Magnetic terahertz resonances above the Néel temperature in the frustrated kagome antiferromagnet averievite
Abstract
Time-domain magneto-THz spectroscopy is utilized to study the frustrated magnet averievite Cu5–xZnxV2O10(CsCl). Pronounced THz resonances are observed in unsubstituted samples (x = 0) when cooling below the onset of short-range magnetic correlations. The influence of external magnetic effects confirms the magnetic origin of these resonances. Increasing Zn substitution suppresses the resonances, as frustration effects dominate, reflecting the nonmagnetic phases for x > 0.25 compounds. The temperature evolution of the THz spectra is complemented with electron spin resonance spectroscopy. This comparison allows a direct probe of the different contributions from magnetic order, frustration, and structural properties in the phase diagram of averievite. Furthermore, our results illustrate the effect of magnetic interactions in THz spectra of frustrated magnets.
- Authors:
-
[1];
[1];
[2];
[3];
- Univ. Stuttgart (Germany)
- TU Wien, Vienna (Austria)
- Argonne National Lab. (ANL), Argonne, IL (United States)
- Publication Date:
- Research Org.:
- Argonne National Laboratory (ANL), Argonne, IL (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; German Research Foundation (DFG)
- OSTI Identifier:
- 1868999
- Grant/Contract Number:
- AC02-06CH11357
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review. B
- Additional Journal Information:
- Journal Volume: 105; Journal Issue: 6; Journal ID: ISSN 2469-9950
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Frustrated magnetism; Magnetic order; Quantum spin liquid; Spin dynamics; Kagome lattice; Electron spin resonance; Terahertz time-domain spectroscopy
Citation Formats
Biesner, Tobias, Roh, Seulki, Pustogow, Andrej, Zheng, Hong, Mitchell, J. F., and Dressel, Martin. Magnetic terahertz resonances above the Néel temperature in the frustrated kagome antiferromagnet averievite. United States: N. p., 2022.
Web. doi:10.1103/physrevb.105.l060410.
Biesner, Tobias, Roh, Seulki, Pustogow, Andrej, Zheng, Hong, Mitchell, J. F., & Dressel, Martin. Magnetic terahertz resonances above the Néel temperature in the frustrated kagome antiferromagnet averievite. United States. https://doi.org/10.1103/physrevb.105.l060410
Biesner, Tobias, Roh, Seulki, Pustogow, Andrej, Zheng, Hong, Mitchell, J. F., and Dressel, Martin. Fri .
"Magnetic terahertz resonances above the Néel temperature in the frustrated kagome antiferromagnet averievite". United States. https://doi.org/10.1103/physrevb.105.l060410. https://www.osti.gov/servlets/purl/1868999.
@article{osti_1868999,
title = {Magnetic terahertz resonances above the Néel temperature in the frustrated kagome antiferromagnet averievite},
author = {Biesner, Tobias and Roh, Seulki and Pustogow, Andrej and Zheng, Hong and Mitchell, J. F. and Dressel, Martin},
abstractNote = {Time-domain magneto-THz spectroscopy is utilized to study the frustrated magnet averievite Cu5–xZnxV2O10(CsCl). Pronounced THz resonances are observed in unsubstituted samples (x = 0) when cooling below the onset of short-range magnetic correlations. The influence of external magnetic effects confirms the magnetic origin of these resonances. Increasing Zn substitution suppresses the resonances, as frustration effects dominate, reflecting the nonmagnetic phases for x > 0.25 compounds. The temperature evolution of the THz spectra is complemented with electron spin resonance spectroscopy. This comparison allows a direct probe of the different contributions from magnetic order, frustration, and structural properties in the phase diagram of averievite. Furthermore, our results illustrate the effect of magnetic interactions in THz spectra of frustrated magnets.},
doi = {10.1103/physrevb.105.l060410},
journal = {Physical Review. B},
number = 6,
volume = 105,
place = {United States},
year = {Fri Feb 25 00:00:00 EST 2022},
month = {Fri Feb 25 00:00:00 EST 2022}
}
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