Anisotropic magnetic properties of the triangular plane lattice material TmMgGaO4

Cevallos, F. Alex; Stolze, Karoline; Kong, Tai; Cava, R. J.

doi:10.1016/j.materresbull.2018.04.042

Title: Anisotropic magnetic properties of the triangular plane lattice material TmMgGaO₄

Abstract

Here, the crystal growth, structure, and basic magnetic properties of TmMgGaO₄ are reported. The Tm ions are located in a planar triangular lattice consisting of distorted TmO6 octahedra, while the Mg and Ga atoms randomly occupy intermediary bilayers of M-O triangular bipyramids. The Tm ions are positionally disordered. The material displays an antiferromagnetic Curie Weiss theta of ~ -20 -25 K, with no clear ordering visible in the magnetic susceptibility down to 1.8 K; the structure and magnetic properties suggest that ordering of the magnetic moments is frustrated by both structural disorder and the triangular magnetic motif. Single crystal magnetization measurements indicate that the magnetic properties are highly anisotropic, with large moments measured perpendicular to the triangular planes. At 2 K, a broad step-like feature is seen in the field-dependent magnetization perpendicular to the plane on applied field near 2 Tesla.

Authors:

Cevallos, F. Alex ^[1]; Stolze, Karoline ^[1]; Kong, Tai ^[1]; Cava, R. J. ^[1]

Princeton Univ., Princeton, NJ (United States)

Publication Date:: Mon Apr 30 00:00:00 EDT 2018

Research Org.:: Princeton Univ., NJ (United States)

Sponsoring Org.:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

OSTI Identifier:: 1441198

Grant/Contract Number:: FG02-08ER46544

Resource Type:: Accepted Manuscript

Journal Name:: Materials Research Bulletin

Additional Journal Information:: Journal Volume: 105; Journal Issue: C; Journal ID: ISSN 0025-5408

Publisher:: Elsevier

Country of Publication:: United States

Language:: English

Subject:: 36 MATERIALS SCIENCE; A. Magnetic materials; A. Layered compounds; A. Oxides

Citation Formats


                    Cevallos, F. Alex, Stolze, Karoline, Kong, Tai, and Cava, R. J. Anisotropic magnetic properties of the triangular plane lattice material TmMgGaO4.  United States: N. p., 2018. 
Web.  doi:10.1016/j.materresbull.2018.04.042.

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                    Cevallos, F. Alex, Stolze, Karoline, Kong, Tai, & Cava, R. J. Anisotropic magnetic properties of the triangular plane lattice material TmMgGaO4.  United States.  https://doi.org/10.1016/j.materresbull.2018.04.042

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                    Cevallos, F. Alex, Stolze, Karoline, Kong, Tai, and Cava, R. J. Mon .  
"Anisotropic magnetic properties of the triangular plane lattice material TmMgGaO4".  United States.  https://doi.org/10.1016/j.materresbull.2018.04.042.  https://www.osti.gov/servlets/purl/1441198.

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@article{osti_1441198,

  title        = {Anisotropic magnetic properties of the triangular plane lattice material TmMgGaO4},

  author       = {Cevallos, F. Alex and Stolze, Karoline and Kong, Tai and Cava, R. J.},

  abstractNote = {Here, the crystal growth, structure, and basic magnetic properties of TmMgGaO4 are reported. The Tm ions are located in a planar triangular lattice consisting of distorted TmO6 octahedra, while the Mg and Ga atoms randomly occupy intermediary bilayers of M-O triangular bipyramids. The Tm ions are positionally disordered. The material displays an antiferromagnetic Curie Weiss theta of ~ -20 -25 K, with no clear ordering visible in the magnetic susceptibility down to 1.8 K; the structure and magnetic properties suggest that ordering of the magnetic moments is frustrated by both structural disorder and the triangular magnetic motif. Single crystal magnetization measurements indicate that the magnetic properties are highly anisotropic, with large moments measured perpendicular to the triangular planes. At 2 K, a broad step-like feature is seen in the field-dependent magnetization perpendicular to the plane on applied field near 2 Tesla.},

  doi          = {10.1016/j.materresbull.2018.04.042},

  journal      = {Materials Research Bulletin},

  number       = C,

  volume       = 105,

  place        = {United States},

  year         = {Mon Apr 30 00:00:00 EDT 2018},

  month        = {Mon Apr 30 00:00:00 EDT 2018}

}

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https://doi.org/10.1016/j.materresbull.2018.04.042

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Cited by: 21 works

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Figures / Tables:

Figure 1: Powder Rietveld refinement of TmMgGaO₄. Inset: A small, colorless transparent single crystal of TmMgGaO₄ on a 1-mm grid.

