DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Diffraction gratings with two-orders-of-magnitude-enhanced dispersion rates for sub-meV resolution soft X-ray spectroscopy

Abstract

Diffraction gratings with large angular dispersion rates are central to obtaining high spectral resolution in grating spectrometers operating over a broad spectral range from infrared to soft X-ray domains. The greatest challenge is of course to achieve large dispersion rates in the short-wavelength X-ray domain. Here it is shown that crystals in non-coplanar asymmetric X-ray Bragg diffraction can function as high-reflectance broadband soft X-ray diffraction gratings with dispersion rates that are at least two orders of magnitude larger than those that are possible with state-of-the-art man-made gratings. Additionally, this opens new opportunities to design and implement soft X-ray resonant inelastic scattering (RIXS) spectrometers with spectral resolutions that are up to two orders of magnitude higher than what is currently possible, to further advance a very dynamic field of RIXS spectroscopy, and to make it competitive with inelastic neutron scattering. Examples of large-dispersion-rate crystal diffraction gratings operating near the 930 eV L3 absorption edge in Cu and of the 2.838 keV L3-edge in Ru are presented.

Authors:
 [1]
  1. Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)
Publication Date:
Research Org.:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Org.:
USDOE Office of Science (SC), Office of Basic Energy Sciences (BES)
OSTI Identifier:
1756934
Grant/Contract Number:  
AC02-06CH11357
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Synchrotron Radiation (Online)
Additional Journal Information:
Journal Name: Journal of Synchrotron Radiation (Online); Journal Volume: 27; Journal Issue: 5; Journal ID: ISSN 1600-5775
Publisher:
International Union of Crystallography
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS; Bragg diffraction; X-rays; crystals; diffraction gratings; spectrometers

Citation Formats

Shvyd'ko, Yuri. Diffraction gratings with two-orders-of-magnitude-enhanced dispersion rates for sub-meV resolution soft X-ray spectroscopy. United States: N. p., 2020. Web. doi:10.1107/s1600577520008292.
Shvyd'ko, Yuri. Diffraction gratings with two-orders-of-magnitude-enhanced dispersion rates for sub-meV resolution soft X-ray spectroscopy. United States. https://doi.org/10.1107/s1600577520008292
Shvyd'ko, Yuri. Thu . "Diffraction gratings with two-orders-of-magnitude-enhanced dispersion rates for sub-meV resolution soft X-ray spectroscopy". United States. https://doi.org/10.1107/s1600577520008292. https://www.osti.gov/servlets/purl/1756934.
@article{osti_1756934,
title = {Diffraction gratings with two-orders-of-magnitude-enhanced dispersion rates for sub-meV resolution soft X-ray spectroscopy},
author = {Shvyd'ko, Yuri},
abstractNote = {Diffraction gratings with large angular dispersion rates are central to obtaining high spectral resolution in grating spectrometers operating over a broad spectral range from infrared to soft X-ray domains. The greatest challenge is of course to achieve large dispersion rates in the short-wavelength X-ray domain. Here it is shown that crystals in non-coplanar asymmetric X-ray Bragg diffraction can function as high-reflectance broadband soft X-ray diffraction gratings with dispersion rates that are at least two orders of magnitude larger than those that are possible with state-of-the-art man-made gratings. Additionally, this opens new opportunities to design and implement soft X-ray resonant inelastic scattering (RIXS) spectrometers with spectral resolutions that are up to two orders of magnitude higher than what is currently possible, to further advance a very dynamic field of RIXS spectroscopy, and to make it competitive with inelastic neutron scattering. Examples of large-dispersion-rate crystal diffraction gratings operating near the 930 eV L3 absorption edge in Cu and of the 2.838 keV L3-edge in Ru are presented.},
doi = {10.1107/s1600577520008292},
journal = {Journal of Synchrotron Radiation (Online)},
number = 5,
volume = 27,
place = {United States},
year = {Thu Jul 30 00:00:00 EDT 2020},
month = {Thu Jul 30 00:00:00 EDT 2020}
}

Works referenced in this record:

μm-resolved high resolution X-ray diffraction imaging for semiconductor quality control
journal, April 2000

  • Lübbert, D.; Baumbach, T.; Härtwig, J.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 160, Issue 4
  • DOI: 10.1016/S0168-583X(99)00619-9

X-Ray Bragg Diffraction in Asymmetric Backscattering Geometry
journal, December 2006


Spin–orbital separation in the quasi-one-dimensional Mott insulator Sr2CuO3
journal, April 2012

  • Schlappa, J.; Wohlfeld, K.; Zhou, K. J.
  • Nature, Vol. 485, Issue 7396
  • DOI: 10.1038/nature10974

Multilayer-coated blazed grating with variable line spacing and a variable blaze angle
journal, January 2014

  • Voronov, D. L.; Warwick, T.; Padmore, H. A.
  • Optics Letters, Vol. 39, Issue 21
  • DOI: 10.1364/OL.39.006134

Theory of angular-dispersive, imaging hard-x-ray spectrographs
journal, May 2015


Complete polarization analysis of high energy soft x-rays by combining a multilayer phase retarder with crystal analyzer
journal, June 2012

