Impact of Anthropogenic Emission Injection Height Uncertainty on Global Sulfur Dioxide and Aerosol Distribution
Abstract
The impact of the uncertainty in injection height of anthropogenic emissions is examined using a global aerosol-climate model. We find a large impact of the assumed effective emission height on near-surface concentration and vertical profile of SO2. The global range of SO2 concentration over land (ocean) due to uncertainty in industrial (international shipping) emission injection height is 81% (76%), relative to the average concentration, whereas the relative range of secondary sulfate is 8% (10%) and primary aerosols such as black carbon and primary organic matter is 53% (28%). During 2005–2014, uncertainty in modeled SO2 and aerosols related to injection heights became increasingly important over East Asia and South Asia. This study reveals different impacts of emission injection height uncertainty on modeling of gases, primary aerosols and secondary aerosols and helps with interpretation of discrepancies between model, measurements and satellite retrievals.
- Authors:
-
- Pacific Northwest National Lab. (PNNL), Richland, WA (United States)
- Pacific Northwest National Lab. (PNNL), College Park, MD (United States)
- Publication Date:
- Research Org.:
- Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). National Energy Research Scientific Computing Center (NERSC); Pacific Northwest National Laboratory (PNNL), Richland, WA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1528914
- Alternate Identifier(s):
- OSTI ID: 1510106; OSTI ID: 1543308
- Report Number(s):
- PNNL-SA-137329
Journal ID: ISSN 2169-897X
- Grant/Contract Number:
- AC05‐76RL01830; AC05-76RL01830
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Journal of Geophysical Research: Atmospheres
- Additional Journal Information:
- Journal Volume: 124; Journal Issue: 8; Journal ID: ISSN 2169-897X
- Publisher:
- American Geophysical Union
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 54 ENVIRONMENTAL SCIENCES; aerosol; injection height; emission; model
Citation Formats
Yang, Yang, Smith, Steven J., Wang, Hailong, Lou, Sijia, and Rasch, Philip J. Impact of Anthropogenic Emission Injection Height Uncertainty on Global Sulfur Dioxide and Aerosol Distribution. United States: N. p., 2019.
Web. doi:10.1029/2018JD030001.
Yang, Yang, Smith, Steven J., Wang, Hailong, Lou, Sijia, & Rasch, Philip J. Impact of Anthropogenic Emission Injection Height Uncertainty on Global Sulfur Dioxide and Aerosol Distribution. United States. https://doi.org/10.1029/2018JD030001
Yang, Yang, Smith, Steven J., Wang, Hailong, Lou, Sijia, and Rasch, Philip J. Sat .
"Impact of Anthropogenic Emission Injection Height Uncertainty on Global Sulfur Dioxide and Aerosol Distribution". United States. https://doi.org/10.1029/2018JD030001. https://www.osti.gov/servlets/purl/1528914.
@article{osti_1528914,
title = {Impact of Anthropogenic Emission Injection Height Uncertainty on Global Sulfur Dioxide and Aerosol Distribution},
author = {Yang, Yang and Smith, Steven J. and Wang, Hailong and Lou, Sijia and Rasch, Philip J.},
abstractNote = {The impact of the uncertainty in injection height of anthropogenic emissions is examined using a global aerosol-climate model. We find a large impact of the assumed effective emission height on near-surface concentration and vertical profile of SO2. The global range of SO2 concentration over land (ocean) due to uncertainty in industrial (international shipping) emission injection height is 81% (76%), relative to the average concentration, whereas the relative range of secondary sulfate is 8% (10%) and primary aerosols such as black carbon and primary organic matter is 53% (28%). During 2005–2014, uncertainty in modeled SO2 and aerosols related to injection heights became increasingly important over East Asia and South Asia. This study reveals different impacts of emission injection height uncertainty on modeling of gases, primary aerosols and secondary aerosols and helps with interpretation of discrepancies between model, measurements and satellite retrievals.},
doi = {10.1029/2018JD030001},
journal = {Journal of Geophysical Research: Atmospheres},
number = 8,
volume = 124,
place = {United States},
year = {Sat Apr 13 00:00:00 EDT 2019},
month = {Sat Apr 13 00:00:00 EDT 2019}
}
Web of Science
Works referenced in this record:
Injection heights of springtime biomass-burning plumes over peninsular Southeast Asia and their impacts on long-range pollutant transport
journal, January 2014
- Jian, Y.; Fu, T. -M.
- Atmospheric Chemistry and Physics, Vol. 14, Issue 8
Effective pollutant emission heights for atmospheric transport modelling based on real-world information
journal, February 2009
- Pregger, Thomas; Friedrich, Rainer
- Environmental Pollution, Vol. 157, Issue 2
The Community Earth System Model: A Framework for Collaborative Research
journal, September 2013
- Hurrell, James W.; Holland, M. M.; Gent, P. R.