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Works referenced in this record:

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Works referencing / citing this record:

Intertwined dipolar and multipolar order in the triangular-lattice magnet TmMgGaO4
journal, October 2019

Shen, Yao; Liu, Changle; Qin, Yayuan
Nature Communications, Vol. 10, Issue 1
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Anisotropic-Exchange Magnets on a Triangular Lattice: Spin Waves, Accidental Degeneracies, and Dual Spin Liquids
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Intrinsic transverse field in frustrated quantum Ising magnets: Physical origin and quantum effects
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Chen, Gang
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Intertwined dipolar and multipolar order in the triangular-lattice magnet TmMgGaO$_4$
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Shen, Yao; Liu, Changle; Qin, Yayuan
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Shen, Yao; Liu, Changle; Qin, Yayuan
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Kosterlitz-Thouless Melting of Magnetic Order in the Triangular Quantum Ising Material TmMgGaO$_4$
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Li, Han; Da Liao, Yuan; Chen, Bin-Bin
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Title: Anisotropic magnetic properties of the triangular plane lattice material TmMgGaO4

Abstract

Citation Formats

Figures / Tables:

Strongly Geometrically Frustrated Magnets journal, August 1994

Geometrical frustration journal, February 2006

Spin liquids in frustrated magnets journal, March 2010

Compounds with the YbFe2O4Structure Type: Frustrated Magnetism and Spin-Glass Behavior journal, November 1998

Quasi-two-dimensional spin correlations in the triangular lattice bilayer spin glass LuCoGaO 4 journal, September 2017

Crystal growth, structure and magnetic behavior of ytterbium cobalt gallium oxide YbCoGaO4 journal, January 2002

Magnetization of Single Crystal YFeMnO 4 journal, December 1990

Helical scattering signatures of strain and electronic textures in YbFe 2 O 4 from three-dimensional reciprocal-space imaging journal, January 2012

Anisotropic giant dielectric tunability in electronic ferroelectric YbFe2O4 journal, August 2010

Ferroelectric properties of triangular charge-frustrated LuFe 2 O 4 journal, October 2008

Charge-Stripe Order in the Electronic Ferroelectric LuFe 2 O 4 journal, June 2007

Die Kristallstruktur von YbFe 2 O 4 journal, August 1975

Rare-Earth Triangular Lattice Spin Liquid: A Single-Crystal Study of YbMgGaO 4 journal, October 2015

Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4 journal, December 2016

Crystalline Electric-Field Randomness in the Triangular Lattice Spin-Liquid YbMgGaO 4 journal, March 2017

Gapless quantum spin liquid ground state in the two-dimensional spin-1/2 triangular antiferromagnet YbMgGaO4 journal, November 2015

Evidence for a spinon Fermi surface in a triangular-lattice quantum-spin-liquid candidate journal, December 2016

Disorder-Induced Mimicry of a Spin Liquid in YbMgGaO 4 journal, October 2017

Ln(GaM2+)O4 and Ln(AlMn2+)O4 compounds having a layer structure [Ln = Lu, Yb, Tm, Er, Ho, and Y, and M = Mg, Mn, Co, Cu, and Zn] journal, February 1982

Spinel, YbFe2O4, and Yb2Fe3O7 types of structures for compounds in the In2O3 and Sc2O3A2O3BO systems [A: Fe, Ga, or Al; B: Mg, Mn, Fe, Ni, Cu, or Zn] at temperatures over 1000°C journal, December 1985

Field-Induced Order and Spin Waves in the Pyrochlore Antiferromagnet Tb 2 Ti 2 O 7 journal, May 2006

Crystalline electric field effects on the paramagnetic susceptibility of polycrystalline materials journal, June 1983

NaSrMn 2 F 7 , NaCaFe 2 F 7 , and NaSrFe 2 F 7 : novel single crystal pyrochlore antiferromagnets journal, November 2016

NaCaN i 2 F 7 : A frustrated high-temperature pyrochlore antiferromagnet with S = 1 N i 2 + journal, July 2015

NaCaCo 2 F 7 : A single-crystal high-temperature pyrochlore antiferromagnet journal, June 2014

Spin Freezing in Geometrically Frustrated Antiferromagnets with Weak Disorder journal, April 2007

Spin-glass transition in geometrically frustrated antiferromagnets with weak disorder journal, January 2010

Liquidlike correlations in single-crystalline Y 2 Mo 2 O 7 : An unconventional spin glass journal, February 2014

Intertwined dipolar and multipolar order in the triangular-lattice magnet TmMgGaO4 journal, October 2019

Anisotropic-Exchange Magnets on a Triangular Lattice: Spin Waves, Accidental Degeneracies, and Dual Spin Liquids journal, April 2019

Robustness of entropy plateaus: A case study of triangular Ising antiferromagnets journal, August 2019

Intrinsic transverse field in frustrated quantum Ising magnets: Physical origin and quantum effects journal, December 2019

Intertwined dipolar and multipolar order in the triangular-lattice magnet TmMgGaO$_4$ text, January 2018

Anisotropic-Exchange Magnets on a Triangular Lattice: Spin Waves, Accidental Degeneracies, and Dual Spin Liquids text, January 2018