  • Wang, H.; Dhesi, S. S.; Maccherozzi, F.
  • Journal of Applied Physics, Vol. 111, Issue 12
  • DOI: 10.1063/1.4730899

High-contrast sub-millivolt inelastic X-ray scattering for nano- and mesoscale science
journal, June 2014

  • Shvyd’ko, Yuri; Stoupin, Stanislav; Shu, Deming
  • Nature Communications, Vol. 5, Issue 1
  • DOI: 10.1038/ncomms5219

SAXES, a high resolution spectrometer for resonant x-ray emission in the 400–1600eV energy range
journal, November 2006

  • Ghiringhelli, G.; Piazzalunga, A.; Dallera, C.
  • Review of Scientific Instruments, Vol. 77, Issue 11
  • DOI: 10.1063/1.2372731

The beamline ID32 at the ESRF for soft X-ray high energy resolution resonant inelastic X-ray scattering and polarisation dependent X-ray absorption spectroscopy
journal, September 2018

  • Brookes, N. B.; Yakhou-Harris, F.; Kummer, K.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 903
  • DOI: 10.1016/j.nima.2018.07.001

Intense paramagnon excitations in a large family of high-temperature superconductors
journal, July 2011

  • Le Tacon, M.; Ghiringhelli, G.; Chaloupka, J.
  • Nature Physics, Vol. 7, Issue 9
  • DOI: 10.1038/nphys2041

Experimental resolution in soft X-ray monochromators
journal, February 1989

  • Kortboyer, S. W.; Goedkoop, J. B.; De Groot, F. M. F.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 275, Issue 2
  • DOI: 10.1016/0168-9002(89)90721-3

A double-crystal monochromator for EXAFS measurement at NSRL
journal, June 1998

  • Xu, Chaoyin; Zhao, Weichang; Pan, Guoqiang
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 410, Issue 2
  • DOI: 10.1016/S0168-9002(98)00202-2

Persistence of magnetic excitations in La2−xSrxCuO4 from the undoped insulator to the heavily overdoped non-superconducting metal
journal, August 2013

  • Dean, M. P. M.; Dellea, G.; Springell, R. S.
  • Nature Materials, Vol. 12, Issue 11
  • DOI: 10.1038/nmat3723

High-resolution soft X-ray beamline ADRESS at the Swiss Light Source for resonant inelastic X-ray scattering and angle-resolved photoelectron spectroscopies
journal, July 2010

  • Strocov, V. N.; Schmitt, T.; Flechsig, U.
  • Journal of Synchrotron Radiation, Vol. 17, Issue 5
  • DOI: 10.1107/S0909049510019862

Modular soft x-ray spectrometer for applications in energy sciences and quantum materials
journal, January 2017

  • Chuang, Yi-De; Shao, Yu-Cheng; Cruz, Alejandro
  • Review of Scientific Instruments, Vol. 88, Issue 1
  • DOI: 10.1063/1.4974356

X-ray diffraction under specular reflection conditions. Ideal crystals
journal, March 1983

  • Afanas'ev, A. M.; Melkonyan, M. K.
  • Acta Crystallographica Section A Foundations of Crystallography, Vol. 39, Issue 2
  • DOI: 10.1107/S0108767383000471

Optical Systems for Soft X Rays
book, January 1986


Magnetic Excitations and Phase Separation in the Underdoped La 2 x Sr x CuO 4 Superconductor Measured by Resonant Inelastic X-Ray Scattering
journal, February 2010


Towards 10 meV resolution: The design of an ultrahigh resolution soft X-ray RIXS spectrometer
journal, November 2016

  • Dvorak, Joseph; Jarrige, Ignace; Bisogni, Valentina
  • Review of Scientific Instruments, Vol. 87, Issue 11
  • DOI: 10.1063/1.4964847

Bragg-Laue diffraction in inclined geometry
journal, November 1984

  • Aleksandrov, P. A.; Afanasiev, A. M.; Stepanov, S. A.
  • Physica Status Solidi (a), Vol. 86, Issue 1
  • DOI: 10.1002/pssa.2210860114

Dispersive charge density wave excitations in Bi2Sr2CaCu2O8+δ
journal, June 2017

  • Chaix, L.; Ghiringhelli, G.; Peng, Y. Y.
  • Nature Physics, Vol. 13, Issue 10
  • DOI: 10.1038/nphys4157

High-order multilayer coated blazed gratings for high resolution soft x-ray spectroscopy
journal, January 2015

  • Voronov, Dmitriy L.; Goray, Leonid I.; Warwick, Tony
  • Optics Express, Vol. 23, Issue 4
  • DOI: 10.1364/OE.23.004771

Hard-X-Ray Spectroscopy with a Spectrographic Approach
journal, August 2019


The Crystal Monochromator at BESSY
conference, December 1987

  • Feldhaus, J.; Schafers, F.; Peatman, W.
  • Soft X-Rays Optics and Technology, SPIE Proceedings
  • DOI: 10.1117/12.964916