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Title: Event-based processing of neutron scattering data at the Spallation Neutron Source

Abstract

Here, the Spallation Neutron Source at Oak Ridge National Laboratory, USA, ushered in a new era of neutron scattering experiments through the use of event-based data. Tagging each neutron event allows pump–probe experiments, measurements with a parameter asynchronous to the source, measurements with continuously varying parameters and novel ways of testing instrument components. This contribution will focus on a few examples. A pulsed magnet has been used to study diffraction under extreme fields. Continuous ramping of temperature is becoming standard on the POWGEN diffractometer. Battery degradation and phase transformations under heat and stress are often studied on the VULCAN diffractometer. Supercooled Al2O3 was studied on NOMAD. A study of a metallic glass through its glass transition was performed on the ARCS spectrometer, and the effect of source variation on chopper stability was studied for the SEQUOIA spectrometer. Besides a summary of these examples, an overview is provided of the hardware and software advances to enable these and many other event-based measurements.

Authors:
ORCiD logo [1]; ORCiD logo [1];  [2]; ORCiD logo [3];  [1]; ORCiD logo [4]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1];  [1]; ORCiD logo [1]; ORCiD logo [1]; ORCiD logo [1]
  1. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  2. California Inst. of Technology (CalTech), Pasadena, CA (United States)
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Paul Scherrer Inst. (PSI), Villigen (Switzerland)
  4. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Cornell Univ., Ithaca, NY (United States)
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE
OSTI Identifier:
1460232
Grant/Contract Number:  
AC05-00OR22725
Resource Type:
Accepted Manuscript
Journal Name:
Journal of Applied Crystallography (Online)
Additional Journal Information:
Journal Name: Journal of Applied Crystallography (Online); Journal Volume: 51; Journal Issue: 3; Journal ID: ISSN 1600-5767
Publisher:
International Union of Crystallography
Country of Publication:
United States
Language:
English
Subject:
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS; neutron diffraction; stroboscopic experiments; event-based data processing; spectroscopy

Citation Formats

Granroth, Garrett E., An, Ke, Smith, Hillary L., Whitfield, Pamela S., Neuefeind, Joerg C., Lee, Jooseop, Zhou, Wenduo, Sedov, Vladislav N., Peterson, Peter F., Parizzi, Andre A., Skorpenske, Harley David, Hartman, Steven M., Huq, Ashfia, and Abernathy, Douglas L. Event-based processing of neutron scattering data at the Spallation Neutron Source. United States: N. p., 2018. Web. doi:10.1107/S1600576718004727.
Granroth, Garrett E., An, Ke, Smith, Hillary L., Whitfield, Pamela S., Neuefeind, Joerg C., Lee, Jooseop, Zhou, Wenduo, Sedov, Vladislav N., Peterson, Peter F., Parizzi, Andre A., Skorpenske, Harley David, Hartman, Steven M., Huq, Ashfia, & Abernathy, Douglas L. Event-based processing of neutron scattering data at the Spallation Neutron Source. United States. https://doi.org/10.1107/S1600576718004727
Granroth, Garrett E., An, Ke, Smith, Hillary L., Whitfield, Pamela S., Neuefeind, Joerg C., Lee, Jooseop, Zhou, Wenduo, Sedov, Vladislav N., Peterson, Peter F., Parizzi, Andre A., Skorpenske, Harley David, Hartman, Steven M., Huq, Ashfia, and Abernathy, Douglas L. Fri . "Event-based processing of neutron scattering data at the Spallation Neutron Source". United States. https://doi.org/10.1107/S1600576718004727. https://www.osti.gov/servlets/purl/1460232.
@article{osti_1460232,
title = {Event-based processing of neutron scattering data at the Spallation Neutron Source},
author = {Granroth, Garrett E. and An, Ke and Smith, Hillary L. and Whitfield, Pamela S. and Neuefeind, Joerg C. and Lee, Jooseop and Zhou, Wenduo and Sedov, Vladislav N. and Peterson, Peter F. and Parizzi, Andre A. and Skorpenske, Harley David and Hartman, Steven M. and Huq, Ashfia and Abernathy, Douglas L.},
abstractNote = {Here, the Spallation Neutron Source at Oak Ridge National Laboratory, USA, ushered in a new era of neutron scattering experiments through the use of event-based data. Tagging each neutron event allows pump–probe experiments, measurements with a parameter asynchronous to the source, measurements with continuously varying parameters and novel ways of testing instrument components. This contribution will focus on a few examples. A pulsed magnet has been used to study diffraction under extreme fields. Continuous ramping of temperature is becoming standard on the POWGEN diffractometer. Battery degradation and phase transformations under heat and stress are often studied on the VULCAN diffractometer. Supercooled Al2O3 was studied on NOMAD. A study of a metallic glass through its glass transition was performed on the ARCS spectrometer, and the effect of source variation on chopper stability was studied for the SEQUOIA spectrometer. Besides a summary of these examples, an overview is provided of the hardware and software advances to enable these and many other event-based measurements.},
doi = {10.1107/S1600576718004727},
journal = {Journal of Applied Crystallography (Online)},
number = 3,
volume = 51,
place = {United States},
year = {Fri May 18 00:00:00 EDT 2018},
month = {Fri May 18 00:00:00 EDT 2018}
}

