Disconnecting structure and dynamics in glassy thin films
Abstract
Nanometrically thin glassy films depart strikingly from the behavior of their bulk counterparts. We investigate whether the dynamical differences between a bulk and thin film polymeric glass former can be understood by differences in local microscopic structure. Machine learning methods have shown that local structure can serve as the foundation for successful, predictive models of particle rearrangement dynamics in bulk systems. By contrast, in thin glassy films, we find that particles at the center of the film and those near the surface are structurally indistinguishable despite exhibiting very different dynamics. Next, we show that structure-independent processes, already present in bulk systems and demonstrably different from simple facilitated dynamics, are crucial for understanding glassy dynamics in thin films. Our analysis suggests a picture of glassy dynamics in which two dynamical processes coexist, with relative strengths that depend on the distance from an interface. Here, one of these processes depends on local structure and is unchanged throughout most of the film, while the other is purely Arrhenius, does not depend on local structure, and is strongly enhanced near the free surface of a film.
- Authors:
-
- Syracuse Univ., Syracuse, NY (United States)
- Google, Mountain View, CA (United States)
- Stanford Univ., Stanford, CA (United States)
- Univ. of Pennsylvania, Philadelphia, PA (United States)
- Publication Date:
- Research Org.:
- Univ. of Pennsylvania, Philadelphia, PA (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1540262
- Alternate Identifier(s):
- OSTI ID: 1856741
- Grant/Contract Number:
- FG02-05ER46199
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Proceedings of the National Academy of Sciences of the United States of America
- Additional Journal Information:
- Journal Volume: 114; Journal Issue: 40; Journal ID: ISSN 0027-8424
- Publisher:
- National Academy of Sciences
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE; 75 CONDENSED MATTER PHYSICS, SUPERCONDUCTIVITY AND SUPERFLUIDITY; Science & Technology; Other Topics; machine learning; glass; thin film; Glass transition, glasses, thin films
Citation Formats
Sussman, Daniel M., Schoenholz, Samuel S., Cubuk, Ekin D., and Liu, Andrea J. Disconnecting structure and dynamics in glassy thin films. United States: N. p., 2017.
Web. doi:10.1073/pnas.1703927114.
Sussman, Daniel M., Schoenholz, Samuel S., Cubuk, Ekin D., & Liu, Andrea J. Disconnecting structure and dynamics in glassy thin films. United States. https://doi.org/10.1073/pnas.1703927114
Sussman, Daniel M., Schoenholz, Samuel S., Cubuk, Ekin D., and Liu, Andrea J. Tue .
"Disconnecting structure and dynamics in glassy thin films". United States. https://doi.org/10.1073/pnas.1703927114. https://www.osti.gov/servlets/purl/1540262.
@article{osti_1540262,
title = {Disconnecting structure and dynamics in glassy thin films},
author = {Sussman, Daniel M. and Schoenholz, Samuel S. and Cubuk, Ekin D. and Liu, Andrea J.},
abstractNote = {Nanometrically thin glassy films depart strikingly from the behavior of their bulk counterparts. We investigate whether the dynamical differences between a bulk and thin film polymeric glass former can be understood by differences in local microscopic structure. Machine learning methods have shown that local structure can serve as the foundation for successful, predictive models of particle rearrangement dynamics in bulk systems. By contrast, in thin glassy films, we find that particles at the center of the film and those near the surface are structurally indistinguishable despite exhibiting very different dynamics. Next, we show that structure-independent processes, already present in bulk systems and demonstrably different from simple facilitated dynamics, are crucial for understanding glassy dynamics in thin films. Our analysis suggests a picture of glassy dynamics in which two dynamical processes coexist, with relative strengths that depend on the distance from an interface. Here, one of these processes depends on local structure and is unchanged throughout most of the film, while the other is purely Arrhenius, does not depend on local structure, and is strongly enhanced near the free surface of a film.},
doi = {10.1073/pnas.1703927114},
journal = {Proceedings of the National Academy of Sciences of the United States of America},
number = 40,
volume = 114,
place = {United States},
year = {Tue Sep 19 00:00:00 EDT 2017},
month = {Tue Sep 19 00:00:00 EDT 2017}
}
Web of Science
Works referenced in this record:
Cooperative motion and growing length scales in supercooled confined liquids
journal, September 2002
- Scheidler, P.; Kob, W.; Binder, K.
