DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Relative permeability of gas and water flow in hydrate-bearing porous media: A micro-scale study by lattice Boltzmann simulation

Abstract

The water-gas relative permeability is an important parameter to characterize multiphase flow in sediments. To study the water-gas relative permeability of hydrate-bearing porous media, multiphase flow simulations were carried out at the pore scale using the lattice Boltzmann method. In this work, the effects of hydrate saturation and hydrate-growth habits on the water-gas relative permeability, which is scaled by the relative permeability considering the hydrate only, were evaluated in a two-dimensional porous medium. Results show that the increase of hydrate saturation causes the decrease of water-gas effective permeability as expected. However, the effect of hydrate saturation on the water-gas relative permeability is different from that of hydrate saturation on the water-gas effective permeability. The water-gas relative permeability increases with the increase of hydrate saturation in the pore-filling case. The water-gas relative permeability decreases with the increase of hydrate saturation in the grain-coating case. The wettability of solid phase has a different effect on the relative permeability of wetting phase and nonwetting phase. The Jamin effect (phase blocking) was observed and may exist in the production of gas from natural gas hydrate reservoirs. This seriously affects the multiphase flow characteristics. The changes of microscale fluid distribution effect the changes of water-gasmore » relative permeability. The relationship between the water-gas relative permeability and the characterization parameters of microscale fluid distribution was analyzed.« less

Authors:
 [1];  [2];  [3];  [4];  [5];  [6];  [6];  [6];  [6]
  1. Ministry of Natural Resources, Qingdao (China); Qingdao National Laboratory for Marine Science and Technology (China); Ministry of Education, Qingdao (China); China University of Petroleum (East China), Qingdao (China)
  2. Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  3. Qingdao National Laboratory for Marine Science and Technology (China); Ministry of Education, Qingdao (China); China University of Petroleum (East China), Qingdao (China)
  4. Eidgenoessische Technische Hochschule (ETH), Zurich (Switzerland)
  5. Ministry of Natural Resources, Qingdao (China); Qingdao National Laboratory for Marine Science and Technology (China)
  6. Ministry of Education, Qingdao (China); China University of Petroleum (East China), Qingdao (China)
Publication Date:
Research Org.:
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); Major Scientific and Technological Projects of CNPC; China Postdoctoral Science Foundation; USDOE Office of Fossil Energy (FE); Swiss National Science Foundation (SNF); National Natural Science Foundation of China (NSFC); Shandong Provincial Natural Science Foundation
OSTI Identifier:
1896479
Grant/Contract Number:  
AC02-05CH11231; 51625403; ZD2019-184-002; 2021M701815; SDBX2021015; 41876051; 52004319; ZR201910220407
Resource Type:
Accepted Manuscript
Journal Name:
Fuel
Additional Journal Information:
Journal Volume: 321; Journal ID: ISSN 0016-2361
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
58 GEOSCIENCES; Relative permeability; Gas hydrate; Porous media; Fluid distribution; LBM

