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Title: Electrode manufacturing for lithium-ion batteries—Analysis of current and next generation processing

Abstract

As modern energy storage needs become more demanding, the manufacturing of lithium-ion batteries (LIBs) represents a sizable area of growth of the technology. Specifically, wet processing of electrodes has matured such that it is a commonly employed industrial technique. Despite its widespread acceptance, wet processing of electrodes faces a number of problems, including expensive and dangerous solvent recovery, cut-off waste, coating inconsistencies, and microstructural defects due to the solvent drying process. This review considers each of these issues and discusses which electrode slurry properties should be considered when optimizing wet slurry fabrication. Simultaneously, methods to replace traditional wet processing of electrodes are being extensively researched. Some of these novel electrode manufacturing techniques prioritize solvent minimization, while others emphasize boosting energy and power density by thickening the electrode and, subsequently, creating an organized pore structure to permit faster ion diffusion. This review contemplates the advantages and disadvantages of each of these approaches and provides a comprehensive outlook on the future of electrode manufacturing.

Authors:
 [1]; ORCiD logo [1]
  1. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Energy Efficiency and Renewable Energy (EERE)
OSTI Identifier:
1546514
Alternate Identifier(s):
OSTI ID: 1781129
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Energy Storage
Additional Journal Information:
Journal Volume: 25; Journal Issue: C; Journal ID: ISSN 2352-152X
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
25 ENERGY STORAGE; Slurry; Electrode processing; Electrode drying; Electrode architecture; Roll-to-roll manufacturing

Citation Formats

Hawley, William, and Li, Jianlin. Electrode manufacturing for lithium-ion batteries—Analysis of current and next generation processing. United States: N. p., 2019. Web. doi:10.1016/j.est.2019.100862.
Hawley, William, & Li, Jianlin. Electrode manufacturing for lithium-ion batteries—Analysis of current and next generation processing. United States. https://doi.org/10.1016/j.est.2019.100862
Hawley, William, and Li, Jianlin. Wed . "Electrode manufacturing for lithium-ion batteries—Analysis of current and next generation processing". United States. https://doi.org/10.1016/j.est.2019.100862. https://www.osti.gov/servlets/purl/1546514.
@article{osti_1546514,
title = {Electrode manufacturing for lithium-ion batteries—Analysis of current and next generation processing},
author = {Hawley, William and Li, Jianlin},
abstractNote = {As modern energy storage needs become more demanding, the manufacturing of lithium-ion batteries (LIBs) represents a sizable area of growth of the technology. Specifically, wet processing of electrodes has matured such that it is a commonly employed industrial technique. Despite its widespread acceptance, wet processing of electrodes faces a number of problems, including expensive and dangerous solvent recovery, cut-off waste, coating inconsistencies, and microstructural defects due to the solvent drying process. This review considers each of these issues and discusses which electrode slurry properties should be considered when optimizing wet slurry fabrication. Simultaneously, methods to replace traditional wet processing of electrodes are being extensively researched. Some of these novel electrode manufacturing techniques prioritize solvent minimization, while others emphasize boosting energy and power density by thickening the electrode and, subsequently, creating an organized pore structure to permit faster ion diffusion. This review contemplates the advantages and disadvantages of each of these approaches and provides a comprehensive outlook on the future of electrode manufacturing.},
doi = {10.1016/j.est.2019.100862},
journal = {Journal of Energy Storage},
number = C,
volume = 25,
place = {United States},
year = {Wed Jul 31 00:00:00 EDT 2019},
month = {Wed Jul 31 00:00:00 EDT 2019}
}

Journal Article:

Citation Metrics:
Cited by: 109 works
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Figures / Tables:

Figure 1 Figure 1: Flowchart illustrating the electrode fabrication process.

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Works referencing / citing this record:

Hydrogel Leclanché Cell: Construction and Characterization
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Hydrogel Leclanche Cell: Construction and Characterization
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