- Europhysics Letters (EPL), Vol. 59, Issue 5
Cooperative Strings and Glassy Interfaces
text, January 2015
- Salez, Thomas; Salez, Justin; Dalnoki-Veress, Kari
- arXiv
Cooperative strings and glassy interfaces
journal, June 2015
- Salez, Thomas; Salez, Justin; Dalnoki-Veress, Kari
- Proceedings of the National Academy of Sciences, Vol. 112, Issue 27
Structure and dynamics in glass-formers: predictability at large length scales
text, January 2007
- Berthier, Ludovic; Jack, Robert L.
- arXiv
Crossovers in the dynamics of supercooled liquids probed by an amorphous wall
journal, May 2014
- Hocky, Glen M.; Berthier, Ludovic; Kob, Walter
- Physical Review E, Vol. 89, Issue 5
A Direct Quantitative Measure of Surface Mobility in a Glassy Polymer
journal, February 2014
- Chai, Y.; Salez, T.; McGraw, J. D.
- Science, Vol. 343, Issue 6174
Lattice model of mobility at interfaces: free surfaces, substrates, and bilayers
journal, January 2013
- Tito, Nicholas B.; Lipson, Jane E. G.; Milner, Scott T.
- Soft Matter, Vol. 9, Issue 39
Measuring the Surface Dynamics of Glassy Polymers
journal, February 2008
- Fakhraai, Z.; Forrest, J. A.
- Science, Vol. 319, Issue 5863
Identifying Structural Flow Defects in Disordered Solids Using Machine-Learning Methods
journal, March 2015
- Cubuk, E. D.; Schoenholz, S. S.; Rieser, J. M.
- Physical Review Letters, Vol. 114, Issue 10
Long-range correlated dynamics in ultra-thin molecular glass films
journal, September 2016
- Zhang, Yue; Glor, Ethan C.; Li, Mu
- The Journal of Chemical Physics, Vol. 145, Issue 11
Is the molecular surface of polystyrene really glassy?
journal, September 1992
- Meyers, Gregory F.; DeKoven, Benjamin M.; Seitz, Jerry T.
- Langmuir, Vol. 8, Issue 9
Vibrational Modes Identify Soft Spots in a Sheared Disordered Packing
journal, August 2011
- Manning, M. L.; Liu, A. J.
- Physical Review Letters, Vol. 107, Issue 10
Direct Measurement of Molecular Motion in Freestanding Polystyrene Thin Films
journal, June 2011
- Paeng, Keewook; Swallen, Stephen F.; Ediger, M. D.
- Journal of the American Chemical Society, Vol. 133, Issue 22
Decoupling of surface diffusion and relaxation dynamics of molecular glasses
journal, April 2017
- Zhang, Yue; Fakhraai, Zahra
- Proceedings of the National Academy of Sciences, Vol. 114, Issue 19
Discrete mobility on the surface of glasses
journal, April 2017
- Chowdhury, Mithun; Priestley, Rodney D.
- Proceedings of the National Academy of Sciences, Vol. 114, Issue 19
Ensemble fluctuations matter for variances of macroscopic variables
journal, February 2021
- George, G.; Klochko, L.; Semenov, A. N.
- The European Physical Journal E, Vol. 44, Issue 2
Cooperative motion and growing length scales in supercooled confined liquids
text, January 2002
- Scheidler, Peter; Kob, Walter; Binder, Kurt
- arXiv
Dynamics near Free Surfaces and the Glass Transition in Thin Polymer Films: A View to the Future
journal, November 2013
- Ediger, M. D.; Forrest, J. A.
- Macromolecules, Vol. 47, Issue 2
Spatial distribution of entanglements in thin free-standing films
journal, July 2016
- Sussman, Daniel M.
- Physical Review E, Vol. 94, Issue 1
Interfacial Dynamic Length Scales in the Glass Transition of a Model Freestanding Polymer Film and Their Connection to Cooperative Motion
journal, December 2013
- Lang, Ryan J.; Simmons, David S.