Citation Formats

Ji, Yunkai, Kneafsey, Timothy J., Hou, Jian, Zhao, Jianlin, Liu, Changling, Guo, Tiankui, Wei, Bei, Zhao, Ermeng, and Bai, Yajie. Relative permeability of gas and water flow in hydrate-bearing porous media: A micro-scale study by lattice Boltzmann simulation. United States: N. p., 2022. Web. doi:10.1016/j.fuel.2022.124013.
Ji, Yunkai, Kneafsey, Timothy J., Hou, Jian, Zhao, Jianlin, Liu, Changling, Guo, Tiankui, Wei, Bei, Zhao, Ermeng, & Bai, Yajie. Relative permeability of gas and water flow in hydrate-bearing porous media: A micro-scale study by lattice Boltzmann simulation. United States. https://doi.org/10.1016/j.fuel.2022.124013
Ji, Yunkai, Kneafsey, Timothy J., Hou, Jian, Zhao, Jianlin, Liu, Changling, Guo, Tiankui, Wei, Bei, Zhao, Ermeng, and Bai, Yajie. Thu . "Relative permeability of gas and water flow in hydrate-bearing porous media: A micro-scale study by lattice Boltzmann simulation". United States. https://doi.org/10.1016/j.fuel.2022.124013. https://www.osti.gov/servlets/purl/1896479.
@article{osti_1896479,
title = {Relative permeability of gas and water flow in hydrate-bearing porous media: A micro-scale study by lattice Boltzmann simulation},
author = {Ji, Yunkai and Kneafsey, Timothy J. and Hou, Jian and Zhao, Jianlin and Liu, Changling and Guo, Tiankui and Wei, Bei and Zhao, Ermeng and Bai, Yajie},
abstractNote = {The water-gas relative permeability is an important parameter to characterize multiphase flow in sediments. To study the water-gas relative permeability of hydrate-bearing porous media, multiphase flow simulations were carried out at the pore scale using the lattice Boltzmann method. In this work, the effects of hydrate saturation and hydrate-growth habits on the water-gas relative permeability, which is scaled by the relative permeability considering the hydrate only, were evaluated in a two-dimensional porous medium. Results show that the increase of hydrate saturation causes the decrease of water-gas effective permeability as expected. However, the effect of hydrate saturation on the water-gas relative permeability is different from that of hydrate saturation on the water-gas effective permeability. The water-gas relative permeability increases with the increase of hydrate saturation in the pore-filling case. The water-gas relative permeability decreases with the increase of hydrate saturation in the grain-coating case. The wettability of solid phase has a different effect on the relative permeability of wetting phase and nonwetting phase. The Jamin effect (phase blocking) was observed and may exist in the production of gas from natural gas hydrate reservoirs. This seriously affects the multiphase flow characteristics. The changes of microscale fluid distribution effect the changes of water-gas relative permeability. The relationship between the water-gas relative permeability and the characterization parameters of microscale fluid distribution was analyzed.},
doi = {10.1016/j.fuel.2022.124013},
journal = {Fuel},
number = ,
volume = 321,
place = {United States},
year = {Thu Mar 31 00:00:00 EDT 2022},
month = {Thu Mar 31 00:00:00 EDT 2022}
}

Works referenced in this record:

Dynamic response of oceanic hydrate deposits to ocean temperature change: DYNAMIC RESPONSE OF OCEANIC HYDRATES
journal, December 2008

  • Reagan, Matthew T.; Moridis, George J.
  • Journal of Geophysical Research: Oceans, Vol. 113, Issue C12
  • DOI: 10.1029/2008JC004938

A huff-and-puff production of gas hydrate deposits in Shenhu area of South China Sea through a vertical well
journal, May 2012


A Nonempirical Relative Permeability Model for Hydrate-Bearing Sediments
journal, April 2019

  • Singh, Harpreet; Myshakin, Evgeniy M.; Seol, Yongkoo
  • SPE Journal, Vol. 24, Issue 02
  • DOI: 10.2118/193996-PA

The water retention curve and relative permeability for gas production from hydrate-bearing sediments: pore-network model simulation: WATER RETENTION AND PERMEABILITY
journal, August 2016

  • Mahabadi, Nariman; Dai, Sheng; Seol, Yongkoo
  • Geochemistry, Geophysics, Geosystems, Vol. 17, Issue 8
  • DOI: 10.1002/2016GC006372

Evolution of gas saturation and relative permeability during gas production from hydrate-bearing sediments: Gas invasion vs. gas nucleation: GAS INVASION VS. GAS SATURATION
journal, January 2014

  • Jang, Jaewon; Santamarina, J. Carlos
  • Journal of Geophysical Research: Solid Earth, Vol. 119, Issue 1
  • DOI: 10.1002/2013JB010480

Experimental Investigation of Production Behavior of Methane Hydrate under Ethylene Glycol Injection in Unconsolidated Sediment
journal, November 2007

  • Li, Gang; Li, Xiao-Sen; Tang, Liang-Guang
  • Energy & Fuels, Vol. 21, Issue 6
  • DOI: 10.1021/ef060644d

Pore scale simulation of liquid and gas two-phase flow based on digital core technology
journal, July 2015


Study on the meniscus-induced motion of droplets and bubbles by a three-phase Lattice Boltzmann model
journal, February 2018


