Strong-field-induced bond rearrangement in triatomic molecules
Abstract
A comparative study of bond rearrangement is reported for the double ionization of three triatomic molecules: carbon dioxide, carbonyl sulfide, and water (D2O). Specifically, we study the formation of the molecular cation AC+ from the edge atoms of a triatomic molecular dication ABC2+ following double ionization by intense, short (23 fs, 790 nm) laser pulses. The comparison is made using the double ionization branching ratio of each molecule, thereby minimizing differences due to differing ionization rates. The rearrangement branching ratio is highest for water, which has a bent initial geometry, while CO2 and OCS are linear molecules. The angular distribution of O2+ fragments arising from CO2 is essentially isotropic, while SO+ from OCS and $$D$$ $$^{+}_{2}$$ from D2O are aligned with the laser polarization. In the CO2 and D2O cases, the angular distributions of the bond rearrangement channels are different from the angular distributions of the dominant dissociative double ionization channels CO+ + O+ and OD+ + D+. Only the angular distribution of SO+ from OCS is both aligned with the laser polarization and similar to the angular distribution of the largest dissociative channel, CO+ + S+. As a result, the mixed behavior observed from the angular distributions of the different molecules stands in contrast to the relative consistency of the magnitude of the bond rearrangement branching ratio.
- Authors:
-
- Augustana Univ., Sioux Falls, SD (United States)
- Kansas State Univ., Manhattan, KS (United States)
- Kansas State Univ., Manhattan, KS (United States); Univ. of Delhi (India)
- Publication Date:
- Research Org.:
- Kansas State Univ., Manhattan, KS (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division; National Science Foundation (NSF); USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1610700
- Alternate Identifier(s):
- OSTI ID: 1512820
- Grant/Contract Number:
- SC0002378; FG02-86ER13491; FG02-09ER16115; PHYS-175777; PHY-1723002
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Physical Review A
- Additional Journal Information:
- Journal Volume: 99; Journal Issue: 5; Journal ID: ISSN 2469-9926
- Publisher:
- American Physical Society (APS)
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 74 ATOMIC AND MOLECULAR PHYSICS; Optics; Physics; Multiphoton or tunneling ionization & excitation; Strong field excitation; Ultrafast phenomena; Molecules
Citation Formats
Zhao, S., Jochim, Bethany, Feizollah, Peyman, Rajput, Jyoti, Ziaee, F., P., Kanaka Raju, Kaderiya, B., Borne, K., Malakar, Y., Berry, Ben, Harrington, J., Rolles, D., Rudenko, A., Carnes, K. D., Wells, Eric, Ben-Itzhak, I., and Severt, T. Strong-field-induced bond rearrangement in triatomic molecules. United States: N. p., 2019.
Web. doi:10.1103/physreva.99.053412.
Zhao, S., Jochim, Bethany, Feizollah, Peyman, Rajput, Jyoti, Ziaee, F., P., Kanaka Raju, Kaderiya, B., Borne, K., Malakar, Y., Berry, Ben, Harrington, J., Rolles, D., Rudenko, A., Carnes, K. D., Wells, Eric, Ben-Itzhak, I., & Severt, T. Strong-field-induced bond rearrangement in triatomic molecules. United States. https://doi.org/10.1103/physreva.99.053412
Zhao, S., Jochim, Bethany, Feizollah, Peyman, Rajput, Jyoti, Ziaee, F., P., Kanaka Raju, Kaderiya, B., Borne, K., Malakar, Y., Berry, Ben, Harrington, J., Rolles, D., Rudenko, A., Carnes, K. D., Wells, Eric, Ben-Itzhak, I., and Severt, T. Wed .
"Strong-field-induced bond rearrangement in triatomic molecules". United States. https://doi.org/10.1103/physreva.99.053412. https://www.osti.gov/servlets/purl/1610700.
@article{osti_1610700,
title = {Strong-field-induced bond rearrangement in triatomic molecules},
author = {Zhao, S. and Jochim, Bethany and Feizollah, Peyman and Rajput, Jyoti and Ziaee, F. and P., Kanaka Raju and Kaderiya, B. and Borne, K. and Malakar, Y. and Berry, Ben and Harrington, J. and Rolles, D. and Rudenko, A. and Carnes, K. D. and Wells, Eric and Ben-Itzhak, I. and Severt, T.},
abstractNote = {A comparative study of bond rearrangement is reported for the double ionization of three triatomic molecules: carbon dioxide, carbonyl sulfide, and water (D2O). Specifically, we study the formation of the molecular cation AC+ from the edge atoms of a triatomic molecular dication ABC2+ following double ionization by intense, short (23 fs, 790 nm) laser pulses. The comparison is made using the double ionization branching ratio of each molecule, thereby minimizing differences due to differing ionization rates. The rearrangement branching ratio is highest for water, which has a bent initial geometry, while CO2 and OCS are linear molecules. The angular distribution of O2+ fragments arising from CO2 is essentially isotropic, while SO+ from OCS and $D$ $^{+}_{2}$ from D2O are aligned with the laser polarization. In the CO2 and D2O cases, the angular distributions of the bond rearrangement channels are different from the angular distributions of the dominant dissociative double ionization channels CO+ + O+ and OD+ + D+. Only the angular distribution of SO+ from OCS is both aligned with the laser polarization and similar to the angular distribution of the largest dissociative channel, CO+ + S+. As a result, the mixed behavior observed from the angular distributions of the different molecules stands in contrast to the relative consistency of the magnitude of the bond rearrangement branching ratio.},
doi = {10.1103/physreva.99.053412},
journal = {Physical Review A},
number = 5,
volume = 99,
place = {United States},
year = {Wed May 15 00:00:00 EDT 2019},
month = {Wed May 15 00:00:00 EDT 2019}
}
Web of Science
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Works referencing / citing this record:
Strong-field control of H3+ production from methanol dications: Selecting between local and extended formation mechanisms
journal, February 2020
- Iwamoto, Naoki; Schwartz, Charles J.; Jochim, Bethany
- The Journal of Chemical Physics, Vol. 152, Issue 5