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Figures / Tables:

Fig. 1 Fig. 1: A timing diagram for a diffractometer with the sample position at 20 m from the source and the detectors at 25 m from the source. Note that the crystal at the sample selects some wavelengths and not others. Furthermore there is a time difference between when neutrons ofmore » a given wavelength are at the sample and when they are at the detector.« less

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Works referenced in this record:

Mantid—Data analysis and visualization package for neutron scattering and μ SR experiments
journal, November 2014

  • Arnold, O.; Bilheux, J. C.; Borreguero, J. M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 764
  • DOI: 10.1016/j.nima.2014.07.029

First Results from the VULCAN Diffractometer at the SNS
journal, May 2010


First In Situ Lattice Strains Measurements Under Load at VULCAN
journal, October 2010

  • An, Ke; Skorpenske, Harley D.; Stoica, Alexandru D.
  • Metallurgical and Materials Transactions A, Vol. 42, Issue 1
  • DOI: 10.1007/s11661-010-0495-9

SEQUOIA: A Newly Operating Chopper Spectrometer at the SNS
journal, November 2010


In-situ TOF neutron diffraction studies of cyclic softening in superelasticity of a NiFeGaCo shape memory alloy
journal, January 2017


Phase-Transformation Ductilization of Brittle High-Entropy Alloys via Metastability Engineering
journal, June 2017


A study of suppressed formation of low-conductivity phases in doped Li 7 La 3 Zr 2 O 12 garnets by in situ neutron diffraction
journal, January 2015

  • Chen, Yan; Rangasamy, Ezhiylmurugan; dela Cruz, Clarina R.
  • Journal of Materials Chemistry A, Vol. 3, Issue 45
  • DOI: 10.1039/C5TA04902D

A review of in situ and/or time resolved neutron scattering
journal, September 2007


Liquid Alumina: Detailed Atomic Coordination Determined from Neutron Diffraction Data Using Empirical Potential Structure Refinement
journal, May 2001


Beating Crystallization in Glass-Forming Metals by Millisecond Heating and Processing
journal, May 2011


A study of stress-induced phase transformation and micromechanical behavior of CuZr-based alloy by in-situ neutron diffraction
journal, March 2017


Time resolved studies on a millisecond time scale by elastic neutron scattering: transient properties of the ferroelectric phase transition in Rb2ZnCl4
journal, August 1994

  • Steigenberger, U.; Eckold, G.; Hagen, M.
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 93, Issue 3
  • DOI: 10.1016/0168-583X(94)95481-X

Visualizing the chemistry and structure dynamics in lithium-ion batteries by in-situ neutron diffraction
journal, October 2012

  • Wang, Xun-Li; An, Ke; Cai, Lu
  • Scientific Reports, Vol. 2, Issue 1
  • DOI: 10.1038/srep00747

Unraveling structural evolution of LiNi0.5Mn1.5O4 by in situ neutron diffraction
journal, January 2013

  • Cai, Lu; Liu, Zengcai; An, Ke
  • Journal of Materials Chemistry A, Vol. 1, Issue 23
  • DOI: 10.1039/c3ta00145h

In-situ neutron diffraction of LaCoO 3 perovskite under uniaxial compression. I. Crystal structure analysis and texture development
journal, July 2014

  • Aman, Amjad; Chen, Yan; Lugovy, Mykola
  • Journal of Applied Physics, Vol. 116, Issue 1
  • DOI: 10.1063/1.4884335

Towards neutron scattering experiments with sub-millisecond time resolution
journal, January 2015

  • Adlmann, F. A.; Gutfreund, P.; Ankner, J. F.
  • Journal of Applied Crystallography, Vol. 48, Issue 1
  • DOI: 10.1107/S1600576714027848

