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Title: Crystal-momentum-resolved contributions to high-order harmonic generation in solids

Abstract

We analytically and numerically investigate the emission of high-order harmonic radiation from model solids by intense few-cycle midinfrared laser pulses. In single-active-electron approximation, we expand the active electron's wave function in a basis of adiabatic Houston states and describe the solid's electronic band structure in terms of an adjustable Kronig-Penney model potential. For high-order harmonic generation (HHG) from MgO crystals, we examine spectra from two-band and converged multiband numerical calculations. We discuss the characteristics of intra- and interband contributions to the HHG spectrum for computations including initial crystal momenta either from the Γ point at the center of the first Brioullin zone (BZ) only or from the entire first BZ. For sufficiently high intensities of the driving laser field, we find relevant contributions to HHG from the entire first BZ. Here, based on numerically calculated spectra, we scrutinize the cutoff harmonic orders as a function of the laser peak intensity and find good qualitative agreement with our analytical saddle-point-approximation predictions and published theoretical data.

Authors:
 [1];  [2]; ORCiD logo [1]
  1. Kansas State Univ., Manhattan, KS (United States)
  2. Inst. of Physics of the ASCR, Prague (Czech Republic)
Publication Date:
Research Org.:
Kansas State Univ., Manhattan, KS (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1610042
Alternate Identifier(s):
OSTI ID: 1560781
Grant/Contract Number:  
FG02-86ER13491; DEFG02-86ER13491
Resource Type:
Accepted Manuscript
Journal Name:
Physical Review A
Additional Journal Information:
Journal Volume: 100; Journal Issue: 3; Journal ID: ISSN 2469-9926
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Optics; Physics; Carrier dynamics; Strong electromagnetic field effects; Ultrafast phenomena

Citation Formats

Navarrete, Francisco, Ciappina, Marcelo F., and Thumm, Uwe. Crystal-momentum-resolved contributions to high-order harmonic generation in solids. United States: N. p., 2019. Web. doi:10.1103/physreva.100.033405.
Navarrete, Francisco, Ciappina, Marcelo F., & Thumm, Uwe. Crystal-momentum-resolved contributions to high-order harmonic generation in solids. United States. https://doi.org/10.1103/physreva.100.033405
Navarrete, Francisco, Ciappina, Marcelo F., and Thumm, Uwe. Mon . "Crystal-momentum-resolved contributions to high-order harmonic generation in solids". United States. https://doi.org/10.1103/physreva.100.033405. https://www.osti.gov/servlets/purl/1610042.
@article{osti_1610042,
title = {Crystal-momentum-resolved contributions to high-order harmonic generation in solids},
author = {Navarrete, Francisco and Ciappina, Marcelo F. and Thumm, Uwe},
abstractNote = {We analytically and numerically investigate the emission of high-order harmonic radiation from model solids by intense few-cycle midinfrared laser pulses. In single-active-electron approximation, we expand the active electron's wave function in a basis of adiabatic Houston states and describe the solid's electronic band structure in terms of an adjustable Kronig-Penney model potential. For high-order harmonic generation (HHG) from MgO crystals, we examine spectra from two-band and converged multiband numerical calculations. We discuss the characteristics of intra- and interband contributions to the HHG spectrum for computations including initial crystal momenta either from the Γ point at the center of the first Brioullin zone (BZ) only or from the entire first BZ. For sufficiently high intensities of the driving laser field, we find relevant contributions to HHG from the entire first BZ. Here, based on numerically calculated spectra, we scrutinize the cutoff harmonic orders as a function of the laser peak intensity and find good qualitative agreement with our analytical saddle-point-approximation predictions and published theoretical data.},
doi = {10.1103/physreva.100.033405},
journal = {Physical Review A},
number = 3,
volume = 100,
place = {United States},
year = {Mon Sep 09 00:00:00 EDT 2019},
month = {Mon Sep 09 00:00:00 EDT 2019}
}

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