DOE PAGES title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Using anisotropies in prompt fission neutron coincidences to assess the neutron multiplication of highly multiplying subcritical plutonium assemblies

Abstract

There is a significant and well-known anisotropy between the prompt neutrons emitted from a single fission event; these neutrons are most likely to be observed at angles near 0° or 180° relative to each other. However, the propagation of this anisotropy through different generations of a fission chain re-action has not been previously studied. We have measured this anisotropy in neutron–neutron coincidences from a subcritical highly-multiplying assembly of plutonium metal. The assembly was a 4.5 kg α-phase plutonium metal sphere composed of 94% 239Pu and 6% 240Pu by mass. Data were collected using two EJ-309 liquid scintillators and two EJ-299 plastic scintillators. The angular distribution of neutron–neutron coincidences was measured at 90° and 180° and found to be largely isotropic. Simulations were performed using MCNPX-PoliMi of similar plutonium metal spheres of varying sizes and a correlation between the neutron multiplication of the assembly and the anisotropy of neutron–neutron coincidences was observed. In principle, this correlation could be used to assess the neutron multi-plication of an unknown assembly.

Authors:
 [1];  [1]
  1. North Carolina State University, Raleigh, NC (United States)
Publication Date:
Research Org.:
North Carolina State University, Raleigh, NC (United States); Univ. of Michigan, Ann Arbor, MI (United States); CNEC/North Carolina State University, Raleigh, NC (United States)
Sponsoring Org.:
USDOE National Nuclear Security Administration (NNSA), Office of Defense Nuclear Nonproliferation
OSTI Identifier:
1438391
Alternate Identifier(s):
OSTI ID: 1359655; OSTI ID: 1367549; OSTI ID: 1437438; OSTI ID: 1487109
Grant/Contract Number:  
NA0002576; NA0002534
Resource Type:
Accepted Manuscript
Journal Name:
Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment
Additional Journal Information:
Journal Volume: 825; Journal Issue: C; Journal ID: ISSN 0168-9002
Publisher:
Elsevier
Country of Publication:
United States
Language:
English
Subject:
73 NUCLEAR PHYSICS AND RADIATION PHYSICS; passive interrogation; plutonium; nonproliferation; special nuclear material; neutron angular anisotropy; neutron detectors

Citation Formats

Mueller, Jonathan M., and Mattingly, J. Using anisotropies in prompt fission neutron coincidences to assess the neutron multiplication of highly multiplying subcritical plutonium assemblies. United States: N. p., 2016. Web. doi:10.1016/j.nima.2016.04.027.
Mueller, Jonathan M., & Mattingly, J. Using anisotropies in prompt fission neutron coincidences to assess the neutron multiplication of highly multiplying subcritical plutonium assemblies. United States. https://doi.org/10.1016/j.nima.2016.04.027
Mueller, Jonathan M., and Mattingly, J. Sat . "Using anisotropies in prompt fission neutron coincidences to assess the neutron multiplication of highly multiplying subcritical plutonium assemblies". United States. https://doi.org/10.1016/j.nima.2016.04.027. https://www.osti.gov/servlets/purl/1438391.
@article{osti_1438391,
title = {Using anisotropies in prompt fission neutron coincidences to assess the neutron multiplication of highly multiplying subcritical plutonium assemblies},
author = {Mueller, Jonathan M. and Mattingly, J.},
abstractNote = {There is a significant and well-known anisotropy between the prompt neutrons emitted from a single fission event; these neutrons are most likely to be observed at angles near 0° or 180° relative to each other. However, the propagation of this anisotropy through different generations of a fission chain re-action has not been previously studied. We have measured this anisotropy in neutron–neutron coincidences from a subcritical highly-multiplying assembly of plutonium metal. The assembly was a 4.5 kg α-phase plutonium metal sphere composed of 94% 239Pu and 6% 240Pu by mass. Data were collected using two EJ-309 liquid scintillators and two EJ-299 plastic scintillators. The angular distribution of neutron–neutron coincidences was measured at 90° and 180° and found to be largely isotropic. Simulations were performed using MCNPX-PoliMi of similar plutonium metal spheres of varying sizes and a correlation between the neutron multiplication of the assembly and the anisotropy of neutron–neutron coincidences was observed. In principle, this correlation could be used to assess the neutron multi-plication of an unknown assembly.},
doi = {10.1016/j.nima.2016.04.027},
journal = {Nuclear Instruments and Methods in Physics Research. Section A, Accelerators, Spectrometers, Detectors and Associated Equipment},
number = C,
volume = 825,
place = {United States},
year = {Sat Apr 09 00:00:00 EDT 2016},
month = {Sat Apr 09 00:00:00 EDT 2016}
}

Journal Article:

Citation Metrics:
Cited by: 11 works
Citation information provided by
Web of Science

Figures / Tables:

Figure 1 Figure 1: The experimental setup used to measure neutrons from the BeRP ball.

