Current status and future directions of all-solid-state batteries with lithium metal anodes, sulfide electrolytes, and layered transition metal oxide cathodes
Abstract
All-solid-state batteries (ASSBs) offer great promise as a next-generation energy storage technology with higher energy density, wider operating temperature range, and improved safety for electric vehicles. ASSBs employing lithium metal anodes (Li), sulfide-based solid-state electrolytes (SSE), and Ni-rich layered transition metal oxide cathodes (LiMO2, M = Ni, Mn, Co, Al) are particularly promising due to its superior electrochemical performance compared to other solid-electrolyte systems. However, the battery cycle life at high cathode mass loading and high current is still limited because the failure mechanism is not fully understood. Lithium dendrite growth at the anode or inside a solid electrolyte still represents as a serious risk of cell failure. Interfacial resistance increases attributed to electrolyte decomposition and interfacial void formation at both cathode–electrolyte and anode–electrolyte interfaces lead to gradual capacity fading. In this Review, we present the fundamental challenges and recent scientific understandings of each component in ASSBs. The novel diagnostic tools for these components, especially the interfaces buried under the surface that are often hard for characterization are mainly examined. Lastly, we offer a perspective for future research directions. We hope this Review will provide a timely snapshot of state-of-the-art research progress in ASSBs to accelerate the development of ASSBs.
- Authors:
-
- University of Houston, TX (United States)
- Zhejiang University of Technology, Hangzhou (China)
- Rice University, Houston, TX (United States)
- Publication Date:
- Research Org.:
- Univ. of Houston, TX (United States)
- Sponsoring Org.:
- USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Sustainable Transportation. Vehicle Technologies Office (VTO); National Natural Science Foundation of China (NSFC); USDOE Office of Energy Efficiency and Renewable Energy (EERE), Transportation Office. Vehicle Technologies Office; USDOE Office of Energy Efficiency and Renewable Energy (EERE)
- OSTI Identifier:
- 1985463
- Alternate Identifier(s):
- OSTI ID: 1782078; OSTI ID: 1787162
- Grant/Contract Number:
- EE0008864; 21972127; U20A20253
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nano Energy
- Additional Journal Information:
- Journal Volume: 87; Journal ID: ISSN 2211-2855
- Publisher:
- Elsevier
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE; All-solid-state battery; Lithium metal anode; Sulfide electrolyte; Layered ternary oxide cathode
Citation Formats
Wu, Chaoshan, Lou, Jiatao, Zhang, Jun, Chen, Zhaoyang, Kakar, Akshay, Emley, Benjamin, Ai, Qing, Guo, Hua, Liang, Yanliang, Lou, Jun, Yao, Yan, and Fan, Zheng. Current status and future directions of all-solid-state batteries with lithium metal anodes, sulfide electrolytes, and layered transition metal oxide cathodes. United States: N. p., 2021.
Web. doi:10.1016/j.nanoen.2021.106081.
Wu, Chaoshan, Lou, Jiatao, Zhang, Jun, Chen, Zhaoyang, Kakar, Akshay, Emley, Benjamin, Ai, Qing, Guo, Hua, Liang, Yanliang, Lou, Jun, Yao, Yan, & Fan, Zheng. Current status and future directions of all-solid-state batteries with lithium metal anodes, sulfide electrolytes, and layered transition metal oxide cathodes. United States. https://doi.org/10.1016/j.nanoen.2021.106081
Wu, Chaoshan, Lou, Jiatao, Zhang, Jun, Chen, Zhaoyang, Kakar, Akshay, Emley, Benjamin, Ai, Qing, Guo, Hua, Liang, Yanliang, Lou, Jun, Yao, Yan, and Fan, Zheng. Sat .
"Current status and future directions of all-solid-state batteries with lithium metal anodes, sulfide electrolytes, and layered transition metal oxide cathodes". United States. https://doi.org/10.1016/j.nanoen.2021.106081. https://www.osti.gov/servlets/purl/1985463.
@article{osti_1985463,
title = {Current status and future directions of all-solid-state batteries with lithium metal anodes, sulfide electrolytes, and layered transition metal oxide cathodes},
author = {Wu, Chaoshan and Lou, Jiatao and Zhang, Jun and Chen, Zhaoyang and Kakar, Akshay and Emley, Benjamin and Ai, Qing and Guo, Hua and Liang, Yanliang and Lou, Jun and Yao, Yan and Fan, Zheng},
abstractNote = {All-solid-state batteries (ASSBs) offer great promise as a next-generation energy storage technology with higher energy density, wider operating temperature range, and improved safety for electric vehicles. ASSBs employing lithium metal anodes (Li), sulfide-based solid-state electrolytes (SSE), and Ni-rich layered transition metal oxide cathodes (LiMO2, M = Ni, Mn, Co, Al) are particularly promising due to its superior electrochemical performance compared to other solid-electrolyte systems. However, the battery cycle life at high cathode mass loading and high current is still limited because the failure mechanism is not fully understood. Lithium dendrite growth at the anode or inside a solid electrolyte still represents as a serious risk of cell failure. Interfacial resistance increases attributed to electrolyte decomposition and interfacial void formation at both cathode–electrolyte and anode–electrolyte interfaces lead to gradual capacity fading. In this Review, we present the fundamental challenges and recent scientific understandings of each component in ASSBs. The novel diagnostic tools for these components, especially the interfaces buried under the surface that are often hard for characterization are mainly examined. Lastly, we offer a perspective for future research directions. We hope this Review will provide a timely snapshot of state-of-the-art research progress in ASSBs to accelerate the development of ASSBs.},
doi = {10.1016/j.nanoen.2021.106081},
journal = {Nano Energy},
number = ,
volume = 87,
place = {United States},
year = {Sat May 08 00:00:00 EDT 2021},
month = {Sat May 08 00:00:00 EDT 2021}
}
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