Permeability measurements of quartz sands with methane hydrate
journal, January 2019


Production behavior and numerical analysis for 2017 methane hydrate extraction test of Shenhu, South China Sea
journal, May 2018

  • Chen, Lin; Feng, Yongchang; Okajima, Junnosuke
  • Journal of Natural Gas Science and Engineering, Vol. 53
  • DOI: 10.1016/j.jngse.2018.02.029

Gas hydrates: entrance to a methane age or climate threat?
journal, July 2009


Gas production potential of disperse low-saturation hydrate accumulations in oceanic sediments
journal, June 2007


Pore-Scale Simulations of Gas Displacing Liquid in a Homogeneous Pore Network Using the Lattice Boltzmann Method
journal, July 2013


Pore-scale investigation of viscous coupling effects for two-phase flow in porous media
journal, August 2005


A lattice Boltzmann study of viscous coupling effects in immiscible two-phase flow in porous media
journal, June 2007

  • Yiotis, Andreas G.; Psihogios, John; Kainourgiakis, Michael E.
  • Colloids and Surfaces A: Physicochemical and Engineering Aspects, Vol. 300, Issue 1-2
  • DOI: 10.1016/j.colsurfa.2006.12.045

Using similarity theory to design natural gas hydrate experimental model
journal, January 2015


The Effect of Wettability Heterogeneity on Relative Permeability of Two-Phase Flow in Porous Media: A Lattice Boltzmann Study
journal, February 2018

  • Zhao, Jianlin; Kang, Qinjun; Yao, Jun
  • Water Resources Research, Vol. 54, Issue 2
  • DOI: 10.1002/2017WR021443

Relative permeabilities and coupling effects in steady-state gas-liquid flow in porous media: A lattice Boltzmann study
journal, September 2009

  • Huang, Haibo; Lu, Xi-yun
  • Physics of Fluids, Vol. 21, Issue 9
  • DOI: 10.1063/1.3225144

Relative permeability to water or gas in the presence of hydrates in porous media from critical path analysis
journal, October 2016


Simulation of Depressurization for Gas Production From Gas Hydrate Reservoirs
journal, November 2005

  • Hong, H.; Pooladi-Darvish, M.
  • Journal of Canadian Petroleum Technology, Vol. 44, Issue 11
  • DOI: 10.2118/05-11-03

Simulation of CO2 storage and methane gas production from gas hydrates in a large scale laboratory reactor
journal, November 2016

  • Castellani, Beatrice; Rossetti, Giacomo; Tupsakhare, Swanand
  • Journal of Petroleum Science and Engineering, Vol. 147
  • DOI: 10.1016/j.petrol.2016.09.016

Relative water and gas permeability for gas production from hydrate-bearing sediments
journal, June 2014

  • Mahabadi, Nariman; Jang, Jaewon
  • Geochemistry, Geophysics, Geosystems, Vol. 15, Issue 6
  • DOI: 10.1002/2014GC005331

Interfacial tension measurements in water−methane system at temperatures from 278.15 K to 298.15 K and pressures up to 10 MPa
journal, April 2016


Key Factors for Depressurization-Induced Gas Production from Oceanic Methane Hydrates
journal, March 2010

  • Konno, Yoshihiro; Masuda, Yoshihiro; Hariguchi, Yosuke
  • Energy & Fuels, Vol. 24, Issue 3
  • DOI: 10.1021/ef901115h

Deep sea NMR: Methane hydrate growth habit in porous media and its relationship to hydraulic permeability, deposit accumulation, and submarine slope stability: DEEP SEA NMR
journal, October 2003

  • Kleinberg, R. L.; Flaum, C.; Griffin, D. D.
  • Journal of Geophysical Research: Solid Earth, Vol. 108, Issue B10
  • DOI: 10.1029/2003JB002389

Effect of Viscosity Ratio on Relative Permeability (includes associated paper 1496-G)
journal, December 1959

  • Odeh, A. S.
  • Transactions of the AIME, Vol. 216, Issue 01
  • DOI: 10.2118/1189-G

Evaluation of Gas Production Potential from Marine Gas Hydrate Deposits in Shenhu Area of South China Sea
journal, November 2010