Save / Share:

Works referenced in this record:

Calculation of fission observables through event-by-event simulation
journal, August 2009


The Energy Dependence of Fission Fragment Anisotropy in Fast-Neutron-Induced Fission of Uranium-235
journal, August 1979

  • Ahmad, S.; Islam, M. M.; Khan, A. H.
  • Nuclear Science and Engineering, Vol. 71, Issue 2
  • DOI: 10.13182/NSE79-A20413

Neutron-neutron angular correlations in spontaneous fission of 252Cf
journal, June 2008

  • Gagarski, A. M.; Guseva, I. S.; Sokolov, V. E.
  • Bulletin of the Russian Academy of Sciences: Physics, Vol. 72, Issue 6
  • DOI: 10.3103/S1062873808060130

Measurements of angular and energy distributions of prompt neutrons from thermal neutron-induced fission
journal, January 2009

  • Vorobyev, A. S.; Shcherbakov, O. A.; Pleva, Yu. S.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 598, Issue 3
  • DOI: 10.1016/j.nima.2008.10.017

New Standard Evaluated Neutron Cross Section Libraries for the GEANT4 Code and First Verification
journal, August 2014

  • Mendoza, Emilio; Cano-Ott, Daniel; Koi, Tatsumi
  • IEEE Transactions on Nuclear Science, Vol. 61, Issue 4
  • DOI: 10.1109/TNS.2014.2335538

Geant4 developments and applications
journal, February 2006

  • Allison, J.; Amako, K.; Apostolakis, J.
  • IEEE Transactions on Nuclear Science, Vol. 53, Issue 1
  • DOI: 10.1109/TNS.2006.869826

A zero-knowledge protocol for nuclear warhead verification
journal, June 2014

  • Glaser, Alexander; Barak, Boaz; Goldston, Robert J.
  • Nature, Vol. 510, Issue 7506
  • DOI: 10.1038/nature13457

Neutron response characterization for an EJ299-33 plastic scintillation detector
journal, September 2014

  • Lawrence, Chris C.; Febbraro, Michael; Massey, Thomas N.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 759
  • DOI: 10.1016/j.nima.2014.04.062

MCNP-PoliMi: a Monte-Carlo code for correlation measurements
journal, November 2003

  • Pozzi, Sara A.; Padovani, Enrico; Marseguerra, Marzio
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 513, Issue 3
  • DOI: 10.1016/j.nima.2003.06.012

Angular correlation of neutrons from thermal-neutron fission of 235U
journal, October 1978


Models for a three-parameter analysis of neutron signal correlation measurements for fissile material assay
journal, November 1986

  • Cifarelli, D. M.; Hage, W.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 251, Issue 3
  • DOI: 10.1016/0168-9002(86)90651-0

Angular Distribution of Fragments in Fission Induced by Mev Neutrons
journal, October 1960


Pulse shape discrimination in inorganic and organic scintillators. I
journal, August 1971

  • Winyard, R. A.; Lutkin, J. E.; McBeth, G. W.
  • Nuclear Instruments and Methods, Vol. 95, Issue 1, p. 141-153
  • DOI: 10.1016/0029-554X(71)90054-1

Neutron angular correlations in spontaneous and neutron-induced fission
journal, December 2014


Using neutron angular anisotropy information to dynamically determine the ratio of the (α,n) rate to spontaneous fission rate for coincidence counting applications
journal, February 2013

  • Holewa, L.; Charlton, W.; Miller, E.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 701
  • DOI: 10.1016/j.nima.2012.11.026

Angular Correlation of Neutrons from Spontaneous Fission of Cf 252
journal, December 1975


Angular Dependence of Coincidences between Fission Neutrons
journal, December 1948


Correlated Neutron Emissions from 252 Cf
journal, October 2014

  • Pozzi, Sara A.; Wieger, Brian; Enqvist, Andreas
  • Nuclear Science and Engineering, Vol. 178, Issue 2
  • DOI: 10.13182/NSE13-96

Gamma-calibration of NE 213 scintillation counters
journal, March 1982


Works referencing / citing this record:

High resolution measurement of tagged two-neutron energy and angle correlations in Cf 252 (sf)
journal, July 2019


Figures/Tables have been extracted from DOE-funded journal article accepted manuscripts.