- Macromolecules, Vol. 46, Issue 24
Facilitation of interfacial dynamics in entangled polymer films
journal, November 2014
- Glor, Ethan C.; Fakhraai, Zahra
- The Journal of Chemical Physics, Vol. 141, Issue 19
Identifying structural flow defects in disordered solids using machine learning methods
text, January 2014
- Cubuk, Ekin D.; Schoenholz, Samuel S.; Rieser, Jennifer M.
- arXiv
Physical Aging, the Local Dynamics of Glass-Forming Polymers under Nanoscale Confinement
journal, July 2014
- Shavit, Amit; Riggleman, Robert A.
- The Journal of Physical Chemistry B, Vol. 118, Issue 30
Structural Properties of Defects in Glassy Liquids
journal, April 2016
- Cubuk, Ekin D.; Schoenholz, Samuel S.; Kaxiras, Efthimios
- The Journal of Physical Chemistry B, Vol. 120, Issue 26
Physical Aging in Ultrathin Polystyrene Films: Evidence of a Gradient in Dynamics at the Free Surface and Its Connection to the Glass Transition Temperature Reductions
journal, October 2010
- Pye, Justin E.; Rohald, Kate A.; Baker, Elizabeth A.
- Macromolecules, Vol. 43, Issue 19
Macroscopic Facilitation of Glassy Relaxation Kinetics: Ultra Stable Glass Films with Front-Like Thermal Response
text, January 2010
- Léonard, Sébastien; Harrowell, Peter
- arXiv
A unifying framework to quantify the effects of substrate interactions, stiffness, and roughness on the dynamics of thin supported polymer films
journal, June 2015
- Hanakata, Paul Z.; Pazmiño Betancourt, Beatriz A.; Douglas, Jack F.
- The Journal of Chemical Physics, Vol. 142, Issue 23
Building Blocks of Dynamical Heterogeneities in Dense Granular Media
journal, February 2009
- Candelier, R.; Dauchot, O.; Biroli, G.
- Physical Review Letters, Vol. 102, Issue 8
Non-monotonic temperature evolution of dynamic correlations in glass-forming liquids
journal, October 2011
- Kob, Walter; Roldán-Vargas, Sándalo; Berthier, Ludovic
- Nature Physics, Vol. 8, Issue 2
Glass Transition Dynamics and Surface Layer Mobility in Unentangled Polystyrene Films
journal, June 2010
- Yang, Z.; Fujii, Y.; Lee, F. K.
- Science, Vol. 328, Issue 5986
Dynamics of entangled linear polymer melts: A molecular‐dynamics simulation
journal, April 1990
- Kremer, Kurt; Grest, Gary S.
- The Journal of Chemical Physics, Vol. 92, Issue 8
Interfacial mobility scale determines the scale of collective motion and relaxation rate in polymer films
journal, June 2014
- Hanakata, Paul Z.; Douglas, Jack F.; Starr, Francis W.
- Nature Communications, Vol. 5, Issue 1
General purpose molecular dynamics simulations fully implemented on graphics processing units
journal, May 2008
- Anderson, Joshua A.; Lorenz, Chris D.; Travesset, A.
- Journal of Computational Physics, Vol. 227, Issue 10
Crossovers in the dynamics of supercooled liquids probed by an amorphous wall
text, January 2014
- Hocky, Glen M.; Berthier, Ludovic; Kob, Walter
- arXiv
Equilibration of long chain polymer melts in computer simulations
journal, December 2003
- Auhl, Rolf; Everaers, Ralf; Grest, Gary S.
- The Journal of Chemical Physics, Vol. 119, Issue 24
Influence of Backbone Rigidity on Nanoscale Confinement Effects in Model Glass-Forming Polymers
journal, June 2013
- Shavit, Amit; Riggleman, Robert A.
- Macromolecules, Vol. 46, Issue 12
A direct quantitative measure of surface mobility in a glassy polymer
text, January 2014
- Chai, Yu; Salez, Thomas; McGraw, Joshua D.
- arXiv
Dynamics on the Way to Forming Glass: Bubbles in Space-Time
journal, March 2010
- Chandler, David; Garrahan, Juan P.
