Field-dependent nonelectronic contributions to thermal conductivity in a metallic ferromagnet with low Gilbert damping
Abstract
Heat conduction in metals is typically dominated by electron transport since electrons carry both charge and heat. In magnetic metals magnons, or spin waves, excitations of the magnetic order can be used to transport information. Heat conduction via magnons has been previously shown mostly for insulating magnets with low Gilbert damping and resulting long spin-wave lifetimes where conduction electrons cannot contribute. Here we show that thin films of properly optimized metallic ferromagnetic (FM) alloys show significant nonelectronic contributions to heat conduction, which furthermore depend on the direction of an applied magnetic field. These measurements are enabled by micromachined thermal isolation platforms optimized for thermal conductivity measurements of thin-film systems. Electrical conductivity measurements on exactly the same samples allow application of the Wiedemann-Franz relation, which shows large nonelectronic contributions to thermal conductivity for the cobalt-iron alloy with 25% Co. This composition has been shown to have exceptionally low damping for a metallic FM. The thermal conductivity of a 75-nm-thick film of the 25% Co alloy changes by more than 20% at some temperatures, while a reference sample with 50% cobalt that has much higher damping shows no field-direction dependence. Our measurements indicate that applied magnetic fields alter the magnon lifetimes inmore »
- Authors:
-
- Univ. of Denver, CO (United States)
- National Inst. of Standards and Technology (NIST), Boulder, CO (United States)
- National Inst. of Standards and Technology (NIST), Boulder, CO (United States); Univ. of Colorado, Boulder, CO (United States)
- Publication Date:
- Research Org.:
- Los Alamos National Laboratory (LANL), Los Alamos, NM (United States). Center for Integrated Nanotechnologies (CINT)
- Sponsoring Org.:
- USDOE; National Science Foundation (NSF)
- OSTI Identifier:
- 1982833
- Grant/Contract Number:
- 89233218CNA000001; DMR-1709646; AC52-06NA25396; AC04-94AL85000
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review Materials
- Additional Journal Information:
- Journal Volume: 5; Journal Issue: 11; Journal ID: ISSN 2475-9953
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; Materials Science
Citation Formats
Natale, M. R., Wesenberg, D. J., Edwards, Eric J., Nembach, Hans T., Shaw, Justin M., and Zink, B. L. Field-dependent nonelectronic contributions to thermal conductivity in a metallic ferromagnet with low Gilbert damping. United States: N. p., 2021.
Web. doi:10.1103/physrevmaterials.5.l111401.
Natale, M. R., Wesenberg, D. J., Edwards, Eric J., Nembach, Hans T., Shaw, Justin M., & Zink, B. L. Field-dependent nonelectronic contributions to thermal conductivity in a metallic ferromagnet with low Gilbert damping. United States. https://doi.org/10.1103/physrevmaterials.5.l111401
Natale, M. R., Wesenberg, D. J., Edwards, Eric J., Nembach, Hans T., Shaw, Justin M., and Zink, B. L. Tue .
"Field-dependent nonelectronic contributions to thermal conductivity in a metallic ferromagnet with low Gilbert damping". United States. https://doi.org/10.1103/physrevmaterials.5.l111401. https://www.osti.gov/servlets/purl/1982833.
@article{osti_1982833,
title = {Field-dependent nonelectronic contributions to thermal conductivity in a metallic ferromagnet with low Gilbert damping},
author = {Natale, M. R. and Wesenberg, D. J. and Edwards, Eric J. and Nembach, Hans T. and Shaw, Justin M. and Zink, B. L.},
abstractNote = {Heat conduction in metals is typically dominated by electron transport since electrons carry both charge and heat. In magnetic metals magnons, or spin waves, excitations of the magnetic order can be used to transport information. Heat conduction via magnons has been previously shown mostly for insulating magnets with low Gilbert damping and resulting long spin-wave lifetimes where conduction electrons cannot contribute. Here we show that thin films of properly optimized metallic ferromagnetic (FM) alloys show significant nonelectronic contributions to heat conduction, which furthermore depend on the direction of an applied magnetic field. These measurements are enabled by micromachined thermal isolation platforms optimized for thermal conductivity measurements of thin-film systems. Electrical conductivity measurements on exactly the same samples allow application of the Wiedemann-Franz relation, which shows large nonelectronic contributions to thermal conductivity for the cobalt-iron alloy with 25% Co. This composition has been shown to have exceptionally low damping for a metallic FM. The thermal conductivity of a 75-nm-thick film of the 25% Co alloy changes by more than 20% at some temperatures, while a reference sample with 50% cobalt that has much higher damping shows no field-direction dependence. Our measurements indicate that applied magnetic fields alter the magnon lifetimes in these films and that these magnons contribute to thermal conductivity in this metallic magnetic alloy with low Gilbert damping.},
doi = {10.1103/physrevmaterials.5.l111401},
journal = {Physical Review Materials},
number = 11,
volume = 5,
place = {United States},
year = {Tue Nov 23 00:00:00 EST 2021},
month = {Tue Nov 23 00:00:00 EST 2021}
}
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