- Bulletin of the American Meteorological Society, Vol. 94, Issue 9
Analysis of regional budgets of sulfur species modeled for the COSAM exercise: Sulfur species modeled for the COSAM exercise
journal, November 2001
- Roelofs, G. J.; Kasibhatla, P.; Barrie, L.
- Tellus B, Vol. 53, Issue 5
Anthropogenic sulfur dioxide emissions: 1850–2005
journal, January 2011
- Smith, S. J.; van Aardenne, J.; Klimont, Z.
- Atmospheric Chemistry and Physics, Vol. 11, Issue 3
Toward a minimal representation of aerosols in climate models: description and evaluation in the Community Atmosphere Model CAM5
journal, January 2012
- Liu, X.; Easter, R. C.; Ghan, S. J.
- Geoscientific Model Development, Vol. 5, Issue 3
Historical (1750–2014) anthropogenic emissions of reactive gases and aerosols from the Community Emissions Data System (CEDS)
journal, January 2018
- Hoesly, Rachel M.; Smith, Steven J.; Feng, Leyang
- Geoscientific Model Development, Vol. 11, Issue 1
Space-based detection of missing sulfur dioxide sources of global air pollution
journal, May 2016
- McLinden, Chris A.; Fioletov, Vitali; Shephard, Mark W.
- Nature Geoscience, Vol. 9, Issue 7
Radiative forcing of the direct aerosol effect from AeroCom Phase II simulations
journal, January 2013
- Myhre, G.; Samset, B. H.; Schulz, M.
- Atmospheric Chemistry and Physics, Vol. 13, Issue 4
Global mapping of maximum emission heights and resulting vertical profiles of wildfire emissions
journal, January 2013
- Sofiev, M.; Vankevich, R.; Ermakova, T.
- Atmospheric Chemistry and Physics, Vol. 13, Issue 14
Emissions of primary aerosol and precursor gases in the years 2000 and 1750 prescribed data-sets for AeroCom
journal, January 2006
- Dentener, F.; Kinne, S.; Bond, T.
- Atmospheric Chemistry and Physics, Vol. 6, Issue 12
SO 2 over central China: Measurements, numerical simulations and the tropospheric sulfur budget : SULFUR COMPOUNDS OVER CENTRAL CHINA
journal, February 2012
- He, Hao; Li, Can; Loughner, Christopher P.
- Journal of Geophysical Research: Atmospheres, Vol. 117, Issue D16
India Is Overtaking China as the World’s Largest Emitter of Anthropogenic Sulfur Dioxide
journal, November 2017
- Li, Can; McLinden, Chris; Fioletov, Vitali
- Scientific Reports, Vol. 7, Issue 1
The AeroCom evaluation and intercomparison of organic aerosol in global models
journal, January 2014
- Tsigaridis, K.; Daskalakis, N.; Kanakidou, M.
- Atmospheric Chemistry and Physics, Vol. 14, Issue 19
Source attribution of black carbon and its direct radiative forcing in China
journal, January 2017
- Yang, Yang; Wang, Hailong; Smith, Steven J.
- Atmospheric Chemistry and Physics, Vol. 17, Issue 6
The Validity of Several Plume Rise Formulas
journal, November 1969
- Carson, James E.; Moses, Harry
- Journal of the Air Pollution Control Association, Vol. 19, Issue 11
MERRA: NASA’s Modern-Era Retrospective Analysis for Research and Applications
journal, July 2011
- Rienecker, Michele M.; Suarez, Max J.; Gelaro, Ronald
- Journal of Climate, Vol. 24, Issue 14
Global source attribution of sulfate concentration and direct and indirect radiative forcing
journal, January 2017
- Yang, Yang; Wang, Hailong; Smith, Steven J.
- Atmospheric Chemistry and Physics, Vol. 17, Issue 14
Satellite-based global volcanic SO 2 emissions and sulfate direct radiative forcing during 2005-2012 : OMI-BASED VOLCANIC EMISSION AND FORCING
journal, April 2016
- Ge, Cui; Wang, Jun; Carn, Simon
- Journal of Geophysical Research: Atmospheres, Vol. 121, Issue 7
Modeling of biomass smoke injection into the lower stratosphere by a large forest fire (Part II): sensitivity studies
journal, January 2006
- Luderer, G.; Trentmann, J.; Winterrath, T.
- Atmospheric Chemistry and Physics, Vol. 6, Issue 12
The influence of the vertical distribution of emissions on tropospheric chemistry
journal, January 2009
- Pozzer, A.; Jöckel, P.; Van Aardenne, J.
- Atmospheric Chemistry and Physics, Vol. 9, Issue 24
Historic global biomass burning emissions for CMIP6 (BB4CMIP) based on merging satellite observations with proxies and fire models (1750–2015)
journal, January 2017
- van Marle, Margreet J. E.; Kloster, Silvia; Magi, Brian I.
