Exploring nonequilibrium phases of photo-doped Mott insulators with generalized Gibbs ensembles
Abstract
Many experiments show that strong excitations of correlated quantum materials can cause non-thermal phases without equilibrium analogues. Understanding the origin and properties of these nonequilibrium states has been challenging due to the limitations of theoretical methods for nonequilibrium strongly correlated systems. In this work, we introduce a generalized Gibbs ensemble description that enables a systematic analysis of the long-time behavior of photo-doped states in Mott insulators based on equilibrium methods. We demonstrate the power of the method by mapping out the nonequilibrium phase diagram of the one-dimensional extended Hubbard model, which featuresη-pairing and charge density wave phases in a wide photo-doping range. We furthermore clarify that the peculiar kinematics of photo-doped carriers, and the interaction between them, play an essential role in the formation of these non-thermal phases. Our results establish a new path for the systematic analysis of nonequilibrium strongly correlated systems.
- Authors:
-
[1];
[3];
[4];
[6]
- Tokyo Institute of Technology (Japan)
- Konan Univ., Kobe (Japan)
- Columbia Univ., New York, NY (United States)
- Jozef Stefan Inst. (IJS), Ljubljana (Slovenia); Univ. of Ljubljana (Slovenia)
- Columbia Univ., New York, NY (United States); Flatiron Institute, New York, NY (United States)
- Univ. of Fribourg (Switzerland)
- Publication Date:
- Research Org.:
- Columbia Univ., New York, NY (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC); Slovenian Research Agency (ARRS); JSPS KAKENHI
- OSTI Identifier:
- 1978732
- Grant/Contract Number:
- SC0019443; 724103; J1-2455; P1-0044; JP19K23425; JP20K14412; JP20H05265; JP21H05017; JP21K03412; JPMJCR1901; JPMJCR19T3
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Communications Physics
- Additional Journal Information:
- Journal Volume: 5; Journal Issue: 1; Journal ID: ISSN 2399-3650
- Publisher:
- Springer Nature
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 71 CLASSICAL AND QUANTUM MECHANICS, GENERAL PHYSICS; Physics; Electronic properties and materials; Phase transitions and critical phenomena
Citation Formats
Murakami, Yuta, Takayoshi, Shintaro, Kaneko, Tatsuya, Sun, Zhiyuan, Golež, Denis, Millis, Andrew J., and Werner, Philipp. Exploring nonequilibrium phases of photo-doped Mott insulators with generalized Gibbs ensembles. United States: N. p., 2022.
Web. doi:10.1038/s42005-021-00799-7.
Murakami, Yuta, Takayoshi, Shintaro, Kaneko, Tatsuya, Sun, Zhiyuan, Golež, Denis, Millis, Andrew J., & Werner, Philipp. Exploring nonequilibrium phases of photo-doped Mott insulators with generalized Gibbs ensembles. United States. https://doi.org/10.1038/s42005-021-00799-7
Murakami, Yuta, Takayoshi, Shintaro, Kaneko, Tatsuya, Sun, Zhiyuan, Golež, Denis, Millis, Andrew J., and Werner, Philipp. Thu .
"Exploring nonequilibrium phases of photo-doped Mott insulators with generalized Gibbs ensembles". United States. https://doi.org/10.1038/s42005-021-00799-7. https://www.osti.gov/servlets/purl/1978732.
@article{osti_1978732,
title = {Exploring nonequilibrium phases of photo-doped Mott insulators with generalized Gibbs ensembles},
author = {Murakami, Yuta and Takayoshi, Shintaro and Kaneko, Tatsuya and Sun, Zhiyuan and Golež, Denis and Millis, Andrew J. and Werner, Philipp},
abstractNote = {Many experiments show that strong excitations of correlated quantum materials can cause non-thermal phases without equilibrium analogues. Understanding the origin and properties of these nonequilibrium states has been challenging due to the limitations of theoretical methods for nonequilibrium strongly correlated systems. In this work, we introduce a generalized Gibbs ensemble description that enables a systematic analysis of the long-time behavior of photo-doped states in Mott insulators based on equilibrium methods. We demonstrate the power of the method by mapping out the nonequilibrium phase diagram of the one-dimensional extended Hubbard model, which featuresη-pairing and charge density wave phases in a wide photo-doping range. We furthermore clarify that the peculiar kinematics of photo-doped carriers, and the interaction between them, play an essential role in the formation of these non-thermal phases. Our results establish a new path for the systematic analysis of nonequilibrium strongly correlated systems.},
doi = {10.1038/s42005-021-00799-7},
journal = {Communications Physics},
number = 1,
volume = 5,
place = {United States},
year = {Thu Jan 13 00:00:00 EST 2022},
month = {Thu Jan 13 00:00:00 EST 2022}
}
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