Columbus, OH (United States). William G. Lowrie Dept. of Chemical and Biomolecular Engineering
The Ohio State Univ., Columbus, OH (United States). William G. Lowrie Dept. of Chemical and Biomolecular Engineering; LG Chem, Ltd., Daejeon (Korea, Republic of). LG Chem Research Park

Here, we apply classical density functional theory to study how salt changes the microphase morphology of diblock copolymers. Polymers are freely jointed and one monomer type favorably interacts with ions, to account for the selective solvation that arises from different dielectric constants of the microphases. By including correlations from liquid state theory of an unbound reference fluid, the theory can treat chain behavior, microphase separation, ion correlations, and preferential solvation, at same coarse grained level. We show good agreement with molecular dynamics simulations.

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Research Organization:: The Ohio State Univ., Columbus, OH (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF)

Grant/Contract Number:: SC0014458; SC0014209; 1454343

OSTI ID:: 1468577

Alternate ID(s):: OSTI ID: 1427878

Journal Information:: Physical Review Letters, Vol. 120, Issue 12; ISSN 0031-9007

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 42 works

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Title: Ion Correlation Effects in Salt-Doped Block Copolymers

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