  • Li, Gang; Moridis, George J.; Zhang, Keni
  • Energy & Fuels, Vol. 24, Issue 11
  • DOI: 10.1021/ef100930m

Methane hydrates bearing synthetic sediments—Experimental and numerical approaches of the dissociation
journal, October 2009


Multiple-relaxation-time color-gradient lattice Boltzmann model for simulating two-phase flows with high density ratio
journal, August 2016


Production performance of gas hydrate accumulation at the GMGS2-Site 16 of the Pearl River Mouth Basin in the South China Sea
journal, November 2015


Masuda’s sandstone core hydrate dissociation experiment revisited
journal, January 2018


Inhibitory effect of water-based drilling fluid on methane hydrate dissociation
journal, May 2019


A Counter-Current Heat-Exchange Reactor for the Thermal Stimulation of Hydrate-Bearing Sediments
journal, June 2013

  • Schicks, Judith; Spangenberg, Erik; Giese, Ronny
  • Energies, Vol. 6, Issue 6
  • DOI: 10.3390/en6063002

Characterization of natural gas hydrate recovered from Pearl River Mouth basin in South China Sea
journal, March 2015


Effect of hydrate nucleation mechanisms and capillarity on permeability reduction in granular media: NUCLEATION-DEPENDENT PERMEABILITY
journal, September 2016

  • Kang, Dong Hun; Yun, Tae Sup; Kim, Kwang Yeom
  • Geophysical Research Letters, Vol. 43, Issue 17
  • DOI: 10.1002/2016GL070511

Pore-scale simulation of liquid CO2 displacement of water using a two-phase lattice Boltzmann model
journal, November 2014


Analysis of formation pressure test results in the Mount Elbert methane hydrate reservoir through numerical simulation
journal, February 2011


The use of huff and puff method in a single horizontal well in gas production from marine gas hydrate deposits in the Shenhu Area of South China Sea
journal, April 2011

  • Li, Gang; Moridis, George J.; Zhang, Keni
  • Journal of Petroleum Science and Engineering, Vol. 77, Issue 1
  • DOI: 10.1016/j.petrol.2011.02.009

Lattice Boltzmann model for crystal growth from supersaturated solution: CRYSTAL GROWTH FROM SUPERSATURATED SOLUTION
journal, November 2004

  • Kang, Qinjun; Zhang, Dongxiao; Lichtner, Peter C.
  • Geophysical Research Letters, Vol. 31, Issue 21
  • DOI: 10.1029/2004GL021107

Permeability of hydrate-bearing sediments
journal, March 2020


Analysis of the influence of wettability on permeability in hydrate-bearing porous media using pore network models combined with computed tomography
journal, September 2015


Techno-economic forecasting of a hypothetical gas hydrate field in the offshore of India
journal, October 2019


Numerical simulation of gas production from hydrate-bearing sediments in the Shenhu area by depressurising: The effect of burden permeability
journal, December 2015


A new hydrate deposition prediction model for gas-dominated systems with free water
journal, May 2017


Influence of reservoir permeability on methane hydrate dissociation by depressurization
journal, December 2016


A Study of the Effects of Colloidal Gas Aphron Composition on Pore Blocking
journal, October 2010

  • Bjorndalen, N. .; Alvarez, J. M. . M.; Jossy, W. E. . E.
  • SPE Drilling & Completion, Vol. 26, Issue 01
  • DOI: 10.2118/121417-PA

Computational modeling of methane hydrate dissociation in a sandstone core
journal, November 2007


Validation of a Modified Carman-Kozeny Equation To Model Two-Phase Relative Permeabilities
conference, October 1999

  • Alpak, Faruk O.; Lake, Larry W.; Embid, Sonia M.
  • SPE Annual Technical Conference and Exhibition, All Days
  • DOI: 10.2118/56479-MS

Effect of hydrate on permeability in porous media: Pore-scale micro-simulation
journal, November 2018


Study on the relations between controlling mechanisms and dissociation front of gas hydrate reservoirs
journal, April 2018


Pore scale study of amphiphilic fluids flow using the Lattice Boltzmann model
journal, August 2019