- Annual Review of Physical Chemistry, Vol. 61, Issue 1
Theory of activated glassy relaxation, mobility gradients, surface diffusion, and vitrification in free standing thin films
journal, December 2015
- Mirigian, Stephen; Schweizer, Kenneth S.
- The Journal of Chemical Physics, Vol. 143, Issue 24
Measurement of growing dynamical length scales and prediction of the jamming transition in a granular material
journal, March 2007
- Keys, Aaron S.; Abate, Adam R.; Glotzer, Sharon C.
- Nature Physics, Vol. 3, Issue 4
Macroscopic facilitation of glassy relaxation kinetics: Ultrastable glass films with frontlike thermal response
journal, December 2010
- Léonard, Sébastien; Harrowell, Peter
- The Journal of Chemical Physics, Vol. 133, Issue 24
Structure and dynamics of glass formers: Predictability at large length scales
journal, October 2007
- Berthier, Ludovic; Jack, Robert L.
- Physical Review E, Vol. 76, Issue 4
Direct observation of a local structural mechanism for dynamic arrest
journal, June 2008
- Patrick Royall, C.; Williams, Stephen R.; Ohtsuka, Takehiro
- Nature Materials, Vol. 7, Issue 7
On the surface of glasses
journal, December 2008
- Stevenson, Jacob D.; Wolynes, Peter G.
- The Journal of Chemical Physics, Vol. 129, Issue 23
The building blocks of dynamical heterogeneities in dense granular media
text, January 2008
- Candelier, R.; Dauchot, O.; Biroli, G.
- arXiv
Irreversible reorganization in a supercooled liquid originates from localized soft modes
journal, July 2008
- Widmer-Cooper, Asaph; Perry, Heidi; Harrowell, Peter
- Nature Physics, Vol. 4, Issue 9
A structural approach to relaxation in glassy liquids
journal, February 2016
- Schoenholz, S. S.; Cubuk, E. D.; Sussman, D. M.
- Nature Physics, Vol. 12, Issue 5
Relationship between local structure and relaxation in out-of-equilibrium glassy systems
journal, December 2016
- Schoenholz, Samuel S.; Cubuk, Ekin D.; Kaxiras, Efthimios
- Proceedings of the National Academy of Sciences, Vol. 114, Issue 2
Works referencing / citing this record:
Machine learning determination of atomic dynamics at grain boundaries
journal, October 2018
- Sharp, Tristan A.; Thomas, Spencer L.; Cubuk, Ekin D.
- Proceedings of the National Academy of Sciences, Vol. 115, Issue 43
Theory of the spatial transfer of interface-nucleated changes of dynamical constraints and its consequences in glass-forming films
journal, January 2019
- Phan, Anh D.; Schweizer, Kenneth S.
- The Journal of Chemical Physics, Vol. 150, Issue 4
Attractive versus truncated repulsive supercooled liquids: The dynamics is encoded in the pair correlation function
journal, January 2020
- Landes, François P.; Biroli, Giulio; Dauchot, Olivier
- Physical Review E, Vol. 101, Issue 1
Machine Learning in a data-limited regime: Augmenting experiments with synthetic data uncovers order in crumpled sheets
text, January 2018
- Hoffmann, Jordan; Bar-Sinai, Yohai; Lee, Lisa
- arXiv
Theory of the Spatial Transfer of Interface-Nucleated Changes of Dynamical Constraints and Its Consequences in Glass-Forming Films
text, January 2019
- Phan, Anh D.; Schweizer, Kenneth S.
- arXiv
Effect of substrate interactions on the glass transition and length-scale of correlated dynamics in ultra-thin molecular glass films
journal, November 2018
- Zhang, Yue; Woods, Connor N.; Alvarez, Mauricio
- The Journal of Chemical Physics, Vol. 149, Issue 18
Comparison of single particle dynamics at the center and on the surface of equilibrium glassy films
journal, August 2018
- Kuon, Nicholas; Flenner, Elijah; Szamel, Grzegorz
- The Journal of Chemical Physics, Vol. 149, Issue 7
Progress towards a phenomenological picture and theoretical understanding of glassy dynamics and vitrification near interfaces and under nanoconfinement
journal, December 2019
- Schweizer, Kenneth S.; Simmons, David S.
