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Title: Magnetic excitations in the spin-1/2 triangular-lattice antiferromagnet Cs2CuBr4

Journal Article · · New Journal of Physics
 [1];  [2];  [2];  [3];  [4];  [5];  [5];  [6];  [7];  [7];  [8]
  1. Helmholtz-Zentrum Dresden-Rossendorf, Dresden (Germany)
  2. Helmholtz-Zentrum Dresden-Rossendorf, Dresden (Germany); Radboud Univ., Nijmegen (Netherlands)
  3. Helmholtz-Zentrum Dresden-Rossendorf, Dresden (Germany); Institute of Solid State Physics at the TU Dresden, Dresden (Germany)
  4. Florida State Univ., Tallahassee, FL (United States). National High Magnetic Field Lab. (MagLab)
  5. Osaka Univ. (Japan). Center for Advanced High Magnetic Field Science (AHMF)
  6. Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.; Stony Brook Univ., NY (United States). Dept. of Physics and Astronomy; Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  7. Brookhaven National Lab. (BNL), Upton, NY (United States). Condensed Matter Physics and Materials Science Dept.; Stony Brook Univ., NY (United States). Dept. of Physics and Astronomy
  8. Institute for Nanoscience and Cryogenics (INAC), Grenoble (France)

We present on high- field electron spin resonance (ESR) studies of magnetic excitations in the spin- 1/2 triangular-lattice antiferromagnet Cs2CuBr4. Frequency- field diagrams of ESR excitations are measured for different orientations of magnetic fields up to 25 T. We show that the substantial zero- field energy gap, Δ ≈ 9.5 K, observed in the low-temperature excitation spectrum of Cs2CuBr4 [Zvyagin et al:, Phys. Rev. Lett. 112, 077206 (2014)], is present well above TN. Noticeably, the transition into the long-range magnetically ordered phase does not significantly affect the size of the gap, suggesting that even below TN the high-energy spin dynamics in Cs2CuBr4 is determined by short-range-order spin correlations. The experimental data are compared with results of model spin-wave-theory calculations for spin-1/2 triangle-lattice antiferromagnet.

Research Organization:
Brookhaven National Lab. (BNL), Upton, NY (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC00112704
OSTI ID:
1240588
Report Number(s):
BNL-111748-2016-JA; R&D Project: PM016; KC0201050
Journal Information:
New Journal of Physics, Vol. 17, Issue 11; ISSN 1367-2630
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 12 works
Citation information provided by
Web of Science

References (41)

Resonating valence bonds: A new kind of insulator? journal February 1973
Exact spectra, spin susceptibilities, and order parameter of the quantum Heisenberg antiferromagnet on the triangular lattice journal October 1994
Long-Range Néel Order in the Triangular Heisenberg Model journal May 1999
Excitation spectra of the spin- 1 2 triangular-lattice Heisenberg antiferromagnet journal December 2006
Neél Order in Square and Triangular Lattice Heisenberg Models journal September 2007
Ordering in Spatially Anisotropic Triangular Antiferromagnets journal February 2007
Order in a spatially anisotropic triangular antiferromagnet journal November 2011
Spin- 1 2 Heisenberg model on the anisotropic triangular lattice: From magnetism to a one-dimensional spin liquid journal July 2009
Spin-liquid phase in an anisotropic triangular-lattice Heisenberg model: Exact diagonalization and density-matrix renormalization group calculations journal July 2006
Incommensurate correlations in the anisotropic triangular Heisenberg lattice journal December 2011
Functional renormalization group for the anisotropic triangular antiferromagnet journal January 2011
Experimental Realization of a 2D Fractional Quantum Spin Liquid journal February 2001
Spinons and triplons in spatially anisotropic frustrated antiferromagnets journal October 2007
Quasiparticles of Spatially Anisotropic Triangular Antiferromagnets in a Magnetic Field journal November 2009
Spin liquids in frustrated magnets journal March 2010
Neutron scattering study of the magnetic structure of journal September 1996
The crystal structure of cesium tetrabromocuprate(II) journal October 1960
Direct Determination of Exchange Parameters in Cs 2 CuBr 4 and Cs 2 CuCl 4 : High-Field Electron-Spin-Resonance Studies journal February 2014
Direct Measurement of the Spin Hamiltonian and Observation of Condensation of Magnons in the 2D Frustrated Quantum Magnet Cs 2 CuCl 4 journal March 2002
Bose-Einstein Condensation of Magnons in Cs 2 CuCl 4 journal September 2005
Cascade of Magnetic-Field-Induced Quantum Phase Transitions in a Spin- 1 2 Triangular-Lattice Antiferromagnet journal June 2009
Field-Induced Phase Transitions Driven by Quantum Fluctuation in S =1/2 Anisotropic Triangular Antiferromagnet Cs 2 CuBr 4 journal January 2005
High-field ESR study of the dimerized-incommensurate phase transition in the spin-Peierls compound CuGeO3 journal April 2004
Continuum in the Spin-Excitation Spectrum of a Haldane Chain Observed by Neutron Scattering in CsNiCl 3 journal June 2001
Extended scattering continua characteristic of spin fractionalization in the two-dimensional frustrated quantum magnet Cs 2 CuCl 4 observed by neutron scattering journal October 2003
Novel Longitudinal Mode in the Coupled Quantum Chain Compound KCuF 3 journal July 2000
Longitudinal magnetic dynamics and dimensional crossover in the quasi-one-dimensional spin- 1 2 Heisenberg antiferromagnet KCuF 3 journal April 2005
Quantum criticality and universal scaling of a quantum antiferromagnet journal March 2005
Magnetic Phase Transition and Magnetization Plateau in Cs 2 CuBr 4 journal January 2002
Spin dynamics of the quasi-two-dimensional spin- 1 2 quantum magnet Cs 2 CuCl 4 journal October 2005
Spin structure factor of the frustrated quantum magnet Cs 2 CuCl 4 journal May 2006
High-Field Electron Spin Resonance and Magnetization in the Dimerized Phase of CuGeO 3 journal September 1994
High magnetic-field ESR in the Haldane spin chains NENP and NINO journal January 2000
High-field ESR Studies of the Quantum Spin Dimer System Ba3Cr2O8 journal September 2012
High-field electron spin resonance spectroscopy of singlet-triplet transitions in the spin-dimer systems Sr 3 Cr 2 O 8 and Ba 3 Cr 2 O 8 journal May 2014
An Electron Spin Resonance Selection Rule for Spin-Gapped Systems journal November 2000
Colloquium : Spontaneous magnon decays journal January 2013
Spin waves in a triangular lattice antiferromagnet: Decays, spectrum renormalization, and singularities journal April 2009
Magnetic resonance in the ordered phases of the two-dimensional frustrated quantum magnet Cs 2 CuCl 4 journal May 2012
Magnetization plateaux of the S = 1/2 two-dimensional frustrated antiferromagnet Cs 2 CuBr 4 journal March 2004
Magnetization plateau in the frustrated quantum spin system Cs 2 CuBr 4 journal March 2003

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