Static and dynamic magnetic properties of honeycomb lattice antiferromagnets Na 2 M 2 TeO 6 , M = Co and Ni

Samarakoon, Anjana M.; Chen, Qiang; Zhou, Haidong; Garlea, V. Ovidiu

doi:10.1103/physrevb.104.184415

Title: Static and dynamic magnetic properties of honeycomb lattice antiferromagnets ${Na}_{2} M_{2} {TeO}_{6}$ , $M = Co$ and Ni

Abstract

The magnetic structures and spin dynamics of ${Na}_{2} {CO}_{2} {TeO}_{6}$ and ${Na}_{2} {Ni}_{2} {TeO}_{6}$ are investigated by means of elastic and inelastic neutron scattering measurements and the results are discussed in the context of a generalized Kitaev-Heisenberg model on a honeycomb lattice with strong spin-orbit coupling. The large number of parameters involved in the Hamiltonian model is evaluated by using an iterative optimization algorithm capable of extracting model solutions and simultaneously estimating their uncertainty. The analyses indicate that both Co²⁺ (d⁷) and Ni²⁺ (d⁸) antiferromagnets realize bond-dependent anisotropic nearest-neighbor interactions and support the theoretical predictions for the realization of Kitaev physics in 3 d electron systems with effective spins S = 1/2 and 1. By studying the Na-doped system Na_2.4Ni₂TeO₆, we show that the control of Na content can provide an effective route for fine-tuning the magnetic lattice dimensionality, as well as to controlling the bond-dependent anisotropic interactions.

Authors:

Samarakoon, Anjana M. ^[1];

^[2]; Zhou, Haidong ^[2];

^[3]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Argonne National Lab. (ANL), Argonne, IL (United States)
Univ. of Tennessee, Knoxville, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Publication Date:: Mon Nov 15 00:00:00 EST 2021

Research Org.:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Sponsoring Org.:: USDOE Office of Science (SC)

OSTI Identifier:: 1831674

Grant/Contract Number:: AC05-00OR22725; DMR-2003117

Resource Type:: Accepted Manuscript

Journal Name:: Physical Review B

Additional Journal Information:: Journal Volume: 104; Journal Issue: 18; Journal ID: ISSN 2469-9950

Publisher:: American Physical Society (APS)

Country of Publication:: United States

Language:: English

Subject:: 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY

Citation Formats


                    Samarakoon, Anjana M., Chen, Qiang, Zhou, Haidong, and Garlea, V. Ovidiu. Static and dynamic magnetic properties of honeycomb lattice antiferromagnets Na 2 M 2 TeO 6 , M = Co and Ni.  United States: N. p., 2021. 
Web.  doi:10.1103/physrevb.104.184415.

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                    Samarakoon, Anjana M., Chen, Qiang, Zhou, Haidong, & Garlea, V. Ovidiu. Static and dynamic magnetic properties of honeycomb lattice antiferromagnets Na 2 M 2 TeO 6 , M = Co and Ni.  United States.  https://doi.org/10.1103/physrevb.104.184415

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                    Samarakoon, Anjana M., Chen, Qiang, Zhou, Haidong, and Garlea, V. Ovidiu. Mon .  
"Static and dynamic magnetic properties of honeycomb lattice antiferromagnets Na 2 M 2 TeO 6 , M = Co and Ni".  United States.  https://doi.org/10.1103/physrevb.104.184415.  https://www.osti.gov/servlets/purl/1831674.

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@article{osti_1831674,

  title        = {Static and dynamic magnetic properties of honeycomb lattice antiferromagnets Na 2 M 2 TeO 6 , M = Co and Ni},

  author       = {Samarakoon, Anjana M. and Chen, Qiang and Zhou, Haidong and Garlea, V. Ovidiu},

  abstractNote = {The magnetic structures and spin dynamics of Na 2 CO 2 TeO 6 and Na 2 Ni 2 TeO 6 are investigated by means of elastic and inelastic neutron scattering measurements and the results are discussed in the context of a generalized Kitaev-Heisenberg model on a honeycomb lattice with strong spin-orbit coupling. The large number of parameters involved in the Hamiltonian model is evaluated by using an iterative optimization algorithm capable of extracting model solutions and simultaneously estimating their uncertainty. The analyses indicate that both Co2+ (d7) and Ni2+ (d8) antiferromagnets realize bond-dependent anisotropic nearest-neighbor interactions and support the theoretical predictions for the realization of Kitaev physics in 3 d electron systems with effective spins S = 1/2 and 1. By studying the Na-doped system Na2.4Ni2TeO6, we show that the control of Na content can provide an effective route for fine-tuning the magnetic lattice dimensionality, as well as to controlling the bond-dependent anisotropic interactions.},

  doi          = {10.1103/physrevb.104.184415},

  journal      = {Physical Review B},

  number       = 18,

  volume       = 104,

  place        = {United States},

  year         = {Mon Nov 15 00:00:00 EST 2021},

  month        = {Mon Nov 15 00:00:00 EST 2021}

}

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Title: Static and dynamic magnetic properties of honeycomb lattice antiferromagnets Na 2 M 2 TeO 6 , M = Co and Ni