- The Journal of Chemical Physics, Vol. 151, Issue 24
Machine learning characterization of structural defects in amorphous packings of dimers and ellipses
journal, February 2019
- Harrington, Matt; Liu, Andrea J.; Durian, Douglas J.
- Physical Review E, Vol. 99, Issue 2
Machine learning determination of atomic dynamics at grain boundaries
text, January 2018
- Sharp, Tristan A.; Thomas, Spencer L.; Cubuk, Ekin D.
- arXiv
Deep Learning for Automated Classification and Characterization of Amorphous Materials
preprint, January 2019
- Swanson, Kirk; Trivedi, Shubhendu; Lequieu, Joshua
- arXiv
Attractive versus truncated repulsive supercooled liquids: The dynamics is encoded in the pair correlation function
text, January 2019
- Landes, François P.; Biroli, Giulio; Dauchot, Olivier
- arXiv
Machine learning in a data-limited regime: Augmenting experiments with synthetic data uncovers order in crumpled sheets
journal, April 2019
- Hoffmann, Jordan; Bar-Sinai, Yohai; Lee, Lisa M.
- Science Advances, Vol. 5, Issue 4
Identifying structural signatures of shear banding in model polymer nanopillars
journal, January 2019
- Ivancic, Robert J. S.; Riggleman, Robert A.
- Soft Matter, Vol. 15, Issue 22
Machine Learning Characterization of Structural Defects in Amorphous Packings of Dimers and Ellipses
text, January 2018
- Harrington, Matt; Liu, Andrea J.; Durian, Douglas J.
- arXiv
Heterogeneous Activation, Local Structure, and Softness in Supercooled Colloidal Liquids
journal, January 2019
- Ma, Xiaoguang; Davidson, Zoey S.; Still, Tim
- Physical Review Letters, Vol. 122, Issue 2
Structure-property relationships from universal signatures of plasticity in disordered solids
journal, November 2017
- Cubuk, E. D.; Ivancic, R. J. S.; Schoenholz, S. S.
- Science, Vol. 358, Issue 6366
Unveiling the predictive power of static structure in glassy systems
journal, April 2020
- Bapst, V.; Keck, T.; Grabska-Barwińska, A.
- Nature Physics, Vol. 16, Issue 4
Correlating fragility and heterogeneous dynamics in polystyrene through single molecule studies
journal, August 2019
- Manz, Alyssa S.; Aly, Mariam; Kaufman, Laura J.
- The Journal of Chemical Physics, Vol. 151, Issue 8
Deep learning for automated classification and characterization of amorphous materials
journal, January 2020
- Swanson, Kirk; Trivedi, Shubhendu; Lequieu, Joshua
- Soft Matter, Vol. 16, Issue 2
Uncovering the effects of interface-induced ordering of liquid on crystal growth using machine learning
journal, June 2020
- Freitas, Rodrigo; Reed, Evan J.
- Nature Communications, Vol. 11, Issue 1
Mutual information, neural networks and the renormalization group
journal, March 2018
- Koch-Janusz, Maciej; Ringel, Zohar
- Nature Physics, Vol. 14, Issue 6
A characteristic energy scale in glasses
journal, June 2018
- Lerner, Edan; Bouchbinder, Eran
- The Journal of Chemical Physics, Vol. 148, Issue 21
Spin-qubit noise spectroscopy from randomized benchmarking by supervised learning
journal, April 2019
- Zhang, Chengxian; Wang, Xin
- Physical Review A, Vol. 99, Issue 4
Collective diffusion within the superionic regime of
Bi 2 O 3
journal, March 2020
- Mohn, Chris E.; Krynski, Marcin
- Physical Review B, Vol. 101, Issue 10
Transition from stress-driven to thermally activated stress relaxation in metallic glasses
journal, September 2016
- Qiao, J. C.; Wang, Yun-Jiang; Zhao, L. Z.
- Physical Review B, Vol. 94, Issue 10
Learning thermodynamics with Boltzmann machines
journal, October 2016
- Torlai, Giacomo; Melko, Roger G.