In-situ observation of inhomogeneous degradation in large format Li-ion cells by neutron diffraction
journal, August 2013


Structure and Dynamics of Octamethyl-POSS Nanoparticles
journal, February 2014

  • Jalarvo, Niina; Gourdon, Olivier; Ehlers, Georg
  • The Journal of Physical Chemistry C, Vol. 118, Issue 10
  • DOI: 10.1021/jp412228r

A table-top, repetitive pulsed magnet for nonlinear and ultrafast spectroscopy in high magnetic fields up to 30 T
journal, December 2013

  • Noe, G. Timothy; Nojiri, Hiroyuki; Lee, Joseph
  • Review of Scientific Instruments, Vol. 84, Issue 12
  • DOI: 10.1063/1.4850675

Millisecond time resolution neutron reflection from a nematic liquid crystal
journal, September 2004

  • Dalgliesh, R. M.; Lau, Y. G. J.; Richardson, R. M.
  • Review of Scientific Instruments, Vol. 75, Issue 9
  • DOI: 10.1063/1.1783596

Event-based processing of neutron scattering data
journal, December 2015

  • Peterson, Peter F.; Campbell, Stuart I.; Reuter, Michael A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 803
  • DOI: 10.1016/j.nima.2015.09.016

In situ neutron diffraction study of twin reorientation and pseudoplastic strain in Ni–Mn–Ga single crystals
journal, September 2011


Measurements of liquid and glass structures using aerodynamic levitation and in-situ high energy x-ray and neutron scattering
journal, January 2014


Field-induced reentrant magnetoelectric phase in LiNiPO 4
journal, February 2017


The Spallation Neutron Source in Oak Ridge: A powerful tool for materials research
journal, November 2006


Development of a readout system employing high-speed network for J-PARC
journal, February 2009

  • Satoh, S.; Muto, S.; Kaneko, N.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 600, Issue 1
  • DOI: 10.1016/j.nima.2008.11.054

Long Range Charge Ordering in Magnetite Below the Verwey Transition
journal, December 2001


α-Phase transformation kinetics of U – 8 wt% Mo established by in situ neutron diffraction
journal, August 2016


Visualizing the Structural Evolution of LSM/xYSZ Composite Cathodes for SOFC by in-situ Neutron Diffraction
journal, June 2014

  • Chen, Yan; Yang, Ling; Ren, Fei
  • Scientific Reports, Vol. 4, Issue 1
  • DOI: 10.1038/srep05179

Investigation of deformation dynamics in a wrought magnesium alloy
journal, November 2014


TOPAS and TOPAS-Academic : an optimization program integrating computer algebra and crystallographic objects written in C++
journal, February 2018


The Nanoscale Ordered MAterials Diffractometer NOMAD at the Spallation Neutron Source SNS
journal, September 2012

  • Neuefeind, Jörg; Feygenson, Mikhail; Carruth, John
  • Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 287
  • DOI: 10.1016/j.nimb.2012.05.037

Corelli: Efficient single crystal diffraction with elastic discrimination
journal, October 2008


Non-Contact Thermophysical Property Measurements of Liquid and Undercooled Alumina
journal, April 2004

  • Paradis, Paul-Francois; Ishikawa, Takehiko; Saita, Yutaka
  • Japanese Journal of Applied Physics, Vol. 43, Issue 4A
  • DOI: 10.1143/JJAP.43.1496

The Spallation Neutron Source accelerator system design
journal, November 2014

  • Henderson, S.; Abraham, W.; Aleksandrov, A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 763
  • DOI: 10.1016/j.nima.2014.03.067

Separating the configurational and vibrational entropy contributions in metallic glasses
journal, May 2017

  • Smith, Hillary L.; Li, Chen W.; Hoff, Andrew
  • Nature Physics, Vol. 13, Issue 9
  • DOI: 10.1038/nphys4142

Recent Developments in the Chemistry of Cubic Polyhedral Oligosilsesquioxanes
journal, April 2010

  • Cordes, David B.; Lickiss, Paul D.; Rataboul, Franck
  • Chemical Reviews, Vol. 110, Issue 4
  • DOI: 10.1021/cr900201r

Design and operation of the wide angular-range chopper spectrometer ARCS at the Spallation Neutron Source
journal, January 2012

  • Abernathy, D. L.; Stone, M. B.; Loguillo, M. J.
  • Review of Scientific Instruments, Vol. 83, Issue 1
  • DOI: 10.1063/1.3680104

