Lattice-contraction triggered synchronous electrochromic actuator
Abstract
Materials with synchronous capabilities of color change and actuation have prospects for application in biomimetic dual-stealth camouflage and artificial intelligence. However, color/shape dual-responsive devices involve stimuli that are difficult to control such as gas, light or magnetism, and the devices show poor coordination. Here, a flexible composite film with electrochromic/actuating (238° bending angle) dual-responsive phenomena, excellent reversibility, high synchronization, and fast response speed (< 5 s) utilizes a single active component, W18O49 nanowires. From in situ synchrotron X-ray diffraction, first principles calculations/numerical simulations, and a series of control experiments, the actuating mechanism for macroscopic deformation is elucidated as pseudocapacitance-based reversible lattice contraction/recovery of W18O49 nanowires (i.e. nanostructure change at the atomic level) during lithium ion intercalation/de-intercalation. Furthermore, we demonstrate the W18O49 nanowires in a solid-state ionic polymer-metal composite actuator that operates stably in air with a significant pseudocapacitive actuation.
- Authors:
-
- Donghua Univ., Shanghai (People's Republic of China)
- Univ. of Cambridge, Cambridge (United Kingdom)
- SLAC National Accelerator Lab., Menlo Park, CA (United States)
- Northwestern Univ., Evanston, IL (United States)
- Georgia Inst. of Technology, Atlanta, GA (United States)
- Univ. of Electronic Science and Technology of China, Chengdu (People's Republic of China)
- Publication Date:
- Research Org.:
- SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)
- Sponsoring Org.:
- USDOE
- OSTI Identifier:
- 1490648
- Grant/Contract Number:
- AC02-76SF00515
- Resource Type:
- Accepted Manuscript
- Journal Name:
- Nature Communications
- Additional Journal Information:
- Journal Volume: 9; Journal Issue: 1; Journal ID: ISSN 2041-1723
- Publisher:
- Nature Publishing Group
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 36 MATERIALS SCIENCE
Citation Formats
Li, Kerui, Shao, Yuanlong, Yan, Hongping, Lu, Zhi, Griffith, Kent J., Yan, Jinhui, Wang, Gang, Fan, Hongwei, Lu, Jingyu, Huang, Wei, Bao, Bin, Liu, Xuelong, Hou, Chengyi, Zhang, Qinghong, Li, Yaogang, Yu, Junsheng, and Wang, Hongzhi. Lattice-contraction triggered synchronous electrochromic actuator. United States: N. p., 2018.
Web. doi:10.1038/s41467-018-07241-7.
Li, Kerui, Shao, Yuanlong, Yan, Hongping, Lu, Zhi, Griffith, Kent J., Yan, Jinhui, Wang, Gang, Fan, Hongwei, Lu, Jingyu, Huang, Wei, Bao, Bin, Liu, Xuelong, Hou, Chengyi, Zhang, Qinghong, Li, Yaogang, Yu, Junsheng, & Wang, Hongzhi. Lattice-contraction triggered synchronous electrochromic actuator. United States. https://doi.org/10.1038/s41467-018-07241-7
Li, Kerui, Shao, Yuanlong, Yan, Hongping, Lu, Zhi, Griffith, Kent J., Yan, Jinhui, Wang, Gang, Fan, Hongwei, Lu, Jingyu, Huang, Wei, Bao, Bin, Liu, Xuelong, Hou, Chengyi, Zhang, Qinghong, Li, Yaogang, Yu, Junsheng, and Wang, Hongzhi. Thu .
"Lattice-contraction triggered synchronous electrochromic actuator". United States. https://doi.org/10.1038/s41467-018-07241-7. https://www.osti.gov/servlets/purl/1490648.
@article{osti_1490648,
title = {Lattice-contraction triggered synchronous electrochromic actuator},
author = {Li, Kerui and Shao, Yuanlong and Yan, Hongping and Lu, Zhi and Griffith, Kent J. and Yan, Jinhui and Wang, Gang and Fan, Hongwei and Lu, Jingyu and Huang, Wei and Bao, Bin and Liu, Xuelong and Hou, Chengyi and Zhang, Qinghong and Li, Yaogang and Yu, Junsheng and Wang, Hongzhi},
abstractNote = {Materials with synchronous capabilities of color change and actuation have prospects for application in biomimetic dual-stealth camouflage and artificial intelligence. However, color/shape dual-responsive devices involve stimuli that are difficult to control such as gas, light or magnetism, and the devices show poor coordination. Here, a flexible composite film with electrochromic/actuating (238° bending angle) dual-responsive phenomena, excellent reversibility, high synchronization, and fast response speed (< 5 s) utilizes a single active component, W18O49 nanowires. From in situ synchrotron X-ray diffraction, first principles calculations/numerical simulations, and a series of control experiments, the actuating mechanism for macroscopic deformation is elucidated as pseudocapacitance-based reversible lattice contraction/recovery of W18O49 nanowires (i.e. nanostructure change at the atomic level) during lithium ion intercalation/de-intercalation. Furthermore, we demonstrate the W18O49 nanowires in a solid-state ionic polymer-metal composite actuator that operates stably in air with a significant pseudocapacitive actuation.},
doi = {10.1038/s41467-018-07241-7},
journal = {Nature Communications},
number = 1,
volume = 9,
place = {United States},
year = {Thu Nov 15 00:00:00 EST 2018},
month = {Thu Nov 15 00:00:00 EST 2018}
}
Web of Science
Figures / Tables:
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Ultrathin W 18 O 49 Nanowire Assemblies for Electrochromic Devices
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Reversible Electrochemical Actuation of Metallic Nanohoneycombs Induced by Pseudocapacitive Redox Processes
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Metallic molybdenum disulfide nanosheet-based electrochemical actuators
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Photonic crystals cause active colour change in chameleons
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Graphitic carbon nitride nanosheet electrode-based high-performance ionic actuator
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Erratum: Photogated humidity-driven motility
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A chameleon-inspired stretchable electronic skin with interactive colour changing controlled by tactile sensing
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- Chou, Ho-Hsiu; Nguyen, Amanda; Chortos, Alex
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V2O5 nanofibre sheet actuators
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Colour-tunable spiral photonic actuators
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- Guayasamin, Juan M.; Krynak, Tim; Krynak, Katherine
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Origami-inspired active graphene-based paper for programmable instant self-folding walking devices
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- Mu, Jiuke; Hou, Chengyi; Wang, Hongzhi
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Camouflage and Display for Soft Machines
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- Morin, S. A.; Shepherd, R. F.; Kwok, S. W.
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