- Physical Review B, Vol. 94, Issue 16
Few-shot machine learning in the three-dimensional Ising model
journal, March 2019
- Zhang, Rui; Wei, Bin; Zhang, Dong
- Physical Review B, Vol. 99, Issue 9
Attractive versus truncated repulsive supercooled liquids: The dynamics is encoded in the pair correlation function
journal, January 2020
- Landes, François P.; Biroli, Giulio; Dauchot, Olivier
- Physical Review E, Vol. 101, Issue 1
Nonequilibrium thermodynamics of restricted Boltzmann machines
journal, August 2017
- Salazar, Domingos S. P.
- Physical Review E, Vol. 96, Issue 2
Local yield stress statistics in model amorphous solids
journal, March 2018
- Barbot, Armand; Lerbinger, Matthias; Hernandez-Garcia, Anier
- Physical Review E, Vol. 97, Issue 3
Matrix product operators for sequence-to-sequence learning
journal, October 2018
- Guo, Chu; Jie, Zhanming; Lu, Wei
- Physical Review E, Vol. 98, Issue 4
Machine learning characterization of structural defects in amorphous packings of dimers and ellipses
journal, February 2019
- Harrington, Matt; Liu, Andrea J.; Durian, Douglas J.
- Physical Review E, Vol. 99, Issue 2
Anisotropic structural predictor in glassy materials
journal, June 2019
- Schwartzman-Nowik, Zohar; Lerner, Edan; Bouchbinder, Eran
- Physical Review E, Vol. 99, Issue 6
Accelerated Search and Design of Stretchable Graphene Kirigami Using Machine Learning
journal, December 2018
- Hanakata, Paul Z.; Cubuk, Ekin D.; Campbell, David K.
- Physical Review Letters, Vol. 121, Issue 25
Averaging Local Structure to Predict the Dynamic Propensity in Supercooled Liquids
journal, August 2021
- Boattini, Emanuele; Smallenburg, Frank; Filion, Laura
- Physical Review Letters, Vol. 127, Issue 8
Atomic nonaffinity as a predictor of plasticity in amorphous solids
journal, February 2021
- Xu, Bin; Falk, Michael L.; Patinet, Sylvain
- Physical Review Materials, Vol. 5, Issue 2
Relationship between two-level systems and quasilocalized normal modes in glasses
journal, May 2021
- Khomenko, Dmytro; Reichman, David R.; Zamponi, Francesco
- Physical Review Materials, Vol. 5, Issue 5
Nuclear liquid-gas phase transition with machine learning
journal, November 2020
- Wang, Rui; Ma, Yu-Gang; Wada, R.
- Physical Review Research, Vol. 2, Issue 4
Revealing Hidden Structural Order Controlling Both Fast and Slow Glassy Dynamics in Supercooled Liquids
journal, March 2018
- Tong, Hua; Tanaka, Hajime
- Physical Review X, Vol. 8, Issue 1
Machine learning in a data-limited regime: Augmenting experiments with synthetic data uncovers order in crumpled sheets
journal, April 2019
- Hoffmann, Jordan; Bar-Sinai, Yohai; Lee, Lisa M.
- Science Advances, Vol. 5, Issue 4
Assessing the structural heterogeneity of supercooled liquids through community inference.
text, January 2020
- Paret, Joris; Jack, Robert; Coslovich, Daniele
- Apollo - University of Cambridge Repository
The Relationship Between Local Structure and Relaxation in Out-of-Equilibrium Glassy Systems
text, January 2016
- Schoenholz, Samuel S.; Cubuk, Ekin D.; Kaxiras, Efthimios
- arXiv
Machine learning quantum phases of matter beyond the fermion sign problem
text, January 2016
- Broecker, Peter; Carrasquilla, Juan; Melko, Roger G.
- arXiv
Machine Learning Phases of Strongly Correlated Fermions
text, January 2016
- Ch'ng, Kelvin; Carrasquilla, Juan; Melko, Roger G.
- arXiv
Machine Learning Topological States
text, January 2016
- Deng, Dong-Ling; Li, Xiaopeng; Sarma, S. Das
- arXiv
Perspectives on opportunities in experimental soft-matter science
text, January 2016
- Nagel, Sidney R.