- Geoscientific Model Development, Vol. 10, Issue 9
Sensitivity of remote aerosol distributions to representation of cloud–aerosol interactions in a global climate model
journal, January 2013
- Wang, H.; Easter, R. C.; Rasch, P. J.
- Geoscientific Model Development, Vol. 6, Issue 3
Vertical emission profiles for Europe based on plume rise calculations
journal, October 2011
- Bieser, J.; Aulinger, A.; Matthias, V.
- Environmental Pollution, Vol. 159, Issue 10
Recent intensification of winter haze in China linked to foreign emissions and meteorology
journal, February 2018
- Yang, Yang; Wang, Hailong; Smith, Steven J.
- Scientific Reports, Vol. 8, Issue 1
A chemical transport model study of plume-rise and particle size distribution for the Athabasca oil sands
journal, January 2018
- Akingunola, Ayodeji; Makar, Paul A.; Zhang, Junhua
- Atmospheric Chemistry and Physics, Vol. 18, Issue 12
The aerosol-climate model ECHAM5-HAM
journal, January 2005
- Stier, P.; Feichter, J.; Kinne, S.
- Atmospheric Chemistry and Physics, Vol. 5, Issue 4
Source Apportionments of Aerosols and Their Direct Radiative Forcing and Long-Term Trends Over Continental United States
journal, June 2018
- Yang, Yang; Wang, Hailong; Smith, Steven J.
- Earth's Future, Vol. 6, Issue 6
Sulfate Aerosol in the Arctic: Source Attribution and Radiative Forcing
journal, February 2018
- Yang, Yang; Wang, Hailong; Smith, Steven J.
- Journal of Geophysical Research: Atmospheres, Vol. 123, Issue 3
Implementation of plume rise and its impacts on emissions and air quality modelling
journal, December 2014
- Guevara, Marc; Soret, Albert; Arévalo, Gustavo
- Atmospheric Environment, Vol. 99
Analysis and quantification of the diversities of aerosol life cycles within AeroCom
journal, January 2006
- Textor, C.; Schulz, M.; Guibert, S.
- Atmospheric Chemistry and Physics, Vol. 6, Issue 7
The sensitivity of aerosol in Europe to two different emission inventories and temporal distribution of emissions
journal, January 2006
- de Meij, A.; Krol, M.; Dentener, F.
- Atmospheric Chemistry and Physics, Vol. 6, Issue 12
Impact of the vertical emission profiles on background gas-phase pollution simulated from the EMEP emissions over Europe
journal, January 2013
- Mailler, S.; Khvorostyanov, D.; Menut, L.
- Atmospheric Chemistry and Physics, Vol. 13, Issue 12
A comparison of plume rise algorithms to stack plume measurements in the Athabasca oil sands
journal, January 2018
- Gordon, Mark; Makar, Paul A.; Staebler, Ralf M.
- Atmospheric Chemistry and Physics, Vol. 18, Issue 19
Anthropogenic sulfur dioxide emissions: 1850–2005
journal, January 2010
- Smith, S. J.; van Aardenne, J.; Klimont, Z.
- Atmospheric Chemistry and Physics Discussions, Vol. 10, Issue 6
The AeroCom evaluation and intercomparison of organic aerosol in global models
journal, January 2014
- Tsigaridis, K.; Daskalakis, N.; Kanakidou, M.
- Atmospheric Chemistry and Physics Discussions, Vol. 14, Issue 5
The Paris Climate Agreement and future sea-level rise from Antarctica
journal, May 2021
- DeConto, Robert M.; Pollard, David; Alley, Richard B.
- Nature, Vol. 593, Issue 7857
Analysis of regional budgets of sulfur species modeled for the COSAM exercise
journal, January 2001
- Roelofs, G. J.; Kasibhatla, P.; Barrie, L.
- Tellus B: Chemical and Physical Meteorology, Vol. 53, Issue 5
Sensitivity of remote aerosol distributions to representation of cloud-aerosol interactions in a global climate model
journal, January 2013
- Wang, H.; Easter, R. C.; Rasch, P. J.
- Geoscientific Model Development Discussions, Vol. 6, Issue 1
Historic global biomass burning emissions for CMIP6 (BB4CMIP) based on merging satellite observations with proxies and fire models (1750-2015)
text, January 2017
- Marle, Margreet J. E. Van; Kloster, Silvia; Magi, Brian I.
- Karlsruhe
Historical (1750 - 2014) anthropogenic emissions of reactive gases and aerosols from the Community Emission Data System (CEDS)
preprint, March 2017
- Hoesly, Rachel M.; Smith, Steven J.; Feng, Leyang
- EGU
Works referencing / citing this record:
Exploring 2016–2017 surface ozone pollution over China: source contributions and meteorological influences
journal, January 2019
- Lu, Xiao; Zhang, Lin; Chen, Youfan
- Atmospheric Chemistry and Physics, Vol. 19, Issue 12