Intertwined dipolar and multipolar order in the triangular-lattice magnet TmMgGaO4 journal, October 2019

Kosterlitz-Thouless Melting of Magnetic Order in the Triangular Quantum Ising Material TmMgGaO$_4$ text, January 2019

Title: Anisotropic magnetic properties of the triangular plane lattice material TmMgGaO₄

Strongly Geometrically Frustrated Magnets
journal, August 1994

Geometrical frustration
journal, February 2006

Spin liquids in frustrated magnets
journal, March 2010

Compounds with the YbFe2O4Structure Type: Frustrated Magnetism and Spin-Glass Behavior
journal, November 1998

Quasi-two-dimensional spin correlations in the triangular lattice bilayer spin glass ${LuCoGaO}_{4}$
journal, September 2017

Crystal growth, structure and magnetic behavior of ytterbium cobalt gallium oxide YbCoGaO4
journal, January 2002

Magnetization of Single Crystal YFeMnO ₄
journal, December 1990

Helical scattering signatures of strain and electronic textures in YbFe $_{2}$ O $_{4}$ from three-dimensional reciprocal-space imaging
journal, January 2012

Anisotropic giant dielectric tunability in electronic ferroelectric YbFe2O4
journal, August 2010

Ferroelectric properties of triangular charge-frustrated LuFe ₂ O ₄
journal, October 2008

Charge-Stripe Order in the Electronic Ferroelectric ${LuFe}_{2} O_{4}$
journal, June 2007

Die Kristallstruktur von YbFe ₂ O ₄
journal, August 1975

Rare-Earth Triangular Lattice Spin Liquid: A Single-Crystal Study of ${YbMgGaO}_{4}$
journal, October 2015

Continuous excitations of the triangular-lattice quantum spin liquid YbMgGaO4
journal, December 2016

Crystalline Electric-Field Randomness in the Triangular Lattice Spin-Liquid ${YbMgGaO}_{4}$
journal, March 2017

Gapless quantum spin liquid ground state in the two-dimensional spin-1/2 triangular antiferromagnet YbMgGaO4
journal, November 2015

Evidence for a spinon Fermi surface in a triangular-lattice quantum-spin-liquid candidate
journal, December 2016

Disorder-Induced Mimicry of a Spin Liquid in ${YbMgGaO}_{4}$
journal, October 2017

Ln(GaM2+)O4 and Ln(AlMn2+)O4 compounds having a layer structure [Ln = Lu, Yb, Tm, Er, Ho, and Y, and M = Mg, Mn, Co, Cu, and Zn]
journal, February 1982

Spinel, YbFe2O4, and Yb2Fe3O7 types of structures for compounds in the In2O3 and Sc2O3A2O3BO systems [A: Fe, Ga, or Al; B: Mg, Mn, Fe, Ni, Cu, or Zn] at temperatures over 1000°C
journal, December 1985

Field-Induced Order and Spin Waves in the Pyrochlore Antiferromagnet ${Tb}_{2} {Ti}_{2} O_{7}$
journal, May 2006

Crystalline electric field effects on the paramagnetic susceptibility of polycrystalline materials
journal, June 1983

NaSrMn ₂ F ₇ , NaCaFe ₂ F ₇ , and NaSrFe ₂ F ₇ : novel single crystal pyrochlore antiferromagnets
journal, November 2016

$NaCaN i_{2} F_{7}$ : A frustrated high-temperature pyrochlore antiferromagnet with $S = 1 N i^{2 +}$
journal, July 2015

${NaCaCo}_{2} F_{7}$ : A single-crystal high-temperature pyrochlore antiferromagnet
journal, June 2014

Spin Freezing in Geometrically Frustrated Antiferromagnets with Weak Disorder
journal, April 2007

Spin-glass transition in geometrically frustrated antiferromagnets with weak disorder
journal, January 2010

Liquidlike correlations in single-crystalline Y $_{2}$ Mo $_{2}$ O $_{7}$ : An unconventional spin glass
journal, February 2014

Intertwined dipolar and multipolar order in the triangular-lattice magnet TmMgGaO4
journal, October 2019

Anisotropic-Exchange Magnets on a Triangular Lattice: Spin Waves, Accidental Degeneracies, and Dual Spin Liquids
journal, April 2019

Robustness of entropy plateaus: A case study of triangular Ising antiferromagnets
journal, August 2019

Intrinsic transverse field in frustrated quantum Ising magnets: Physical origin and quantum effects
journal, December 2019

Intertwined dipolar and multipolar order in the triangular-lattice magnet TmMgGaO$_4$
text, January 2018

Anisotropic-Exchange Magnets on a Triangular Lattice: Spin Waves, Accidental Degeneracies, and Dual Spin Liquids
text, January 2018

Intertwined dipolar and multipolar order in the triangular-lattice magnet TmMgGaO4
journal, October 2019

Kosterlitz-Thouless Melting of Magnetic Order in the Triangular Quantum Ising Material TmMgGaO$_4$
text, January 2019