- arXiv
Quantum Entanglement in Neural Network States
text, January 2017
- Deng, Dong-Ling; Li, Xiaopeng; Sarma, S. Das
- arXiv
Neural-network-designed pulse sequences for robust control of singlet-triplet qubits
text, January 2017
- Yang, Xu-Chen; Yung, Man-Hong; Wang, Xin
- arXiv
Orientational Order in Disordered Colloidal Suspensions
preprint, January 2017
- Yang, Xiunan; Wang, Wei-Hua; Chen, Ke
- arXiv
Combining Machine Learning and Physics to Understand Glassy Systems
text, January 2017
- Schoenholz, Samuel S.
- arXiv
Machine Learning Bell Nonlocality in Quantum Many-body Systems
text, January 2017
- Deng, Dong-Ling
- arXiv
Machine learning determination of atomic dynamics at grain boundaries
text, January 2018
- Sharp, Tristan A.; Thomas, Spencer L.; Cubuk, Ekin D.
- arXiv
Autonomous data-driven design of inorganic materials with AFLOW
preprint, January 2018
- Oses, Corey; Toher, Cormac; Curtarolo, Stefano
- arXiv
Data-driven studies of magnetic two-dimensional materials
preprint, January 2018
- Rhone, Trevor David; Chen, Wei; Desai, Shaan
- arXiv
Migrating Knowledge between Physical Scenarios based on Artificial Neural Networks
preprint, January 2018
- Qu, Yurui; Jing, Li; Shen, Yichen
- arXiv
Bypassing sluggishness: SWAP algorithm and glassiness in high dimensions
text, January 2018
- Berthier, Ludovic; Charbonneau, Patrick; Kundu, Joyjit
- arXiv
The "glass transition'' as a topological defect driven transition in a distribution of crystals and a prediction of a universal viscosity collapse
text, January 2019
- Nussinov, Z.; Weingartner, N. B.; Nogueira, F. S.
- arXiv
Dynamic facilitation theory: A statistical mechanics approach to dynamic arrest
text, January 2019
- Speck, Thomas
- arXiv
On the Structure of Liquids: More order than expected
preprint, January 2019
- Zhang, Zhen; Kob, Walter
- arXiv
Deep Learning for Automated Classification and Characterization of Amorphous Materials
preprint, January 2019
- Swanson, Kirk; Trivedi, Shubhendu; Lequieu, Joshua
- arXiv
Predicting plasticity in disordered solids from structural indicators
text, January 2020
- Richard, D.; Ozawa, M.; Patinet, S.
- arXiv
How to "measure" a structural relaxation time that is too long to be measured?
text, January 2020
- Berthier, Ludovic; Ediger, Mark D.
- arXiv
Glasses and aging: A Statistical Mechanics Perspective
preprint, January 2020
- Arceri, Francesco; Landes, François P.; Berthier, Ludovic
- arXiv
Energy barriers and cooperative motion at the surface of freestanding glassy polystyrene films
text, January 2020
- Fujimoto, Derek; MacFarlane, W. Andrew; Rottler, Joerg
- arXiv
Interplay of rearrangements, strain, and local structure during avalanche propagation
preprint, January 2020
- Zhang, Ge; Ridout, Sean; Liu, Andrea J.
- arXiv
Direct evidence of void induced structural relaxations in colloidal glass formers
text, January 2020
- Yip, Cho-Tung; Isobe, Masaharu; Chan, Chor-Hoi
- arXiv
A Theory of Localized Excitations in Supercooled Liquids
text, January 2021
- Hasyim, Muhammad R.; Mandadapu, Kranthi K.
- arXiv
Multi-component generalized mode-coupling theory: Predicting dynamics from structure in glassy mixtures
text, January 2021
- Ciarella, Simone; Luo, Chengjie; Debets, Vincent E.
- arXiv
Effects of Polydispersity on the Plastic Behaviors of Dense 2D Granular Systems Under Shear
preprint, January 2022
- Jiang, Yonglun; Sussman, Daniel M.; Weeks, Eric R.
- arXiv