Abstract

Citation Formats

Rethinking α − RuCl 3 journal, July 2020

Possible Kitaev Quantum Spin Liquid State in 2D Materials with S = 3 / 2 journal, February 2020

Pseudospin exchange interactions in d 7 cobalt compounds: Possible realization of the Kitaev model journal, January 2018

Spin-1 Kitaev-Heisenberg model on a honeycomb lattice journal, September 2020

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Anyons in an exactly solved model and beyond journal, January 2006

Concept and realization of Kitaev quantum spin liquids journal, March 2019

Kitaev-Heisenberg Hamiltonian for high-spin d 7 Mott insulators journal, January 2018

Magnetic properties of the honeycomb oxide Na 2 Co 2 TeO 6 journal, December 2016

Symmetry-Based Computational Tools for Magnetic Crystallography journal, July 2015

Structure and basic magnetic properties of the honeycomb lattice compounds Na2Co2TeO6 and Na3Co2SbO6 journal, March 2007

Magnetic order in single crystals of Na 3 Co 2 SbO 6 with a honeycomb arrangement of 3 d 7 Co 2 + ions journal, July 2019

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Kitaev Spin Liquid in 3 d Transition Metal Compounds journal, July 2020

Studies on solid solutions based on layered honeycomb-ordered phases P2-Na2M2TeO6 (M=Co, Ni, Zn) journal, December 2012

Recent advances in magnetic structure determination by neutron powder diffraction journal, October 1993

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Generic Spin Model for the Honeycomb Iridates beyond the Kitaev Limit journal, February 2014

Tensor network wave function of S = 1 Kitaev spin liquids journal, August 2020

Hunting Majorana Fermions in Kitaev Magnets journal, January 2020

Machine-learning-assisted insight into spin ice Dy2Ti2O7 journal, February 2020

Crystal growth and magnetic ordering of Na 2 Ni 2 TeO 6 with honeycomb layers and Na 2 Cu 2 TeO 6 with Cu spin dimers journal, January 2014

Kitaev interactions in the Co honeycomb antiferromagnets Na 3 Co 2 SbO 6 and Na 2 Co 2 TeO 6 journal, December 2020

VESTA 3 for three-dimensional visualization of crystal, volumetric and morphology data journal, October 2011

Orbitally induced hierarchy of exchange interactions in the zigzag antiferromagnetic state of honeycomb silver delafossite Ag 3 Co 2 SbO 6 journal, January 2016

Microscopic Mechanism for a Higher-Spin Kitaev Model journal, July 2019

Kitaev-Heisenberg- J 2 - J 3 model for the iridates A 2 IrO 3 journal, November 2011

Zigzag antiferromagnetic ground state with anisotropic correlation lengths in the quasi-two-dimensional honeycomb lattice compound N a 2 C o 2 Te O 6 journal, March 2017

Spin Correlations and Short‐Range Magnetic Order in the Honeycomb‐Layered Na 2 Ni 2 TeO 6 journal, August 2019

Competing antiferromagnetic-ferromagnetic states in a d 7 Kitaev honeycomb magnet journal, December 2020

Structure and Magnetic Properties of the α-NaFeO 2 -Type Honeycomb Compound Na 3 Ni 2 BiO 6 journal, November 2013

Zig-zag magnetic ordering in honeycomb-layered Na3Co2SbO6 journal, November 2016

Interplay between Kitaev interaction and single ion anisotropy in ferromagnetic CrI3 and CrGeTe3 monolayers journal, November 2018

Spin-orbit phase behavior of Na 2 Co 2 TeO 6 at low temperatures journal, May 2021

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A New Family of Fast Sodium Ion Conductors: Na 2 M 2 TeO 6 (M = Ni, Co, Zn, Mg) journal, March 2011

Materials design of Kitaev spin liquids beyond the Jackeli–Khaliullin mechanism journal, June 2020

Recent progress on HYSPEC, and its polarization analysis capabilities journal, January 2015

Linear spin wave theory for single-Q incommensurate magnetic structures journal, March 2015

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Title: Static and dynamic magnetic properties of honeycomb lattice antiferromagnets ${Na}_{2} M_{2} {TeO}_{6}$ , $M = Co$ and Ni

Rethinking $α − {RuCl}_{3}$
journal, July 2020

Possible Kitaev Quantum Spin Liquid State in 2D Materials with $S = 3 / 2$
journal, February 2020

Pseudospin exchange interactions in $d^{7}$ cobalt compounds: Possible realization of the Kitaev model
journal, January 2018

