Supramolecular Energy Materials
Abstract
Abstract Self‐assembly is a bioinspired strategy to craft materials for renewable and clean energy technologies. In plants, the alignment and assembly of the light‐harvesting protein machinery in the green leaf optimize the ability to efficiently convert light from the sun to form chemical bonds. In artificial systems, strategies based on self‐assembly using noncovalent interactions offer the possibility to mimic this functional correlation among molecules to optimize photocatalysis, photovoltaics, and energy storage. One of the long‐term objectives of the field described here as supramolecular energy materials is to learn how to design soft materials containing light‐harvesting assemblies and catalysts to generate fuels and useful chemicals. Supramolecular energy materials also hold great potential in the design of systems for photovoltaics in which intermolecular interactions in self‐assembled structures, for example, in electron donor and acceptor phases, maximize charge transport and avoid exciton recombination. Possible pathways to integrate organic and inorganic structures by templating strategies and electrodeposition to create materials relevant to energy challenges including photoconductors and supercapacitors are also described. The final topic discussed is the synthesis of hybrid perovskites in which organic molecules are used to modify both structure and functions, which may include chemical stability, photovoltaics, and light emission.
- Authors:
-
- Northwestern Univ., Evanston, IL (United States)
- Northwestern Univ., Evanston, IL (United States); Northwestern Univ., Chicago, IL (United States)
- Publication Date:
- Research Org.:
- Energy Frontier Research Centers (EFRC) (United States). Center for Bio-Inspired Energy Science (CBES)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1822875
- Alternate Identifier(s):
- OSTI ID: 1604217
- Grant/Contract Number:
- FG02-00ER45810
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 32; Journal Issue: 17; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 99 GENERAL AND MISCELLANEOUS; supramolecular chemistry; self-assembly; soft materials; solar cells; photocatalysis; hybrid materials
Citation Formats
Dumele, Oliver, Chen, Jiahao, Passarelli, James V., and Stupp, Samuel I. Supramolecular Energy Materials. United States: N. p., 2020.
Web. doi:10.1002/adma.201907247.
Dumele, Oliver, Chen, Jiahao, Passarelli, James V., & Stupp, Samuel I. Supramolecular Energy Materials. United States. https://doi.org/10.1002/adma.201907247
Dumele, Oliver, Chen, Jiahao, Passarelli, James V., and Stupp, Samuel I. Thu .
"Supramolecular Energy Materials". United States. https://doi.org/10.1002/adma.201907247. https://www.osti.gov/servlets/purl/1822875.
@article{osti_1822875,
title = {Supramolecular Energy Materials},
author = {Dumele, Oliver and Chen, Jiahao and Passarelli, James V. and Stupp, Samuel I.},
abstractNote = {Abstract Self‐assembly is a bioinspired strategy to craft materials for renewable and clean energy technologies. In plants, the alignment and assembly of the light‐harvesting protein machinery in the green leaf optimize the ability to efficiently convert light from the sun to form chemical bonds. In artificial systems, strategies based on self‐assembly using noncovalent interactions offer the possibility to mimic this functional correlation among molecules to optimize photocatalysis, photovoltaics, and energy storage. One of the long‐term objectives of the field described here as supramolecular energy materials is to learn how to design soft materials containing light‐harvesting assemblies and catalysts to generate fuels and useful chemicals. Supramolecular energy materials also hold great potential in the design of systems for photovoltaics in which intermolecular interactions in self‐assembled structures, for example, in electron donor and acceptor phases, maximize charge transport and avoid exciton recombination. Possible pathways to integrate organic and inorganic structures by templating strategies and electrodeposition to create materials relevant to energy challenges including photoconductors and supercapacitors are also described. The final topic discussed is the synthesis of hybrid perovskites in which organic molecules are used to modify both structure and functions, which may include chemical stability, photovoltaics, and light emission.},
doi = {10.1002/adma.201907247},
journal = {Advanced Materials},
number = 17,
volume = 32,
place = {United States},
year = {Thu Mar 12 00:00:00 EDT 2020},
month = {Thu Mar 12 00:00:00 EDT 2020}
}
Web of Science
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