SEQUOIA: A fine resolution chopper spectrometer at the SNS
journal, November 2006


Kinetics of phase transitions in modulated ferroelectrics: Time-resolved neutron diffraction from Rb 2 ZnCl 4
journal, October 1998


Miniature pulsed magnet system for synchrotron x-ray measurements
journal, July 2008

  • van der Linden, Peter J. E. M.; Mathon, Olivier; Strohm, Cornelius
  • Review of Scientific Instruments, Vol. 79, Issue 7
  • DOI: 10.1063/1.2949873

Dynamical structure factor and frequency distribution of the metallic glass Cu 46 Zr 54 at room temperature
journal, March 1980

  • Suck, J. -B; Rudin, H.; Guntherodt, H. -J
  • Journal of Physics C: Solid State Physics, Vol. 13, Issue 8
  • DOI: 10.1088/0022-3719/13/8/006

Unraveling cyclic deformation mechanisms of a rolled magnesium alloy using in situ neutron diffraction
journal, February 2015


Operando Lithium Dynamics in the Li-Rich Layered Oxide Cathode Material via Neutron Diffraction
journal, January 2016


A portable high-field pulsed-magnet system for single-crystal x-ray scattering studies
journal, November 2009

  • Islam, Zahirul; Ruff, Jacob P. C.; Nojiri, Hiroyuki
  • Review of Scientific Instruments, Vol. 80, Issue 11
  • DOI: 10.1063/1.3251273

Deformation dynamics study of a wrought magnesium alloy by real-time in situ neutron diffraction
journal, September 2013


Electronic Conduction of Magnetite (Fe3O4) and its Transition Point at Low Temperatures
journal, August 1939


Understanding low-cycle fatigue life improvement mechanisms in a pre-twinned magnesium alloy
journal, January 2016


Long Range Charge Ordering in Magnetite Below the Verwey Transition
text, January 2001

  • Attfield, J. P.; Radaelli, P. G.; Wright, J. P.
  • The American Physical Society
  • DOI: 10.17877/de290r-4770

Long Range Charge Ordering in Magnetite Below the Verwey Transition
text, January 2001


Works referencing / citing this record:

Time filtering of event based neutron scattering data: A pathway to study the dynamic structural responses of materials
journal, September 2018

  • Fancher, C. M.; Hoffmann, C.; Sedov, V.
  • Review of Scientific Instruments, Vol. 89, Issue 9
  • DOI: 10.1063/1.5031798

RHEGAL: Resistive heating gas enclosure loadframe for in situ neutron scattering
journal, September 2018

  • An, Ke; Armitage, Douglas P.; Yu, Zhenzhen
  • Review of Scientific Instruments, Vol. 89, Issue 9
  • DOI: 10.1063/1.5033566

A suite-level review of the neutron powder diffraction instruments at Oak Ridge National Laboratory
journal, September 2018

  • Calder, S.; An, K.; Boehler, R.
  • Review of Scientific Instruments, Vol. 89, Issue 9
  • DOI: 10.1063/1.5033906

Probing orientation information using 3-dimensional reciprocal space volume analysis
journal, January 2019

  • Fancher, C. M.; Hoffmann, C. M.; Frontzek, M. D.
  • Review of Scientific Instruments, Vol. 90, Issue 1
  • DOI: 10.1063/1.5034135

Advances in utilizing event based data structures for neutron scattering experiments
journal, September 2018

  • Peterson, Peter F.; Olds, Daniel; Savici, Andrei T.
  • Review of Scientific Instruments, Vol. 89, Issue 9
  • DOI: 10.1063/1.5034782

Preface: Special Topic on Advances in Modern Neutron Diffraction at Oak Ridge National Laboratory
journal, September 2018

  • Page, Katharine; Haberl, Bianca; Coates, Leighton
  • Review of Scientific Instruments, Vol. 89, Issue 9
  • DOI: 10.1063/1.5055785

Foreword to the special issue on advanced neutron scattering instrumentation
journal, June 2018


Deep learning-based super-resolution for small-angle neutron scattering data: attempt to accelerate experimental workflow
journal, January 2020

  • Chang, Ming-Ching; Wei, Yi; Chen, Wei-Ren
  • MRS Communications, Vol. 10, Issue 1
  • DOI: 10.1557/mrc.2019.166

Bending Behavior of a Wrought Magnesium Alloy Investigated by the In Situ Pinhole Neutron Diffraction Method
journal, August 2018