Spin-1 Kitaev-Heisenberg model on a honeycomb lattice
journal, September 2020

Ferrimagnetism and anisotropic phase tunability by magnetic fields in ${Na}_{2} {Co}_{2} {TeO}_{6}$
journal, February 2020

Anyons in an exactly solved model and beyond
journal, January 2006

Concept and realization of Kitaev quantum spin liquids
journal, March 2019

Kitaev-Heisenberg Hamiltonian for high-spin $d^{7}$ Mott insulators
journal, January 2018

Magnetic properties of the honeycomb oxide ${Na}_{2} {Co}_{2} {TeO}_{6}$
journal, December 2016

Symmetry-Based Computational Tools for Magnetic Crystallography
journal, July 2015

Structure and basic magnetic properties of the honeycomb lattice compounds Na2Co2TeO6 and Na3Co2SbO6
journal, March 2007

Magnetic order in single crystals of ${Na}_{3} {Co}_{2} {SbO}_{6}$ with a honeycomb arrangement of ${3 d}^{7} {Co}^{2 +}$ ions
journal, July 2019

Field-induced quantum spin disordered state in spin-1/2 honeycomb magnet Na2Co2TeO6
journal, September 2021

Kitaev Spin Liquid in $3 d$ Transition Metal Compounds
journal, July 2020

Studies on solid solutions based on layered honeycomb-ordered phases P2-Na2M2TeO6 (M=Co, Ni, Zn)
journal, December 2012

Recent advances in magnetic structure determination by neutron powder diffraction
journal, October 1993

Models and materials for generalized Kitaev magnetism
journal, November 2017

Generic Spin Model for the Honeycomb Iridates beyond the Kitaev Limit
journal, February 2014

Tensor network wave function of $S = 1$ Kitaev spin liquids
journal, August 2020

Hunting Majorana Fermions in Kitaev Magnets
journal, January 2020

Machine-learning-assisted insight into spin ice Dy2Ti2O7
journal, February 2020

Crystal growth and magnetic ordering of Na ₂ Ni ₂ TeO ₆ with honeycomb layers and Na ₂ Cu ₂ TeO ₆ with Cu spin dimers
journal, January 2014

Kitaev interactions in the Co honeycomb antiferromagnets ${Na}_{3} {Co}_{2} {SbO}_{6}$ and ${Na}_{2} {Co}_{2} {TeO}_{6}$
journal, December 2020

VESTA 3 for three-dimensional visualization of crystal, volumetric and morphology data
journal, October 2011

Orbitally induced hierarchy of exchange interactions in the zigzag antiferromagnetic state of honeycomb silver delafossite Ag ₃ Co ₂ SbO ₆
journal, January 2016

Microscopic Mechanism for a Higher-Spin Kitaev Model
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Kitaev-Heisenberg- $J_{2}$ - $J_{3}$ model for the iridates $A_{2}$ IrO $_{3}$
journal, November 2011

Zigzag antiferromagnetic ground state with anisotropic correlation lengths in the quasi-two-dimensional honeycomb lattice compound $N a_{2} C o_{2} Te O_{6}$
journal, March 2017

Spin Correlations and Short‐Range Magnetic Order in the Honeycomb‐Layered Na ₂ Ni ₂ TeO ₆
journal, August 2019

Competing antiferromagnetic-ferromagnetic states in a $d^{7}$ Kitaev honeycomb magnet
journal, December 2020

Structure and Magnetic Properties of the α-NaFeO ₂ -Type Honeycomb Compound Na ₃ Ni ₂ BiO ₆
journal, November 2013

Zig-zag magnetic ordering in honeycomb-layered Na3Co2SbO6
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Interplay between Kitaev interaction and single ion anisotropy in ferromagnetic CrI3 and CrGeTe3 monolayers
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Spin-orbit phase behavior of ${Na}_{2} {Co}_{2} {TeO}_{6}$ at low temperatures
journal, May 2021

Long-range and short-range ordering in 2D honeycomb-lattice magnet Na2Ni2TeO6
journal, April 2020

Topological Spin Excitations in Honeycomb Ferromagnet ${CrI}_{3}$
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A New Family of Fast Sodium Ion Conductors: Na ₂ M ₂ TeO ₆ (M = Ni, Co, Zn, Mg)
journal, March 2011

Materials design of Kitaev spin liquids beyond the Jackeli–Khaliullin mechanism
journal, June 2020

Recent progress on HYSPEC, and its polarization analysis capabilities
journal, January 2015

Linear spin wave theory for single-Q incommensurate magnetic structures
journal, March 2015

The high-resolution powder diffractometer at the high flux isotope reactor
journal, March 2010

Mott Insulators in the Strong Spin-Orbit Coupling Limit: From Heisenberg to a Quantum Compass and Kitaev Models
journal, January 2009

Exotic Magnetic Field-Induced Spin-Superstructures in a Mixed Honeycomb-Triangular Lattice System
journal, February 2019