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Title: Structural feature controlling superconductivity in compressed BaFe 2 As 2

Journal Article · · Journal of Applied Physics
DOI:https://doi.org/10.1063/1.4867159· OSTI ID:1385736
 [1];  [2];  [3];  [4];  [4];  [5]
  1. Center for High Pressure Science and Technology Advanced Research, Shanghai (China); Carnegie Inst. of Washington, Washington, DC (United States)
  2. Chinese Academy of Sciences (CAS), Hefei (China)
  3. Center for High Pressure Science and Technology Advanced Research, Shanghai (China); South China Univ. of Technology (SCUT), Guangzhou (China)
  4. Zhejiang Univ., Hangzhou (China)
  5. Center for High Pressure Science and Technology Advanced Research, Shanghai (China); Chinese Academy of Sciences (CAS), Hefei (China) ; Carnegie Inst. of Washington, Washington, DC (United States)

Superconductivity can be induced with the application of pressure but it disappears eventually upon heavy compression in the iron-based parent compound BaFe2As2. Structural evolution with pressure is used to understand this behavior. By performing synchrotron X-ray powder diffraction measurements with diamond anvil cells up to 26.1 GPa, we find an anomalous behavior of the lattice parameter with a $$S$$ shape along the a axis but a monotonic decrease in the $$c$$-axis lattice parameter with increasing pressure. The close relationship between the axial ratio $c/a$ and the superconducting transition temperature $$T_c$$ is established for this parent compound. The $c/a$ ratio is suggested to be a measure of the spin fluctuation strength. The reduction of $$T_c$$ with the further increase of pressure is a result of the pressure-driven weakness of the spin-fluctuation strength in this material.

Research Organization:
Energy Frontier Research Centers (EFRC) (United States). Energy Frontier Research in Extreme Environments (EFree)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC0001057
OSTI ID:
1385736
Journal Information:
Journal of Applied Physics, Vol. 115, Issue 8; Related Information: EFree partners with Carnegie Institution of Washington (lead); California Institute of Technology; Colorado School of Mines; Cornell University; Lehigh University; Pennsylvania State University; ISSN 0021-8979
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 5 works
Citation information provided by
Web of Science

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